Experimental Demonstration of Input-Output Indefiniteness in a Single Quantum Device.

Quantum theory allows information to flow through a single device in a coherent superposition of two opposite directions, resulting into situations where the input-output direction is indefinite. Here we introduce a theoretical method to witness input-output indefiniteness in a single quantum device, and we experimentally demonstrate it by constructing a photonic setup that exhibits input-output indefiniteness with a statistical significance exceeding 69 standard deviations. Our results provide a way to characterize input-output indefiniteness as a resource for quantum information and photonic quantum technologies and enable tabletop simulations of hypothetical scenarios exhibiting quantum indefiniteness in the direction of time.

Preparation of multiphoton high-dimensional GHZ states.

The physics associated with multipartite high-dimensional entanglement is different from that of multipartite two-dimensional entanglement. Therefore, preparing multipartite high-dimensional entanglements with linear optics is challenging. This study proposes a preparation protocol of multiphoton GHZ state with arbitrary dimensions for optical systems. Auxiliary entanglements realize a high-dimensional entanglement gate to connect the high-dimensional entangled pairs to a multipartite high-dimensional GHZ state. Specifically, we use the path degrees of freedom of photons to prepare a four-partite, three-dimensional GHZ state. Our method can be extended to other degrees of freedom to generate arbitrary GHZ entanglements in any dimension.

Certification of non-classicality in all links of a photonic star network without assuming quantum mechanics.

Networks composed of independent sources of entangled particles that connect distant users are a rapidly developing quantum technology and an increasingly promising test-bed for fundamental physics. Here we address the certification of their post-classical properties through demonstrations of full network nonlocality. Full network nonlocality goes beyond standard nonlocality in networks by falsifying any model in which at least one source is classical, even if all the other sources are limited only by the no-signaling principle. We report on the observation of full network nonlocality in a star-shaped network featuring three independent sources of photonic qubits and joint three-qubit entanglement-swapping measurements. Our results demonstrate that experimental observation of full network nonlocality beyond the bilocal scenario is possible with current technology.

Experimental one-step deterministic polarization entanglement purification.

Entanglement purification is to distill high-quality entangled states from low-quality entangled states. It is a key step in quantum repeaters, determines the efficiency and communication rates of quantum communication protocols, and is hence of central importance in long-distance communications and quantum networks. In this work, we report the first experimental demonstration of deterministic entanglement purification using polarization and spatial mode hyperentanglement. After purification, the fidelity of polarization entanglement arises from 0.268±0.002 to 0.989±0.001. Assisted with robust spatial mode entanglement, the total purification efficiency can be estimated as 109 times that of the entanglement purification protocols using two copies of entangled states when one uses the spontaneous parametric down-conversion sources. Our work may have the potential to be implemented as a part of full repeater protocols.

Experimental Demonstration that No Tripartite-Nonlocal Causal Theory Explains Nature's Correlations.

Quantum theory predicts the existence of genuinely tripartite-entangled states, which cannot be obtained from local operations over any bipartite-entangled states and unlimited shared randomness. Some of us recently proved that this feature is a fundamental signature of quantum theory. The state |GHZ_{3}⟩=(|000⟩+|111⟩)/sqrt[2] gives rise to tripartite quantum correlations that cannot be explained by any causal theory limited to bipartite nonclassical common causes of any kind (generalizing entanglement) assisted with unlimited shared randomness. Hence, any conceivable physical theory that would reproduce quantum predictions will necessarily include genuinely tripartite resources. In this Letter, we verify that such tripartite correlations are experimentally achievable. We derive a new device-independent witness capable of falsifying causal theories wherein nonclassical resources are merely bipartite. Using a high-performance photonic |GHZ_{3}⟩ state with fidelities of 0.9741±0.002, we provide a clear experimental violation of that witness by more than 26.3 standard deviations, under the locality and fair sampling assumption. We generalize our Letter to the |GHZ_{4}⟩ state, obtaining correlations that cannot be explained by any causal theory limited to tripartite nonclassical common causes assisted with unlimited shared randomness.

High-Dimensional Bell Test without Detection Loophole.

