Dispersion-assisted high-dimensional photodetector.

Intensity, polarization and wavelength are intrinsic characteristics of light. Characterizing light with arbitrarily mixed information on polarization and spectrum is in high demand1-4. Despite the extensive efforts in the design of polarimeters5-18 and spectrometers19-27, concurrently yielding high-dimensional signatures of intensity, polarization and spectrum of the light fields is challenging and typically requires complicated integration of polarization- and/or wavelength-sensitive elements in the space or time domains. Here we demonstrate that simple thin-film interfaces with spatial and frequency dispersion can project and tailor polarization and spectrum responses in the wavevector domain. By this means, high-dimensional light information can be encoded into single-shot imaging and deciphered with the assistance of a deep residual network. To the best of our knowledge, our work not only enables full characterization of light with arbitrarily mixed full-Stokes polarization states across a broadband spectrum with a single device and a single measurement but also presents comparable, if not better, performance than state-of-the-art single-purpose miniaturized polarimeters or spectrometers. Our approach can be readily used as an alignment-free retrofit for the existing imaging platforms, opening up new paths to ultra-compact and high-dimensional photodetection and imaging.

Photogating-assisted tunneling boosts the responsivity and speed of heterogeneous WSe2/Ta2NiSe5 photodetectors.

Photogating effect is the dominant mechanism of most high-responsivity two-dimensional (2D) material photodetectors. However, the ultrahigh responsivities in those devices are intrinsically at the cost of very slow response speed. In this work, we report a WSe2/Ta2NiSe5 heterostructure detector whose photodetection gain and response speed can be enhanced simultaneously, overcoming the trade-off between responsivity and speed. We reveal that photogating-assisted tunneling synergistically allows photocarrier multiplication and carrier acceleration through tunneling under an electrical field. The photogating effect in our device features low-power consumption (in the order of nW) and shows a dependence on the polarization states of incident light, which can be further tuned by source-drain voltages, allowing for wavelength discrimination with just a two-electrode planar structure. Our findings offer more opportunities for the long-sought next-generation photodetectors with high responsivity, fast speed, polarization detection, and multi-color sensing, simultaneously.

Asymptotic dispersion engineering for ultra-broadband meta-optics.

Dispersion decomposes compound light into its monochromatic components, which is detrimental to broadband imaging but advantageous for spectroscopic applications. Metasurfaces provide a unique path to modulate the dispersion by adjusting structural parameters on a two-dimensional plane. However, conventional linear phase compensation does not adequately match the meta-unit's dispersion characteristics with required complex dispersion, hindering at-will dispersion engineering over a very wide bandwidth particularly. Here, we propose an asymptotic phase compensation strategy for ultra-broadband dispersion-controlled metalenses. Metasurfaces with extraordinarily high aspect ratio nanostructures have been fabricated for arbitrary dispersion control in ultra-broad bandwidth, and we experimentally demonstrate the single-layer achromatic metalenses in the visible to infrared spectrum (400 nm~1000 nm, NA = 0.164). Our proposed scheme provides a comprehensive theoretical framework for single-layer meta-optics, allowing for arbitrary dispersion manipulation without bandwidth restrictions. This development is expected to have significant applications in ultra-broadband imaging and chromatography detection, among others.

Polychromatic full-polarization control in mid-infrared light.

Objects with different shapes, materials and temperatures can emit distinct polarizations and spectral information in mid-infrared band, which provides a unique signature in the transparent window for object identification. However, the crosstalk among various polarization and wavelength channels prevents from accurate mid-infrared detections at high signal-to-noise ratio. Here, we report full-polarization metasurfaces to break the inherent eigen-polarization constraint over the wavelengths in mid-infrared. This recipe enables to select arbitrary orthogonal polarization basis at individual wavelength independently, therefore alleviating the crosstalk and efficiency degradation. A six-channel all-silicon metasurface is specifically presented to project focused mid-infrared light to distinct positions at three wavelengths, each with a pair of arbitrarily chosen orthogonal polarizations. An isolation ratio of 117 between neighboring polarization channels is experimentally recorded, exhibiting detection sensitivity one order of magnitude higher than existing infrared detectors. Remarkably, the high aspect ratio ~30 of our meta-structures manufactured by deep silicon etching technology at temperature -150 °C guarantees the large and precise phase dispersion control over a broadband from 3 to 4.5 µm. We believe our results would benefit the noise-immune mid-infrared detections in remote sensing and space-to-ground communications.

