Free-carrier-induced soliton fission unveiled by in situ measurements in nanophotonic waveguides.

Solitons are localized waves formed by a balance of focusing and defocusing effects. These nonlinear waves exist in diverse forms of matter yet exhibit similar properties including stability, periodic recurrence and particle-like trajectories. One important property is soliton fission, a process by which an energetic higher-order soliton breaks apart due to dispersive or nonlinear perturbations. Here we demonstrate through both experiment and theory that nonlinear photocarrier generation can induce soliton fission. Using near-field measurements, we directly observe the nonlinear spatial and temporal evolution of optical pulses in situ in a nanophotonic semiconductor waveguide. We develop an analytic formalism describing the free-carrier dispersion (FCD) perturbation and show the experiment exceeds the minimum threshold by an order of magnitude. We confirm these observations with a numerical nonlinear Schrödinger equation model. These results provide a fundamental explanation and physical scaling of optical pulse evolution in free-carrier media and could enable improved supercontinuum sources in gas based and integrated semiconductor waveguides.

Cross-phase modulation-induced spectral broadening in silicon waveguides.

We analytically and experimentally investigate cross-phase modulation (XPM) in silicon waveguides. In contrast to the well known result in pure Kerr media, the spectral broadening ratio of XPM to self-phase modulation is not two in the presence of either two-photon absorption (TPA) or free carriers. The physical origin of this change is different for each effect. In the case of TPA, this nonlinear absorption attenuates and slightly modifies the pulse shape due to differential absorption in the pulse peak and wings. When free carriers are present two different mechanisms modify the dynamics. First, free-carrier absorption performs a similar role to TPA, but is additionally asymmetric due to the delayed free-carrier response. Second, free-carrier dispersion induces an asymmetric blue phase shift which competes directly with the symmetric Kerr-induced XPM red shift. We confirm this analysis with pump-probe experiments in a silicon photonic crystal waveguide.

Non-degenerate two-photon absorption in silicon waveguides: analytical and experimental study.

We theoretically and experimentally investigate the nonlinear evolution of two optical pulses in a silicon waveguide. We provide an analytic solution for the weak probe wave undergoing non-degenerate two-photon absorption (TPA) from the strong pump. At larger pump intensities, we employ a numerical solution to study the interplay between TPA and photo-generated free carriers. We develop a simple and powerful approach to extract and separate out the distinct loss contributions of TPA and free-carrier absorption from readily available experimental data. Our analysis accounts accurately for experimental results in silicon photonic crystal waveguides.

Low-threshold Brillouin laser at 2 µm based on suspended-core chalcogenide fiber.

We present, to the best of our knowledge, the first demonstration of a 2 µm Brillouin laser based on a thulium-doped fiber pump and a chalcogenide fiber. A short 1.5 m piece of suspended-core chalcogenide As38Se62 fiber is employed as a gain medium, taking advantage of its small effective mode area and high Brillouin gain coefficient. A record-low lasing threshold of 52 mW is achieved, which is about 10 times lower than previously demonstrated in silica fiber cavities.

Phase-sensitive amplification in silicon photonic crystal waveguides.

We experimentally demonstrate phase-sensitive amplification in a silicon photonic crystal waveguide based on pump-degenerate four-wave mixing. An 11 dB phase-extinction ratio is obtained in a record compact 196 µm nanophotonic device due to broadband slow light, in spite of the presence of two-photon absorption and free carriers. Numerical calculations show good agreement with the experimental results.

Hybrid Brillouin/thulium multiwavelength fiber laser with switchable single- and double-Brillouin-frequency spacing.

We demonstrate a multiwavelength laser at 2 µm based on a hybrid gain scheme consisting of a Brillouin gain medium and a thulium-doped fiber. The laser has switchable frequency spacing, corresponding to the single and double Brillouin frequency shifts. In the 20 dB bandwidth, seven lasing channels with a frequency spacing of 0.1 nm (7.62 GHz) and eleven channels with a double-spacing of 0.2 nm (15.24 GHz) are obtained. A wavelength tunability of 1.3 nm is realized for both laser configurations by shifting the pump wavelength. Strong four wave mixing is observed in the double-spacing laser resulting in an improved performance: larger number of channels and better temporal stability.

Fiber optical parametric oscillator for coherent anti-Stokes Raman scattering microscopy.