Violation of Bell's inequalities shows strong conflict between quantum mechanics and local realism. Loophole-free Bell tests not only deepen understanding of quantum mechanics, but are also important foundations for device-independent (DI) tasks in quantum information. High-dimensional quantum systems offer a significant advantage over qubits for closing the detection loophole. In the symmetric scenario, a detection efficiency as low as 61.8% can be tolerated using four-dimensional states and a four-setting Bell inequality [Phys. Rev. Lett. 104, 060401 (2010)PRLTAO0031-900710.1103/PhysRevLett.104.060401]. For the first time, we show that four-dimensional entangled photons violate a Bell inequality while closing the detection loophole in experiment. The detection efficiency of the four-dimensional entangled source is about 71.7%, and the fidelity of the state is 0.995±0.001. Combining the technique of multicore fibers, the realization of loophole-free high-dimensional Bell tests and high-dimensional quantum DI technologies are promising.

Entanglement Swapping and Quantum Correlations via Symmetric Joint Measurements.

We use hyperentanglement to experimentally realize deterministic entanglement swapping based on quantum elegant joint measurements. These are joint projections of two qubits onto highly symmetric, isoentangled bases. We report measurement fidelities no smaller than 97.4%. We showcase the applications of these measurements by using the entanglement swapping procedure to demonstrate quantum correlations in the form of proof-of-principle violations of both bilocal Bell inequalities and more stringent correlation criteria corresponding to full network nonlocality. Our results are a foray into entangled measurements and nonlocality beyond the paradigmatic Bell state measurement and they show the relevance of more general measurements in entanglement swapping scenarios.

Optimized Detection of High-Dimensional Entanglement.

Entanglement detection is one of the most conventional tasks in quantum information processing. While most experimental demonstrations of high-dimensional entanglement rely on fidelity-based witnesses, these are powerless to detect entanglement within a large class of entangled quantum states, the so-called unfaithful states. In this Letter, we introduce a highly flexible automated method to construct optimal tests for entanglement detection given a bipartite target state of arbitrary dimension, faithful or unfaithful, and a set of local measurement operators. By restricting the number or complexity of the considered measurement settings, our method outputs the most convenient protocol which can be implemented using a wide range of experimental techniques such as photons, superconducting qudits, cold atoms, or trapped ions. With an experimental quantum optics setup that can prepare and measure arbitrary high-dimensional mixed states, we implement some three-setting protocols generated by our method. These protocols allow us to experimentally certify two- and three-unfaithful entanglement in four-dimensional photonic states, some of which contain well above 50% of noise.

Pathways for Entanglement-Based Quantum Communication in the Face of High Noise.

Entanglement-based quantum communication offers an increased level of security in practical secret shared key distribution. One of the fundamental principles enabling this security-the fact that interfering with one photon will destroy entanglement and thus be detectable-is also the greatest obstacle. Random encounters of traveling photons, losses, and technical imperfections make noise an inevitable part of any quantum communication scheme, severely limiting distance, key rate, and environmental conditions in which quantum key distribution can be employed. Using photons entangled in their spatial degree of freedom, we show that the increased noise resistance of high-dimensional entanglement can indeed be harnessed for practical key distribution schemes. We perform quantum key distribution in eight entangled paths at various levels of environmental noise and show key rates that, even after error correction and privacy amplification, still exceed 1 bit per photon pair and furthermore certify a secure key at noise levels that would prohibit comparable qubit based schemes from working.

Nonlocality, Steering, and Quantum State Tomography in a Single Experiment.

We investigate whether paradigmatic measurements for quantum state tomography, namely mutually unbiased bases and symmetric informationally complete measurements, can be employed to certify quantum correlations. For this purpose, we identify a simple and noise-robust correlation witness for entanglement detection, steering, and nonlocality that can be evaluated based on the outcome statistics obtained in the tomography experiment. This allows us to perform state tomography on entangled qutrits, a test of Einstein-Podolsky-Rosen steering and a Bell inequality test, all within a single experiment. We also investigate the trade-off between quantum correlations and subsets of tomographically complete measurements as well as the quantification of entanglement in the different scenarios. Finally, we perform a photonics experiment in which we demonstrate quantum correlations under these flexible assumptions, namely with both parties trusted, one party untrusted and both parties untrusted.

