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1.
iScience ; 27(5): 109721, 2024 May 17.
Article in English | MEDLINE | ID: mdl-38706853

ABSTRACT

This article designs and implements a fast and high-precision multi-robot environment modeling method based on bidirectional filtering and scene identification. To solve the problem of feature tracking failure caused by large angle rotation, a bidirectional filtering mechanism is introduced to improve the error-matching elimination algorithm. A global key frame database for multiple robots is proposed based on a pretraining dictionary to convert images into a bag of words vectors. The images captured by different sub-robots are compared with the database for similarity score calculation, so as to realize fast identification and search of similar scenes. The coordinate transformation from local map to global map and the cooperative SLAM exploration of multiple robots is completed by the best matching image and the transformation matrix. The experimental results show that the proposed algorithm can effectively close the predicted trajectory of the sub-robot, thus achieving high-precision collaborative environment modeling.

2.
Dalton Trans ; 52(39): 14210-14219, 2023 Oct 10.
Article in English | MEDLINE | ID: mdl-37766470

ABSTRACT

Developing a high-performance piezocatalyst that directly transforms mechanical energy into hydrogen is highly desirable in the field of new energy. Herein, the Aurivillius-layered Bi2WO6 (BWO) nanoplates are prepared through a hydrothermal reaction at a moderate temperature of 160 °C, and exhibit strong piezoelectric properties, enabling them to catalyze water splitting through ultrasonic-induced piezocatalysis effect. The hydrogen evolution reaction (HER) and H2O2 generation efficiencies are measured to be 0.43 and 0.36 mmol g-1 h-1, respectively. To further boost piezocatalytic performance, cobalt oxide nanoparticles are intentionally photo-deposited onto these nanoplates as cocatalyst. This configuration results in a significantly boosted HER performance with an efficiency of 3.59 mmol g-1 h-1, which is 2.8 times higher than that of pristine nanoplates and demonstrates strong competitiveness compared to other reported piezocatalysts. The cobalt oxide cocatalyst plays a crucial role in facilitating efficient charge separation and migration, increasing the charge concentration, and ultimately enhancing piezocatalytic HER activity. Overall, this work highlights the potential of Aurivillius-layered bismuth oxide compounds as efficient piezocatalysts and provides valuable insights for designing high-performance piezocatalysts in the field of new energy.

3.
Inflamm Regen ; 43(1): 36, 2023 Jul 14.
Article in English | MEDLINE | ID: mdl-37452367

ABSTRACT

BACKGROUND: Impaired wound re-epithelialization contributes to cutaneous barrier reconstruction dysfunction. Recently, N6-methyladenosine (m6A) RNA modification has been shown to participate in the determination of RNA fate, and its aberration triggers the pathogenesis of numerous diseases. Howbeit, the function of m6A in wound re-epithelialization remains enigmatic. METHODS: Alkbh5‒/‒ mouse was constructed to study the rate of wound re-epithelialization after ALKBH5 ablation. Integrated high-throughput analysis combining methylated RNA immunoprecipitation sequencing (MeRIP-seq) and RNA-seq was used to identify the downstream target of ALKBH5. In vitro and in vivo rescue experiments were conducted to verify the role of the downstream target on the functional phenotype of ALKBH5-deficient cells or animals. Furthermore, the interacting reader protein and regulatory mechanisms were determined through RIP-qPCR, RNA pull-down, and RNA stability assays. RESULTS: ALKBH5 was specifically upregulated in the wound edge epidermis. Ablation of ALKBH5 suppressed keratinocyte migration and resulted in delayed wound re-epithelialization in Alkbh5‒/‒ mouse. Integrated high-throughput analysis revealed that PELI2, an E3 ubiquitin protein ligase, serves as the downstream target of ALKBH5. Concordantly, exogenous PELI2 supplementation partially rescued keratinocyte migration and accelerated re-epithelialization in ALKBH5-deficient cells, both in vitro and in vivo. In terms of its mechanism, ALKBH5 promoted PELI2 expression by removing the m6A modification from PELI2 mRNA and enhancing its stability in a YTHDF2-dependent manner. CONCLUSIONS: This study identifies ALKBH5 as an endogenous accelerator of wound re-epithelialization, thereby benefiting the development of a reprogrammed m6A targeted therapy for refractory wounds.