Single-shot isotropic differential interference contrast microscopy.

Differential interference contrast (DIC) microscopy allows high-contrast, low-phototoxicity, and label-free imaging of transparent biological objects, and has been applied in the field of cellular morphology, cell segmentation, particle tracking, optical measurement and others. Commercial DIC microscopy based on Nomarski or Wollaston prism resorts to the interference of two polarized waves with a lateral differential offset (shear) and axial phase shift (bias). However, the shear generated by these prisms is limited to the rectilinear direction, unfortunately resulting in anisotropic contrast imaging. Here we propose an ultracompact metasurface-assisted isotropic DIC (i-DIC) microscopy based on a grand original pattern of radial shear interferometry, that converts the rectilinear shear into rotationally symmetric along radial direction, enabling single-shot isotropic imaging capabilities. The i-DIC presents a complementary fusion of typical meta-optics, traditional microscopes and integrated optical system, and showcases the promising and synergetic advancements in edge detection, particle motion tracking, and label-free cellular imaging.

Deep-Learning-Empowered Holographic Metasurface with Simultaneously Customized Phase and Amplitude.

Metasurfaces with simultaneously and independently controllable amplitude and phase have provided a higher degree of freedom in manipulating electromagnetic (EM) waves. Compared with phase- or amplitude-only modulation, the capability of simultaneously controlling the phase and amplitude of EM waves can enable holography with a higher resolution. However, this drastically increases the design complexity of holographic metasurfaces, and the design process is usually quite time-consuming. In this paper, we propose an inverse design of meta-atoms that can simultaneously and independently tailor the phase and amplitude of transmitted waves using customized deep ResNet while eliminating the coupling of parameters. To demonstrate the design method, two holographic metasurfaces were designed using the trained network without the need for parameter sweeping, which will significantly enhance design efficiency. Prototypes were fabricated and measured. Both the simulated and measured results show that high-resolution holography is obtained, which sufficiently verifies the reliability of the design method. Our work paves the way for the intelligent design of metasurfaces and can also be applied to the design of other artificial materials or surfaces.

Relative-phase simulated annealing for time-efficient and large-scale inverse design of achromatic thin lenses.

High-efficiency, broadband, wafer-size, and ultra-thin lenses are highly demanded, due to its great potential in abundant applications such as compact imaging modules. It is usually conceived that this target might be attainable given the advancement in nanofabrication, computation power and emerging algorithms, though challenging. Here, we reveal the inconvenient truth that for ultra-thin lenses, there actually exists intrinsic check-and-balance between size, broadband and performance. Unveiled by our inverse design algorithm, Relative-Phase Simulated Annealing (RPSA), focusing efficiency inevitably drops with refining wavelength intervals for better achromatic broadband features in optimized lens; and drops exponentially with increasing diameter and bandwidth, supported by our empirical formula. Meanwhile, with a slightly compromised goal, the powerfulness of RPSA is unlocked since it could provide a globally optimized design recipe whose time complexity relates to lens scale linearly rather than exponentially. This work, as a fast search engine for optimal solutions, paves the way towards practical large-scale achromatic ultra-thin lenses.

Molding Broadband Dispersion in Twisted Trilayer Hyperbolic Polaritonic Surfaces.

Recent advancement in twisted layered metasurfaces can be employed to control the nanoscale flow of light, including the exotic hyperbolic-to-elliptic topological transitions in twisted bilayers (tBL). Such topological transitions can only occur to limited frequency ranges, restricted by the intrinsic in-plane dispersion of individual hyperbolic surfaces. Here, we report that, by controlling interlayer evanescent coupling in twisted polaritonic trilayers, moldable topological transitions of light can be achieved in broadband. We reveal that the required minimum open angle of the individual hyperbolic polaritonic surface for open-to-close topological transitions can be significantly lowered compared to that of the twisted bilayer counterpart. This increases the degree of freedom to enhance and control near-field light-matter interactions and energy management. As an example, we demonstrate a knob to manipulate near-field radiative heat transfer (NFRHT). By rotating the relative angles of trilayers, exotic and tunable thermal conductance can be achieved. Our findings enrich the controllability of light at the nanoscale in broadband, bringing twisted optical materials one step closer to practical applications.