Determining a vibrational distribution with a broadband optical source.

This work presents an experimental protocol conceived to determine the vibrational distribution of barium monofluoride molecules seeded in a supersonic beam of argon. Here, as in many cases, the detection signal is related to the number of molecules by an efficiency involving several parameters that may be difficult to determine properly. In particular, this efficiency depends on the vibrational level of the detected molecules. Our approach avoids these complications by comparing different detection signals generated by different vibrational excitations. Such an excitation is made possible by the use of a broadband optical source that depletes a specific vibrational level whose population is redistributed in the other levels.

Rovibrational cooling of molecules by optical pumping.

We demonstrate rotational and vibrational cooling of cesium dimers by optical pumping techniques. We use two laser sources exciting all the populated rovibrational states, except a target state that thus behaves like a dark state where molecules pile up thanks to absorption-spontaneous emission cycles. We are able to accumulate photoassociated cold Cs(2) molecules in their absolute ground state (v = 0, J = 0) with up to 40% efficiency. Given its simplicity, the method could be extended to other molecules and molecular beams. It also opens up general perspectives in laser cooling the external degrees of freedom of molecules.

Deeply bound cold caesium molecules formed after 0(-)(g) resonant coupling.

Translationally cold caesium molecules are created by photoassociation below the 6s + 6p(1/2) excited state and selectively detected by resonance enhanced two photon ionization (RE2PI). A series of excited vibrational levels belonging to the 0(-)(g) symmetry is identified. The regular progression of the vibrational spacings and of the rotational constants of the 0(-)(g) (6s + 6p(1/2)) levels is strongly altered in two energy domains. These deviations are interpreted in terms of resonant coupling with deeply bound energy levels of two upper 0(-)(g) states dissociating into the 6s + 6p(3/2) and 6s + 5d(3/2) asymptotes. A theoretical model is proposed to explain the coupling and a quantum defect analysis of the perturbed level position is performed. Moreover, the resonant coupling changes dramatically the spontaneous decay products of the photoexcited molecules, strongly enhancing the decay into deeply bound levels of the a(3)Σ(+)(u) triplet state and of the X(1)Σ(+)(g) ground state. These results may be relevant when conceiving population transferring schemes in cold molecule systems.

Time-resolved measurement of Landau-Zener tunneling in periodic potentials.

We report time-resolved measurements of Landau-Zener tunneling of Bose-Einstein condensates in accelerated optical lattices, clearly resolving the steplike time dependence of the band populations. Using different experimental protocols we were able to measure the tunneling probability both in the adiabatic and in the diabatic bases of the system. We also experimentally determine the contribution of the momentum width of the Bose condensates to the temporal width of the tunneling steps and discuss the implications for measuring the jump time in the Landau-Zener problem.

Observation of photon-assisted tunneling in optical lattices.

We have observed tunneling suppression and photon-assisted tunneling of Bose-Einstein condensates in an optical lattice subjected to a constant force plus a sinusoidal shaking. For a sufficiently large constant force, the ground energy levels of the lattice are shifted out of resonance and tunneling is suppressed; when the shaking is switched on, the levels are coupled by low-frequency photons and tunneling resumes. Our results agree well with theoretical predictions and demonstrate the usefulness of optical lattices for studying solid-state phenomena.

Resonantly enhanced tunneling of Bose-Einstein condensates in periodic potentials.

We report on measurements of resonantly enhanced tunneling of Bose-Einstein condensates loaded into an optical lattice. By controlling the initial conditions of our system we were able to observe resonant tunneling in the ground and the first two excited states of the lattice wells. We also investigated the effect of the intrinsic nonlinearity of the condensate on the tunneling resonances.

Dynamical control of matter-wave tunneling in periodic potentials.

We report on measurements of dynamical suppression of interwell tunneling of a Bose-Einstein condensate (BEC) in a strongly driven optical lattice. The strong driving is a sinusoidal shaking of the lattice corresponding to a time-varying linear potential, and the tunneling is measured by letting the BEC freely expand in the lattice. The measured tunneling rate is reduced and, for certain values of the shaking parameter, completely suppressed. Our results are in excellent agreement with theoretical predictions. Furthermore, we have verified that, in general, the strong shaking does not destroy the phase coherence of the BEC, opening up the possibility of realizing quantum phase transitions by using the shaking strength as the control parameter.