Towards space-deployable laser stabilization systems based on vibration-insensitive cubic cavities with crystalline coatings.

We present the development of a transportable laser frequency stabilization system with application to both optical clocks and a next-generation gravity mission (NGGM) in space. This effort leverages a 5-cm long cubic cavity with crystalline coatings operating at room temperature and with a center wavelength of 1064 nm. The cavity is integrated in a custom vacuum chamber with dedicated low-noise locking electronics. Our vacuum-mounted cavity and control system are well suited for space applications, exhibiting state-of-the-art noise performance while being resilient to radiation exposure, vibration, shock, and temperature variations. Furthermore, we demonstrate a robust means of automatically (re)locking the laser to the cavity when resonance is lost. We show that the mounted cavity is capable of reaching technology readiness level (TRL) 6, paving the way for high-performance ultrastable laser systems and eventually optical atomic clocks amenable to future satellite platforms.

An Artificial Neural Network to Eliminate the Detrimental Spectral Shift on Mid-Infrared Gas Spectroscopy.

We demonstrate the successful implementation of an artificial neural network (ANN) to eliminate detrimental spectral shifts imposed in the measurement of laser absorption spectrometers (LASs). Since LASs rely on the analysis of the spectral characteristics of biological and chemical molecules, their accuracy and precision is especially prone to the presence of unwanted spectral shift in the measured molecular absorption spectrum over the reference spectrum. In this paper, an ANN was applied to a scanning grating-based mid-infrared trace gas sensing system, which suffers from temperature-induced spectral shifts. Using the HITRAN database, we generated synthetic gas absorbance spectra with random spectral shifts for training and validation. The ANN was trained with these synthetic spectra to identify the occurrence of spectral shifts. Our experimental verification unambiguously proves that such an ANN can be an excellent tool to accurately retrieve the gas concentration from imprecise or distorted spectra of gas absorption. Due to the global shift of the measured gas absorption spectrum, the accuracy of the retrieved gas concentration using a typical least-mean-squares fitting algorithm was considerably degraded by 40.3%. However, when the gas concentration of the same measurement dataset was predicted by the proposed multilayer perceptron network, the sensing accuracy significantly improved by reducing the error to less than ±1% while preserving the sensing sensitivity.

Digital OPLL-based distributed Brillouin sensing system in optical fibers.

A digital optical phase-locked loop (OPLL) has been implemented to develop a distributed Brillouin sensing system in optical fibers. In our experiment, two commercial semiconductor lasers are phase-locked to each other with a highly flexible offset frequency using field programmable gate array (FPGA)-based electronics. Then, the difference frequency between the two lasers is highly stabilized and scanned by a desired step frequency in the vicinity of the Brillouin frequency of standard single-mode optical fibers. Consequently, the distribution of Brillouin frequency shift over a 50 km-long sensing fiber has been successfully measured by a very simple and low-cost Brillouin optical time-domain reflectometry (BOTDR) sensing system without any penalty in the sensing performance. The measurement repeatability at 50 km position of sensing fiber with a 5 m spatial resolution was measured be 4.5 MHz under fast measurement conditions: the number of trace averaging of 2000 and the frequency scan step of 12.8 MHz, showing the figure-of-merit of 3.0.

Visible blue-to-red 10 GHz frequency comb via on-chip triple-sum-frequency generation.

A broadband visible (VIS) blue-to-red, 10 GHz repetition rate frequency comb is generated by combined spectral broadening and triple-sum-frequency generation in an on-chip silicon nitride waveguide. Ultra-short pulses of 150 pJ pulse energy, generated via electro-optic modulation of a 1560 nm continuous-wave laser (CW), are coupled to a silicon nitride waveguide giving rise to a broadband near-infrared (NIR) supercontinuum. Modal phase matching inside the waveguide allows direct triple-sum-frequency transfer of the NIR supercontinuum into the VIS wavelength range covering more than 250 THz from below 400 to above 600 nm wavelength. This scheme directly links the mature optical telecommunication band technology to the VIS wavelength band and can find application in astronomical spectrograph calibration, as well as referencing of CW lasers.

Frequency comb up- and down-conversion in synchronously driven χ(2) optical microresonators.

Optical frequency combs are key to optical precision measurements. While most frequency combs operate in the near-infrared (NIR) regime, many applications require combs at mid-infrared (MIR), visible (VIS), or even ultra-violet (UV) wavelengths. Frequency combs can be transferred to other wavelengths via nonlinear optical processes; however, this becomes exceedingly challenging for high-repetition-rate frequency combs. Here it is demonstrated that a synchronously driven high-Q microresonator with a second-order optical nonlinearity can efficiently convert high-repetition-rate NIR frequency combs to VIS, UV, and MIR wavelengths, providing new opportunities for microresonator and electro-optic combs in applications including molecular sensing, astronomy, and quantum optics.

Quantitative Micro-Raman Spectroscopy for Partial Pressure Measurement in Small Volumes.