Experimental Demonstration of Instrument-Specific Quantum Memory Effects and Non-Markovian Process Recovery for Common-Cause Processes.

The duration, strength, and structure of memory effects are crucial properties of physical evolution. Because of the invasive nature of quantum measurement, such properties must be defined with respect to the probing instruments employed. Here, using a photonic platform, we experimentally demonstrate this necessity via two paradigmatic processes: future-history correlations in the first process can be erased by an intermediate quantum measurement; for the second process, a noisy classical measurement blocks the effect of history. We then apply memory truncation techniques to recover an efficient description that approximates expectation values for multitime observables. Our proof-of-principle analysis paves the way for experiments concerning more general non-Markovian quantum processes and highlights where standard open systems techniques break down.

Long-Distance Entanglement Purification for Quantum Communication.

High-quality long-distance entanglement is essential for both quantum communication and scalable quantum networks. Entanglement purification is to distill high-quality entanglement from low-quality entanglement in a noisy environment and it plays a key role in quantum repeaters. The previous significant entanglement purification experiments require two pairs of low-quality entangled states and were demonstrated in tabletop. Here we propose and report a high-efficiency and long-distance entanglement purification using only one pair of hyperentangled state. We also demonstrate its practical application in entanglement-based quantum key distribution (QKD). One pair of polarization spatial-mode hyperentanglement was distributed over 11 km multicore fiber (noisy channel). After purification, the fidelity of polarization entanglement arises from 0.771 to 0.887 and the effective key rate in entanglement-based QKD increases from 0 to 0.332. The values of Clauser-Horne-Shimony-Holt inequality of polarization entanglement arises from 1.829 to 2.128. Moreover, by using one pair of hyperentanglement and deterministic controlled-NOT gates, the total purification efficiency can be estimated as 6.6×10^{3} times than the experiment using two pairs of entangled states with spontaneous parametric down-conversion sources. Our results offer the potential to be implemented as part of a full quantum repeater and large-scale quantum network.

Experimental High-Dimensional Quantum Teleportation.

Quantum teleportation provides a way to transmit unknown quantum states from one location to another. In the quantum world, multilevel systems which enable high-dimensional systems are more prevalent. Therefore, to completely rebuild the quantum states of a single particle remotely, one needs to teleport multilevel (high-dimensional) states. Here, we demonstrate the teleportation of high-dimensional states in a three-dimensional six-photon system. We exploit the spatial mode of a single photon as the high-dimensional system, use two auxiliary entangled photons to realize a deterministic three-dimensional Bell state measurement. The fidelity of teleportation process matrix is F=0.596±0.037. Through this process matrix, we can prove that our teleportation is both nonclassical and genuine three dimensional. Our work paves the way to rebuild complex quantum systems remotely and to construct complex quantum networks.

Efficient Generation of High-Dimensional Entanglement through Multipath Down-Conversion.

High-dimensional entanglement promises to greatly enhance the performance of quantum communication and enable quantum advantages unreachable by qubit entanglement. One of the great challenges, however, is the reliable production, distribution, and local certification of high-dimensional sources of entanglement. In this Letter, we present an optical setup capable of producing quantum states with an exceptionally high level of scalability, control, and quality that, together with novel certification techniques, achieve the highest amount of entanglement recorded so far. We showcase entanglement in 32-spatial dimensions with record fidelity to the maximally entangled state (F=0.933±0.001) and introduce measurement efficient schemes to certify entanglement of formation (E_{oF}=3.728±0.006). Combined with the existing multicore fiber technology, our results will lay a solid foundation for the construction of high-dimensional quantum networks.

Experimental Transmission of Quantum Information Using a Superposition of Causal Orders.

