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1.
Opt Lett ; 44(6): 1435-1438, 2019 Mar 15.
Article in English | MEDLINE | ID: mdl-30874669

ABSTRACT

We demonstrate time-resolved temperature measurements in shock-heated mixtures of carbon monoxide over a temperature range of 1000-1800 K for two pressure ranges, 2.0-2.9 atm and 7.6-10.7 atm, at rates up to 250 kHz using a single acousto-optically modulated quantum cascade laser with mid-infrared output spanning from 1975 to 2260 cm-1. Measured temperatures were in excellent agreement with values determined by ideal shock relations, and the temperature profile after the passage of the reflected shock wave was found to be well-modeled by an isentropic compression assumption. Temperature measurements made with this setup are largely immune to effects of emissions and beam steering, making the diagnostic system well-suited for studying high-temperature gas-phase reactions of energetic materials such as octahydro-1,3,5,7-tetranitro-1,3,5,7-tetrazocine and hexahydro-1,3,5-trinitro-1,3,5-triazine.

2.
Opt Lett ; 43(1): 21, 2018 Jan 01.
Article in English | MEDLINE | ID: mdl-29328223

ABSTRACT

This erratum reports a correction to the labeling of Figs. 2(b) and 3(b) in the original manuscript, Opt. Lett.42, 4756 (2017)OPLEDP0146-959210.1364/OL.42.004756.

3.
Opt Lett ; 42(22): 4756-4759, 2017 11 15.
Article in English | MEDLINE | ID: mdl-29140361

ABSTRACT

We report an octave-wide mid-IR spectrum (2.3-4.8 µm) obtained from a subharmonic optical parametric oscillator (OPO) based on a newly developed nonlinear crystal, orientation-patterned gallium phosphide (OP-GaP), which was synchronously pumped by a femtosecond 1560 nm fiber laser. We proved that the octave-wide output is in the form of a single frequency comb. The observed f-to-2f frequency beats, originating directly from the OPO, can be used for self-referencing and phase locking of the pump laser comb with no need for supercontinuum generation. With an average output power of ∼30 mW, this setup might be beneficial for a variety of spectroscopic applications in the mid-IR.

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