We demonstrate the quantitative capabilities of Raman confocal microscopy as a nondestructive method to measure the partial pressure of molecular gases in mm3 range sealed volume having an optical access. Thanks to a calibration procedure, we apply this technique for the characterization of the absolute nitrogen partial pressure inside buffered micro electromechanical system (MEMS) atomic vapor cells developed for atomic clocks. Our results are compared with measurements obtained by rubidium hyperfine frequency spectroscopy and a good agreement is demonstrated between the two methods, with a three-sigma detection limit below 10 mbar for a 1 h integration time, using a 33 mW 532 nm excitation laser. These results prove the potential of confocal micro-Raman spectroscopy as a simple and nondestructive method for small-scale pressure measurements.

Lifetime assessment of RbN3-filled MEMS atomic vapor cells with Al2O3 coating.

Micro-fabricated (MEMS) alkali vapor cells are at the heart of the miniaturization of atomic devices such as atomic magnetometers, atomic gyroscopes and atomic clocks. Among the different techniques used to fill microfabricated alkali vapor cell, UV decomposition of rubidium azide (RbN3) into metallic Rb and nitrogen in Al2O3 coated cells is a very promising approach for low-cost wafer-level fabrication. Here we present a detailed lifetime study of such cells. The rubidium consumption being the main identified cell failure mode, it is monitored with an novel image analysis technique and with high temperature long term aging tests.

Repetition rate stabilization of an optical frequency comb based on solid-state laser technology with an intra-cavity electro-optic modulator.

The repetition rate stabilization of an optical frequency comb based on diode-pumped solid-state laser technology is demonstrated using an intra-cavity electro-optic modulator. The large feedback bandwidth of such modulators allows disciplining the comb repetition rate on a cavity-stabilized continuous-wave laser with a locking bandwidth up to 700 kHz. This surpasses what can be achieved with any other type of actuator reported so far. An in-loop integrated phase noise of 133 mrad has been measured and the PM-to-AM coupling of the electro-optic modulator has been investigated as well.

Efficient carrier-envelope offset frequency stabilization through gain modulation via stimulated emission.

A novel scheme for intracavity control of the carrier-envelope offset (CEO) frequency of a 100 MHz mode-locked Er:Yb:glass diode-pumped solid-state laser (DPSSL) based on the modulation of the laser gain via stimulated emission of the excited Er(3+) ions is demonstrated. This method allows us to bypass the ytterbium system few-kHz low-pass filter in the f(CEO) stabilization loop and thus to push the phase lock bandwidth up to a limit close to the relaxation oscillations frequency of the erbium system. A phase lock bandwidth above 70 kHz has been achieved with the fully stabilized laser, leading to an integrated phase noise [1 Hz-1 MHz] of 120 mrad.

Ultra-low phase-noise microwave generation using a diode-pumped solid-state laser based frequency comb and a polarization-maintaining pulse interleaver.

We report ultra-low phase-noise microwave generation at a 9.6 GHz carrier frequency from optical frequency combs based on diode-pumped solid-state lasers emitting at telecom wavelength and referenced to a common cavity-stabilized continuous-wave laser. Using a novel fibered polarization-maintaining pulse interleaver, a single-oscillator phase-noise floor of -171 dBc/Hz at 10 MHz offset frequency has been measured with commercial PIN InGaAs photodiodes, constituting a record for this type of detector. Also, a direct optical measurement of the stabilized frequency combs' timing jitter was performed using a balanced optical cross correlator, allowing for an identification of the origin of the phase-noise limitations in the system.

Radiation hard mode-locked laser suitable as a spaceborne frequency comb.

We report ground-level gamma and proton radiation tests of a passively mode-locked diode-pumped solid-state laser (DPSSL) with Yb:KYW gain medium. A total gamma dose of 170 krad(H(2)O) applied in 5 days generates minor changes in performances while maintaining solitonic regime. Pre-irradiation specifications are fully recovered over a day to a few weeks timescale. A proton fluence of 9.76·10(10) cm(-2) applied in few minutes shows no alteration of the laser performances. Furthermore, complete stabilization of the laser shows excellent noise properties. From our results, we claim that the investigated femtosecond DPSSL technology can be considered rad-hard and would be suitable for generating frequency combs compatible with long duration space missions.

Self-referenceable frequency comb from a gigahertz diode-pumped solid-state laser.

We present carrier envelope offset (CEO) frequency detection of a diode-pumped Yb:KGW (ytterbium-doped potassium gadolinium tungstate) laser with a repetition rate of 1 GHz. The SESAM-soliton-modelocked laser delivers 2.2-W average power in 290-fs pulses. This corresponds to a peak power of 6.7 kW and the optical-to-optical efficiency is 38%. With a passive pulse compression the duration is reduced to 100 fs at an average power of 1.1 W. Coherent supercontinuum (SC) generation in a highly nonlinear photonic crystal fiber (PCF) is achieved without additional amplification. Furthermore we have demonstrated that pulse compression towards lower soliton orders of approximately 10 was required for coherent SC generation and CEO detection. Additional numerical simulations further confirm these experimental results.

Optical parametric oscillator with a pulse repetition rate of 39 GHz and 2.1-W signal average output power in the spectral region near 1.5 microm.

We present a singly resonant, synchronously pumped optical parametric oscillator with a record-high repetition rate of 39 GHz. The transform-limited 2.2-ps pulses at 1570 nm have as much as 2.1-W average output power. The all-solid-state pump source is based on a diode-pumped passively mode-locked 39-GHz Nd:YVO4 laser and an efficient ytterbium-doped fiber amplifier.