Communication in a network generally takes place through a sequence of intermediate nodes connected by communication channels. In the standard theory of communication, it is assumed that the communication network is embedded in a classical spacetime, where the relative order of different nodes is well defined. In principle, a quantum theory of spacetime could allow the order of the intermediate points between sender and receiver to be in a coherent superposition. Here we experimentally realize a tabletop simulation of this exotic possibility on a photonic system, demonstrating high-fidelity transmission of quantum information over two noisy channels arranged in a superposition of two alternative causal orders.

Experimental Measurement-Device-Independent Quantum Steering and Randomness Generation Beyond Qubits.

In a measurement-device-independent or quantum-refereed protocol, a referee can verify whether two parties share entanglement or Einstein-Podolsky-Rosen (EPR) steering without the need to trust either of the parties or their devices. The need for trusting a party is substituted by a quantum channel between the referee and that party, through which the referee encodes the measurements to be performed on that party's subsystem in a set of nonorthogonal quantum states. In this Letter, an EPR-steering inequality is adapted as a quantum-refereed EPR-steering witness, and the trust-free experimental verification of higher dimensional quantum steering is reported via preparing a class of entangled photonic qutrits. Further, with two measurement settings, we extract 1.106±0.023 bits of private randomness per every photon pair from our observed data, which surpasses the one-bit limit for projective measurements performed on qubit systems. Our results advance research on quantum information processing tasks beyond qubits.

Demonstrating Quantum Coherence and Metrology that is Resilient to Transversal Noise.

Quantum systems can be exploited for disruptive technologies but in practice quantum features are fragile due to noisy environments. Quantum coherence, a fundamental such feature, is a basis-dependent property that is known to exhibit a resilience to certain types of Markovian noise. Yet, it is still unclear whether this resilience can be relevant in practical tasks. Here, we experimentally investigate the resilient effect of quantum coherence in a photonic Greenberger-Horne-Zeilinger state under Markovian bit-flip noise, and explore its applications in a noisy metrology scenario. In particular, using up to six-qubit probes, we demonstrate that the standard quantum limit can be outperformed under a transversal noise strength of approximately equal magnitude to the signal, providing experimental evidence of metrological advantage even in the presence of uncorrelated Markovian noise. This work highlights the important role of passive control in noisy quantum hardware, which can act as a low-overhead complement to more traditional approaches such as quantum error correction, thus impacting on the deployment of quantum technologies in real-world settings.

Entanglement Detection by Violations of Noisy Uncertainty Relations: A Proof of Principle.

It is well known that the violation of a local uncertainty relation can be used as an indicator for the presence of entanglement. Unfortunately, the practical use of these nonlinear witnesses has been limited to few special cases in the past. However, new methods for computing uncertainty bounds have become available. Here we report on an experimental implementation of uncertainty-based entanglement witnesses, benchmarked in a regime dominated by strong local noise. We combine the new computational method with a local noise tomography in order to design noise-adapted entanglement witnesses. This proof-of-principle experiment shows that quantum noise can be successfully handled by a fully quantum model in order to enhance the ability to detect entanglement.

Experimental test of fine-grained entropic uncertainty relation in the presence of quantum memory.

The uncertainty principle, which gives the constraints on obtaining precise outcomes for incompatible measurements, provides a new vision of the real world that we are not able to realize from the classical knowledge. In recent years, numerous theoretical and experimental developments about the new forms of the uncertainty principle have been achieved. Among these efforts, one attractive goal is to find tighter bounds of the uncertainty relation. Here, using an all optical setup, we experimentally investigate a most recently proposed form of uncertainty principle-the fine-grained uncertainty relation assisted by a quantum memory. The experimental results on the case of two-qubit state with maximally mixed marginal demonstrate that the fine-graining method can help to get a tighter bound of the uncertainty relation. Our results might contribute to further understanding and utilizing of the uncertainty principle.

Experimental realization of sequential weak measurements of non-commuting Pauli observables.

Sequential weak measurements of non-commuting observables are not only fundamentally interesting in terms of quantum measurement but also show potential in various applications. Previously reported methods, however, can only make limited sequential weak measurements experimentally. In this article, we propose the realization of sequential measurements of non-commuting Pauli observables and experimentally demonstrate for the first time the measurement of sequential weak values of three non-commuting Pauli observables using genuine single photons.