We present a synchronously pumped fiber optical parametric oscillator for coherent anti-Stokes Raman scattering microscopy. Pulses from a 1 µm Yb-doped fiber laser are amplified and frequency converted to 779-808 nm through normal dispersion four-wave mixing in a photonic crystal fiber. The idler frequency is resonant in the oscillator cavity, and we find that bandpass filtering the feedback is essential for stable, narrow-bandwidth output. Experimental results agree quite well with numerical simulations of the device. Transform-limited 2 ps pulses with energy up to 4 nJ can be generated at the signal wavelength. The average power is 180 mW, and the relative-intensity noise is much lower than that of a similar parametric amplifier. High-quality coherent Raman images of mouse tissues recorded with this source are presented.

High-energy similariton fiber laser using chirally coupled core fiber.

We present a high-energy amplifier similariton laser based on a chirally coupled core (3C) fiber. Chirped pulse energies up to 61 nJ at 3.3 W average power are obtained with effectively single-mode output. The pulses can be compressed with a simple grating compressor to durations below 90 fs. We demonstrate for the first time a fused pump-signal combiner to confirm the integration potential of 3C fiber.

Fiber four-wave mixing source for coherent anti-Stokes Raman scattering microscopy.

We present a fiber-format picosecond light source for coherent anti-Stokes Raman scattering microscopy. Pulses from a Yb-doped fiber amplifier are frequency converted by four-wave mixing (FWM) in normal-dispersion photonic crystal fiber to produce a synchronized two-color picosecond pulse train. We show that seeding the FWM process overcomes the deleterious effects of group-velocity mismatch and allows efficient conversion into narrow frequency bands. The source generates more than 160 mW of nearly transform-limited pulses tunable from 775 to 815 nm. High-quality coherent Raman images of animal tissues and cells acquired with this source are presented.

Scaling Fiber Lasers to Large Mode Area: An Investigation of Passive Mode-Locking Using a Multi-Mode Fiber.

The mode-locking of dissipative soliton fiber lasers using large mode area fiber supporting multiple transverse modes is studied experimentally and theoretically. The averaged mode-locking dynamics in a multi-mode fiber are studied using a distributed model. The co-propagation of multiple transverse modes is governed by a system of coupled Ginzburg-Landau equations. Simulations show that stable and robust mode-locked pulses can be produced. However, the mode-locking can be destabilized by excessive higher-order mode content. Experiments using large core step-index fiber, photonic crystal fiber, and chirally-coupled core fiber show that mode-locking can be significantly disturbed in the presence of higher-order modes, resulting in lower maximum single-pulse energies. In practice, spatial mode content must be carefully controlled to achieve full pulse energy scaling. This paper demonstrates that mode-locking performance is very sensitive to the presence of multiple waveguide modes when compared to systems such as amplifiers and continuous-wave lasers.

Energy scaling of mode-locked fiber lasers with chirally-coupled core fiber.

We report a mode-locked dissipative soliton laser based on large-mode-area chirally-coupled-core Yb-doped fiber. This demonstrates scaling of a fiber oscillator to large mode area in a format that directly holds the lowest-order mode and that is also compatible with standard fiber integration. With an all-normal-dispersion cavity design, chirped pulse energies above 40 nJ are obtained with dechirped durations below 200 fs. Using a shorter fiber, dechirped durations close to 100 fs are achieved at pump-limited energies. The achievement of correct energy scaling is evidence of single-transverse-mode operation, which is confirmed by beam-quality and spectral-interference measurements.

Scaling of dissipative soliton fiber lasers to megawatt peak powers by use of large-area photonic crystal fiber.

We report an all-normal dispersion femtosecond laser based on large-mode-area Yb-doped photonic crystal fiber. Self-starting mode-locked pulses are obtained with an average power of 12 W at 84 MHz repetition rate, corresponding to 140 nJ of chirped pulse energy. These are dechirped to a near transform-limited duration of 115 fs. Experimental results are consistent with numerical simulations of dissipative soliton intra-cavity pulse evolution, and demonstrate scaling of 100 fs pulses to megawatt peak powers.

Visualizing the frontier orbitals of a conformationally adapted metalloporphyrin.

We present a molecular-level study of the geometric and electronic properties of Co(II) tetraphenylporphyrin molecules adsorbed on the Cu(111) surface. A combination of low-temperature scanning tunneling microscopy and near-edge X-ray absorption fine structure observations reveals how the metal substrate induces a conformational adaptation into a distorted saddle-shaped geometry. By scanning tunneling spectroscopy we identified the discrete energy levels of the molecule and mapped their spatial electron-density distributions. These results, along with a simple theoretical description, provide a direct correlation between the shape of frontier molecular orbitals and intramolecular structural features.