4.
Small ; 19(44): e2303586, 2023 Nov.
Article in English | MEDLINE | ID: mdl-37386814

ABSTRACT

Piezocatalysis is an emerging technique that holds great promise for the conversion of ubiquitous mechanical energy into electrochemical energy through piezoelectric effect. However, mechanical energies in natural environment (such as wind energy, water flow energy, and noise) are typically tiny, scattered, and featured with low frequency and low power. Therefore, a high response to these tiny mechanical energies is critical to achieving high piezocatalytic performance. In comparison to nanoparticles or 1D piezoelectric materials, 2D piezoelectric materials possess characteristics such as high flexibility, easy deformation, large surface area, and rich active sites, showing more promise in future for practical applications. In this review, state-of-the-art research progresses on 2D piezoelectric materials and their applications in piezocatalysis are provided. First, a detailed description of 2D piezoelectric materials are offered. Then a comprehensive summary of the piezocatalysis technique is presented and examines the piezocatalysis applications of 2D piezoelectric materials in various fields, including environmental remediation, small-molecule catalysis, and biomedicine. Finally, the main challenges and prospects of 2D piezoelectric materials and their applications in piezocatalysis are discussed. It is expected that this review can fuel the practical application of 2D piezoelectric materials in piezocatalysis.

5.
J Colloid Interface Sci ; 646: 159-166, 2023 Sep 15.
Article in English | MEDLINE | ID: mdl-37187049

ABSTRACT

Developing piezocatalysts with excellent piezocatalytic hydrogen evolution reaction (HER) performance is highly desired but also challenging. Here, facet engineering and cocatalyst engineering are employed to synergistically improve the piezocatalytic HER efficiency of BiVO4 (BVO). Monoclinic BVO catalysts with distinct exposed facets are synthesized by adjusting pH of hydrothermal reaction. The BVO with highly exposed {110} facet exhibits a superior piezocatalytic HER performance (617.9 µmol g-1h-1) compared with that with {010} facet, owing to the strong piezoelectric property, high charge transfer efficiency, and excellent hydrogen adsorption/desorption capacity. The HER efficiency is enhanced by 44.7% by selectively depositing cocatalyst of Ag nanoparticles specifically on the reductive {010} facet of BVO, where the Ag-BVO interface provides the directional electron transport for high-efficiency charge separation. Under the collaboration between cocatalyst of CoOx on {110} facet and the hole sacrificial agent of methanol, the piezocatalytic HER efficiency is evidently enhanced by 2 times because CoOx and methanol can impede the water oxidation and improve the charge separation. This easy and simple strategy provides an alternative perspective on designing high-performance piezocatalysts.

6.
Plast Reconstr Surg ; 147(5): 1105-1115, 2021 May 01.
Article in English | MEDLINE | ID: mdl-33890892

ABSTRACT

BACKGROUND: Vascular supercharge and flap prefabrication are two surgical maneuvers to improve flap blood supply. Although these techniques have been studied intensively, few studies have focused on the differences between supercharge and prefabricated flaps regarding their flap survival areas, vasculatures, and hemodynamics. METHODS: In this study, 21 male Sprague-Dawley rats were divided into three groups as follows: group A, single perforator flap; group B, supercharge flap; and group C, prefabricated flap. Flap survival was measured 1 week after flap elevation. Indocyanine green angiography was applied to visualize flap vascularity and to analyze flap hemodynamics. Von Willebrand factor immunohistochemical staining was applied to assess the number of microvessels in the choke zone of the abdominal wall. RESULTS: The flap survival areas were expanded significantly in the arteriovenous supercharge group and the vascular bundle prefabricated group compared with that in the single-perforator group (81.34 ± 8.12 percent and 75.51 ± 8.08 percent versus 46.27 ± 10.01 percent, respectively; p < 0.05). Hemodynamic analysis suggested that although a significant increase in arterial infusion could be achieved with flap prefabrication, the venous effusion of the prefabricated flap was the worst among the three groups, indicating greater susceptibility to compromised venous return. Active neovascularization was confirmed by an increased number of microvessels in group C. Specifically, the dilatation of choke vessels and the newly formed vessels of the prefabricated pedicle could be appreciated by indocyanine green angiographic mapping. CONCLUSIONS: Both vascular supercharge and flap prefabrication can augment the blood supply of the perforator flap but by means of different mechanisms. Because a supercharge flap is less susceptible to venous compromise, it is suggested to first consider the use of vascular supercharging when feasible.


