ABSTRACT
The interplay between light polarization and matter is the basis of many fundamental physical processes and applications. However, the electromagnetic wave nature of light in free space sets a fundamental limit on the three-dimensional polarization orientation of a light beam. Although a high numerical aperture objective can be used to bend the wavefront of a radially polarized beam to generate the longitudinal polarization state in the focal volume, the arbitrary three-dimensional polarization orientation of a beam has not been achieved yet. Here we present a novel technique for generating arbitrary three-dimensional polarization orientation by a single optically configured vectorial beam. As a consequence, by applying this technique to gold nanorods, orientation-unlimited polarization encryption with ultra-security is demonstrated. These results represent a new landmark of the orientation-unlimited three-dimensional polarization control of the light-matter interaction.
ABSTRACT
This Letter presents a scheme to embed both angular/spectral surface plasmon resonance (SPR) in a unique far-field rainbow feature by tightly focusing (effective NA=1.45) a polychromatic radially polarized beam on an Au (20 nm)/SiO2 (500 nm)/Au (20 nm) sandwich structure. Without the need for angular or spectral scanning, the virtual spectral probe snapshots a wide operation range (n=1-1.42; λ=400-700 nm) of SPR excitation in a locally nanosized region. Combined with the high-speed spectral analysis, a proof-of-concept scenario was given by monitoring the NaCl liquid concentration change in real time. The proposed scheme will certainly has a promising impact on the development of objective-based SPR sensor and biometric studies due to its rapidity and versatility.
ABSTRACT
In this paper, we demonstrated a far-field scheme for the manipulation of locally excited surface plasmon polaritons (SPPs). This scheme features steering and shaping capabilities, and relies on the focusing of a high numerical aperture, in conjunction with spatially inhomogeneous polarized (SIP) illumination. We were able to control the propagation and direction of SPPs, via the field distribution of polarization at the entrance pupil, without the need for an aperture, protrusion or any other near-field features. Depending on the axial position of the focus, the field distribution of excited SPPs revealed either counter-propagating interference or a multi-casting plasmonic source. The results of near-field imaging demonstrated the versatility of the SPPs, showing strong agreement with the predictions made during simulations. Due to the simplicity and versatility of the proposed method, we believe that it could have a significant impact the processes employed in the excitation of a variety of SPPs.