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Productive trapping of NAD-type radicals. Non-biomimetic reduction of pyridinium salts.
Lavilla, Rodolfo; Bernabeu, M Carmen; Brillas, Enric; Carranco, Inés; Díaz, José Luis; Llorente, Nereida; Rayo, Marta; Spada, Alessandro.
Chem Commun (Camb) ; (8): 850-1, 2002 Apr 21.
Article in English | MEDLINE | ID: mdl-12123010

ABSTRACT

One-electron reduction of pyridinium salts (NAD+ analogues) generates dihydropyridyl radicals which may then be engaged in radical addition processes to regioselectively form gamma-substituted dihydropyridines.


Subject(s)
Electrons , Pyridinium Compounds/chemistry , Free Radicals , Kinetics , Models, Chemical , NAD , Niacinamide/analogs & derivatives , Oxidation-Reduction
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