Subject(s)
Perforator Flap/blood supply , Animals , Male , Models, Animal , Rats , Rats, Sprague-Dawley , Plastic Surgery Procedures/methods , Vascular Surgical Procedures/methods
7.
Nanotechnology ; 32(21)2021 Mar 03.
Article in English | MEDLINE | ID: mdl-33556929

ABSTRACT

In this work, high-dielectric-constant (high-k) erbium oxide(Er2O3)film is fabricated using the spin coating method, and annealed at a series of temperatures (from 400 °C to 700 °C). The effect of annealing temperature on the microstructural and electrical properties of Er2O3nanofilm is investigated. To demonstrate the applicability of the Er2O3film, the indium oxide (In2O3) thin film transistor (TFT)-based amorphous Er2O3dielectric film is fabricated at different temperatures. The TFT-based EO-600 shows a low-operating voltage and good electrical properties. The inverter demonstrates that the Er2O3nanofilm synthesized by the sol-gel method could be a promising candidate as the dielectric layer in a low-voltage electronic device.

8.
ACS Appl Mater Interfaces ; 12(15): 17443-17451, 2020 Apr 15.
Article in English | MEDLINE | ID: mdl-32195558

ABSTRACT

Piezocatalysts have attracted much attention due to their excellent degradation ability for organics. In this work, three types of BaTiO3 (BTO) nanostructures, including hydrothermally synthesized nanocubes (NCs), sol-gel calcined nanoparticles (NPs), and electrospun nanofibers (NFs), are prepared for catalyzing the dye degradation. Compared with the NCs and NPs, the NFs exhibit a higher piezocatalytic degradation performance due to the large specific surface area, fine crystal size, and easy deformation structure. Moreover, the kinetic factors, including initial dye concentration, ionic strength, ultrasonic power, and applied action, influencing the degradation performance of the BTO NFs are analyzed deeply. A high degradation rate constant of 0.0736 min-1 is achieved for rhodamine B, which is superior compared with the previous reports. The excellent stability of BTO NFs is demonstrated by the cycling tests, where a high degradation efficiency of 97.6% within 110 min is still obtained after the third cycle. Furthermore, the mechanism of piezocatalysis revealed that the hydroxyl and superoxide radicals are the main reactive species in the degradation process. This work is of importance for the development of high-performance piezocatalysts and highlights the potential of piezocatalysis for water remediation.

9.
Beilstein J Nanotechnol ; 9: 2788-2793, 2018.
Article in English | MEDLINE | ID: mdl-30498651

ABSTRACT

The wastage of near-infrared light seriously restricts the photoelectric conversion efficiency of hydrogenated amorphous silicon (a-Si:H) thin film solar cells. Spectral upconversion is of great significance in reducing the wastage. Herein, the upconverting compound NaYF4:Yb3+/Er3+ was synthesized via a hydrothermal method. SEM and XRD results revealed the morphology and a phase transition from cubic to hexagonal NaYF4. Photoluminescence spectra indicated that the hexagonal NaYF4:Yb3+/Er3+ nanorods convert near-infrared light of 980 nm to the visible light with wavelength peaks at 654, 541 and 522 nm. Hence, the upconverting rods were incorporated in a polymethylmethacrylate (PMMA) layer on the rear side of a-Si:H solar cell. Under AM1.5 solar irradiation, a facile optical filter was used to scrutinize the effect of upconversion on the cell performance. Compared with a bare cell, the NaYF4:Yb3+/Er3+-based a-Si:H cell exhibited an 25% improved short-circuit current and an appreciable improvement of the near-infrared response of the external quantum efficiency. Moreover, because the size of the nanorods is comparable to the wavelength of visible light, the rods effectively scattered light, thus enhancing the visible light harvesting.

10.
Chemistry ; 22(31): 10877-83, 2016 Jul 25.
Article in English | MEDLINE | ID: mdl-27346720

ABSTRACT

SnFe2 O4 nanocrystals (NC), prepared with a simple one-step carrier-solvent-assisted interfacial reaction process, were developed as highly efficient catalysts for hydrogen peroxide sensing. These NCs, with a size of around 7 nm, served as the sensing catalyst and were decorated onto the pore surfaces of a porous fluorine-doped tin oxide (PFTO) host electrode, prepared from commercial FTO glass with a simple anodic treatment, to form the sensing electrode for hydrogen peroxide. The SnFe2 O4 NCs-loaded PFTO electrode exhibited an ultra-high sensitivity of 1027 mA m(-1) cm(-2) toward hydrogen peroxide, outperforming Pt NCs-loaded PFTO electrodes. The SnFe2 O4 NCs-loaded PFTO electrode proved a promising relatively low cost, high performance sensing electrode for hydrogen peroxide.

