ABSTRACT
The Fourier transform-infrared (FT-IR) spectrometer is a widely used high-resolution spectral characterization method in materials, chemicals, and more. However, the inverse relation between the spectral resolution and the interferometer's arm length yields a tradeoff between spectral resolution and spectrometer footprint. Here, we introduce a novel method to overcome this traditional FT-IR resolution limit. The enhanced high-resolution multi-scan compact FT-IR spectrometer we present achieves an effectively long interferogram by combining multiple short FT-IR scans. Simulation and experimental results demonstrate a significant increase in the spectral resolution of a FT-IR spectrometer by employing our interferogram stitching algorithm.
ABSTRACT
We experimentally demonstrate an efficient broadband second-harmonic generation (SHG) process with a tunable mode-locked Ti:sapphire oscillator. We have achieved a robust broadband and efficient flat conversion of more than 35 nm wavelength by designing an adiabatic aperiodically poled potassium titanyl phosphate crystal. Moreover, we have shown that with such efficient flat conversion, we can shape and control broadband second-harmonic pulses. More specifically, we assign a spectral phase of absolute value and π-step, which allows wavelength tunable intense pump-probe and amplitude modulation of the broadband second-harmonic output. Such spectral phases serve as a proof of concept for other pulse-shaping applications for nonlinear spectroscopy and imaging.
