Method of spectral response to stochastic processes for measuring the nonreciprocal effective interactions.

The theoretical background of the nonperturbative method of spectral response to stochastic processes (SRSP) for measuring the nonreciprocal interparticle effective interactions in strongly coupled underdamped systems is described. Analytical expressions for vibrational spectral density of confined Brownian particles with a nonreciprocal effective interaction are presented. The changes in the vibrational spectral density with varying different parameters of the system (nonreciprocity, viscosity, ratios of particle sizes, and intensities of random processes acting on each particle) are discussed using the example of a pair of nonidentical particles in a harmonic trap. The SRSP method is compared to three other nonperturbative methods. The SRSP method demonstrates an undeniable advantage when processing particle trajectories with errors in particle tracking.

Motion of a self-propelled particle with rotational inertia.

Overdamped active Brownian motion of self-propelled particles in a liquid has been fairly well studied. However, there are a variety of situations in which the overdamped approximation is not justified, for instance, when self-propelled particles move in a low-viscosity medium or when their rotational diffusivity is enhanced by internal active processes or external control. Examples of various origins include biofilaments driven by molecular motors, living and artificial microflyers and interfacial surfers, field-controlled and superfluid microswimmers, vibration-driven granular particles and autonomous mini-robots with sensorial delays, etc. All of them extend active Brownian motion to the underdamped case, i.e., to active Langevin motion, which takes into account inertia. Despite a rich experimental background, there is a gap in the theory in the field where rotational inertia significantly affects the random walk of active particles on all time scales. In particular, although the well-known models of active Brownian and Ornstein-Uhlenbeck particles include a memory effect of the direction of motion, they are not applicable in the underdamped case, because the rotational inertia, which they do not account for, can partially prevent "memory loss" with increasing rotational diffusion. We describe the two-dimensional motion of a self-propelled particle with both translational and rotational inertia and velocity fluctuations. The proposed generalized analytical equations for the mean kinetic energy, mean-square displacement and noise-averaged trajectory of the self-propelled particle are confirmed by numerical simulations in a wide range of self-propulsion velocities, moments of inertia, rotational diffusivities, medium viscosities and observation times.

Active Brownian particle in homogeneous media of different viscosities: numerical simulations.

Self-propelled colloids, active polymers and membranes, driven (vibrated) granular layers and hybrid synthetic-biological systems are striking examples of systems containing synthetic active Brownian particles. Such particles autonomously convert the available energy of the environment into their own directed mechanical motion. In most studies the self-propelled Brownian particles move in overdamped media. Recently, experiments with Janus particles in a low-pressure plasma have appeared. A distinctive feature of such a medium is an extremely low viscosity at which the inertial effects play a significant role, resulting in underdamped Brownian motion. At present, there is a lack of statistical theory describing the underdamped Brownian motion of self-propelled particles at all time scales. This paper presents the numerical simulation results of active Brownian motion in homogeneous media of different viscosities. The calculations are performed using a mathematical model of a self-propelled Brownian sphere with translational and rotational inertia. The time-dependent mean square displacement and mean linear displacement (the noise-averaged trajectory) of the particle are investigated as a function of medium viscosity, self-propulsion velocity and moment of inertia. Our simulation reveals that the dynamics of a self-propelled spherical particle significantly depends on two independent dimensionless parameters of the particle: the ratio of the self-propulsion velocity to the characteristic thermal velocity and the ratio of the friction coefficient to the rotational diffusion coefficient. The obtained statistical characteristics of active Brownian motion are compared with the known theoretical models in a wide range of medium viscosities. We propose simple corrections to the basic theory of overdamped active Brownian motion, which allow one to calculate the effective diffusion coefficient and the persistence length of a self-propelled Brownian particle in a medium with any dynamic viscosity. The results obtained are discussed in relation to active particles in a colloidal plasma and superfluid helium.

Experimental study of the nonreciprocal effective interactions between microparticles in an anisotropic plasma.

There is a variety of cases in nature when the action-reaction symmetry is broken. In particular, suitable conditions for this are realized in colloidal suspensions and complex plasmas. Since the first theories and simulations of the nonreciprocal effective interactions between microparticles in complex plasmas were published in 1995-1996, there have been hundreds of studies in the theoretical development of this theme. However, despite such a rich theoretical background, one of the important unsolved problems is a direct experimental determination of the nonreciprocal interparticle interaction forces. Here, we studied experimentally in detail the forces of the nonreciprocal effective interaction between microparticles suspended a radio-frequency produced plasma sheath. For this purpose, an experimental method based on an analysis of the spectral density of random processes in an open dissipative two-particle system was developed. In contrast to previous investigations, the proposed method takes into account random and dissipative processes in the system, does not require a special design of the experimental setup and any external perturbations, pre-measurements of external fields and any assumptions about the type of interaction. We found that even small charge changes of one particle, caused by its thermal motion in a wake field of another particle, can lead to a significant change in the effective (measurable) interaction between the particles.

Self-confined particle pairs in complex plasmas.

The liquid-crystal type of phase transition in complex plasmas has been observed repeatedly. However, more studies need to be done on the liquid-vapor transition in complex plasmas. In this paper, the phenomenon of coupling (condensation) of particles into self-confined particle pairs in an anisotropic plasma medium with ion flow is considered analytically and numerically using the Langevin molecular dynamics method. We obtain the stability conditions of the pair (bound) state depending on the interaction parameters and particle kinetic energy. It was shown that the breakup of the particle pair is very sensitive to the ratio of particle charges; for example, it is determined by the influence of the upper particle on the ion flow around the lower one. We also show that a self-confined pair of particles exists even if their total kinetic energy is much greater than the potential well depth for the pair state. This phenomenon occurs due to velocity correlation of particles, which arises with the nonreciprocity of interparticle interaction.

Determination of pair interaction forces between particles in nonideal dissipative systems.

A new technique for analyzing the pair interaction forces between particles in nonideal dissipative systems is presented. The technique is based on a solution of the inverse problem describing the movement of dust particles by a system of Langevin equations. Numerical simulations in a wide range of the parameters typical for dusty plasma experiments were performed to verify the solutions of the inverse problem. The first approbations of the proposed technique for analysis of intergrain interactions in a plasma of rf discharge are presented.