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2.
Opt Express ; 31(9): 15045-15057, 2023 Apr 24.
Article in English | MEDLINE | ID: mdl-37157355

ABSTRACT

The performance of modular, networked quantum technologies will be strongly dependent upon the quality of their quantum light-matter interconnects. Solid-state colour centres, and in particular T centres in silicon, offer competitive technological and commercial advantages as the basis for quantum networking technologies and distributed quantum computing. These newly rediscovered silicon defects offer direct telecommunications-band photonic emission, long-lived electron and nuclear spin qubits, and proven native integration into industry-standard, CMOS-compatible, silicon-on-insulator (SOI) photonic chips at scale. Here we demonstrate further levels of integration by characterizing T centre spin ensembles in single-mode waveguides in SOI. In addition to measuring long spin T1 times, we report on the integrated centres' optical properties. We find that the narrow homogeneous linewidth of these waveguide-integrated emitters is already sufficiently low to predict the future success of remote spin-entangling protocols with only modest cavity Purcell enhancements. We show that further improvements may still be possible by measuring nearly lifetime-limited homogeneous linewidths in isotopically pure bulk crystals. In each case the measured linewidths are more than an order of magnitude lower than previously reported and further support the view that high-performance, large-scale distributed quantum technologies based upon T centres in silicon may be attainable in the near term.

3.
J Phys Condens Matter ; 25(31): 316001, 2013 Aug 07.
Article in English | MEDLINE | ID: mdl-23835606

ABSTRACT

The effects of iron substitution on the structural and magnetic properties of the GdCo(12-x)Fe(x)B6 (0 ≤ x ≤ 3) series of compounds have been studied. All of the compounds form in the rhombohedral SrNi12B6-type structure and exhibit ferrimagnetic behaviour below room temperature: T(C) decreases from 158 K for x = 0 to 93 K for x = 3. (155)Gd Mössbauer spectroscopy indicates that the easy magnetization axis changes from axial to basal-plane upon substitution of Fe for Co. This observation has been confirmed using neutron powder diffraction. The axial to basal-plane transition is remarkably sensitive to the Fe content and comparison with earlier (57)Fe-doping studies suggests that the boundary lies below x = 0.1.

4.
J Phys Condens Matter ; 23(10): 106003, 2011 Mar 16.
Article in English | MEDLINE | ID: mdl-21339578

ABSTRACT

GdAgSb(2) has been studied using (155)Gd Mössbauer spectroscopy and neutron powder diffraction at a wavelength of 2.3672(1) Å. Commensurate antiferromagnetic order develops below T(N) = 13.8(4) K with the 6.2(3) µ(B) Gd moments lying in the ab-plane of the tetragonal cell. The magnetic ordering is characterized by a [½ 0 0] propagation vector (i.e. the magnetic cell is doubled along one of the crystallographic basal plane axes) with the Gd moments oriented perpendicular to the doubled direction. These results are fully consistent with an earlier determination by x-ray resonant magnetic exchange scattering.


Subject(s)
Alloys/chemistry , Magnetics/methods , Models, Molecular , Spectroscopy, Mossbauer/methods , Antimony/chemistry , Crystallization/methods , Crystallography, X-Ray/methods , Gadolinium/chemistry , Neutron Diffraction/methods , Powder Diffraction/methods , Silver/chemistry , Temperature
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