11.
Opt Lett ; 40(22): 5180-3, 2015 Nov 15.
Article in English | MEDLINE | ID: mdl-26565829

ABSTRACT

Efficient light management for micromorph tandem solar cells is achieved in this Letter by the combined application of TiO(2) and SiO(x) interlayers. Here, TiO(2) is incorporated into a ZnO/a-Si interface as an antireflection layer and SiO(x) is incorporated into an a-Si/µc-Si interface as an intermediate reflecting layer. Solar cells with such architecture not only increase the light absorption but also reduce the mismatch losses of current between the top and bottom cells. The key results, as evidenced by the spectral response measurements, are that the total photocurrent increases from 22.62 to 24.35 mA/cm(2), as well as the short circuit current density of the two component cells is reached to a delicate balance. The influences of the interlayer thickness and morphology on the improvement have been investigated using an electromagnetic simulation in order to take full advantage of this design.

12.
Opt Lett ; 40(7): 1290-3, 2015 Apr 01.
Article in English | MEDLINE | ID: mdl-25831315

ABSTRACT

Here we report on an efficient light-coupling scheme with a periodic microstructured surface to enhance the performance of thin film silicon solar cells. The centerpiece of the surface structure is the hemispherical pit arrays (HPAs), which are fabricated using an inexpensive and scalable process. The integration of HPAs into micromorph tandem thin film silicon solar cells leads to superior broadband reflection suppression properties. With this design, the reflection losses of the tandem cell are reduced to only 1.5%. We demonstrate an efficiency increase from 11.67% to 12.23% compared to a conventional cell with a flat surface, with a 4.6% increase in short circuit current density. The surface microstructures reported here can be applied to a variety of photovoltaic devices to further improve their performance.

13.
Cancer Biol Ther ; 6(10): 1539-45, 2007 Oct.
Article in English | MEDLINE | ID: mdl-18293492

ABSTRACT

CIAPIN1, a newly identified apoptosis-related molecule, was found to be downregulated in human gastric cancer tissues as compared to the matched adjacent nonneoplastic tissues. In this study, we investigated the effect of CIAPIN1 on in vitro and in vivo proliferation of gastric cancer cells. Ectopic expression and knockdown of CIAPIN1 in gastric cancer cells SGC7901 and MKN45 were achieved by transduction with recombinant adenoviruses expressing human CIAPIN1 (Ad-CIAPIN1) and human CIAPIN1-specific small interference RNA (Ad-CIAPIN1 siRNA). Gastric cancer cells with upregulated expression of CIAPIN1 exhibited significantly decreased proliferation, while cellswith downregulated CIAPIN1 expression showed significantly quicker growth rate as compared with their respective controls in both in vitro and in vivo tests. Also, CIAPIN1suppressed colony formation of SGC7901 and MKN45 cells in soft agar cloning test.Furthermore, cell cycle distribution analysis revealed that CIAPIN1 induced cell cycle arrest at G1/S phase. Downregulation of CyclyinD1 and upregulation of P27 might contribute, at least in part, to this altered cell cycle distribution. This study demonstrates that CIAPIN1 is a suppressor of gastric cancer cell proliferation and suggests CIAPIN1might play an important role in the development of human gastric cancer.


Subject(s)
Cyclin D1/metabolism , Cyclin-Dependent Kinase Inhibitor p27/metabolism , Intracellular Signaling Peptides and Proteins/physiology , Stomach Neoplasms/genetics , Tumor Suppressor Proteins/physiology , Cell Cycle , Cell Line, Tumor , Cell Proliferation , Down-Regulation , Humans , Intracellular Signaling Peptides and Proteins/antagonists & inhibitors , Intracellular Signaling Peptides and Proteins/genetics , RNA, Small Interfering/pharmacology , Stomach Neoplasms/metabolism , Stomach Neoplasms/pathology , Transduction, Genetic , Tumor Suppressor Proteins/antagonists & inhibitors , Tumor Suppressor Proteins/genetics , Up-Regulation
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