Generation of THz radiation through molecular modulation in hydrogen-filled hybrid anti-resonant fibers.

We study the generation of narrowband terahertz (THz) pulses by stimulated Raman scattering and molecular modulation in hydrogen-filled hybrid hollow-core fibers. Using a judicious combination of materials and transverse structures, this waveguide design enables simultaneous confinement of optical and THz signals with reasonably low attenuation, as well as high nonlinear overlap. The THz pulses are then generated as the second Stokes band of a ns-long near-infrared pump pulse, aided by Raman coherence waves excited in the gaseous core by the beat-note created by the pump and its first Stokes band. Optimization of the fiber characteristics facilitates phase matching between the corresponding transitions and coherence waves while avoiding coherent gain suppression, resulting in potential optical-to-THz conversion efficiencies up to 60%, as confirmed by rigorous numerical modelling under ideal zero-loss conditions. When the current optical material constraints are considered, however, the attainable efficiencies relax to 0.2%, a still competitive value compared to other systems. The approach is in principle power and energy scalable, as well as tunable in the 1-10 THz range without any spectral gaps, thereby opening new pathways to the development of fiber-based THz sources complementary to other mature technologies such as quantum cascade lasers.

Effect of Photoinitiators Doped in PDMS for Femtosecond-Laser Writing: Characterization and Outcomes.

Herein, we have characterized in depth the effect of femtosecond (fs)-laser writing on various polydimethylsiloxane (PDMS)-based composites. The study combines systematic and nanoscale characterizations for the PDMS blends that include various photoinitiators (organic and inorganic agents) before and after fs-laser writing. The results exhibit that the photoinitiators can dictate the mechanical properties of the PDMS, in which Young's modulus of PDMS composites has higher elasticity. The study illustrates a major improvement in refractive index change by 15 times higher in the case of PDMS/BP-Ge [benzophenone (BP) allytriethylgermane] and Irgacure 184. Additional enhancement was achieved in the optical performance levels of the PDMS composites (the PDMS composites of Irgacure 184/500, BP-Ge, and Ge-ATEG have a relative difference of less than 5% in comparison with pristine PDMS), which are on par with glasses. This insightful study can guide future investigators in choosing photoinitiators for particular applications in photonics and polymer chemistry.

Fs laser written volume Raman-Nath grating for integrated spectrometer on smartphone.

In this work we demonstrate the integration of a spectrometer directly into smartphone screen by femtosecond laser inscription of a weak Raman-Nath volume grating either into the Corning Gorilla glass screen layer or in the tempered aluminosilicate glass protector screen placed in front of the phone camera. Outside the thermal accumulation regime, a new writing regime yielding positive refractive index change was found for both glasses which is fluence dependent. The upper-bound threshold for this thermal-accumulation-less writing regime was found for both glasses and were, respectively at a repetition rate less than 150 kHz and 101 kHz for fluence of 8.7 × 106 J/m2 and 1.4 × 107 J/m2. A weak volume Raman-Nath grating of dimension 0.5 by 3 mm and 3 µm pitch was placed in front of a Samsung Galaxy S21 FE cellphone to record the spectrum using the 2nd diffraction order. This spectrometer covers the visible band from 401 to 700 nm with a 0.4 nm/pixel detector resolution and 3 nm optical resolution. It was used to determine the concentration detection limit of Rhodamine 6G in water which was found to be 0.5 mg/L. This proof of concept paves the way to in-the-field absorption spectroscopy for quick information gathering.

Femtosecond laser direct-writing of high quality first-order Bragg gratings with arbitrary complex apodization by phase modulation.

Femtosecond laser direct-writing is an attractive technique to fabricate fiber Bragg gratings and to achieve through-the-coating inscription. In this article, we report the direct inscription of high-quality first-order gratings in optical fiber, without the use of an index-matching medium. A new alignment technique based on the inscription of weak probe gratings is used to track the relative position between the focal spot and fiber core. A simple and flexible method to precisely control the position of each grating plane is also presented. With this method, periodic phase modulation of grating structures is achieved and used to inscribe arbitrary apodization and phase profiles. It is shown that a burst of multiple laser pulses used to inscribe each grating plane leads to a significant increase in the grating strength, while maintaining low insertion loss, critical for many applications.

Photosensitization agents for fs laser writing in PDMS.

This study aims at identifying compounds incorporated into Polydimethylsiloxane (PDMS) which produce large refractive index change under fs laser exposition, potentially leading to optimal writing of waveguides or photonic devices in such a soft host. Germanium derivative, titania and zirconite derivatives, benzophenone (Bp), irgacure-184/500/1173 and 2959 are investigated. We show a mapping of the RI index change relative to the writing speed (1 to 40 mm/s), the repetition rate (606 to 101 kHz) and the number of passes (1 to 8) from which we establish quantitative parameters to allow the comparison between samples. We show that the organic materials, especially irgacure-184 and benzophenone yield a significantly higher maximum refractive index change in the order of 10-2. We also show that the strongest photosensitivity is achieved with a mixture of organic/organo-metallic material of Bp + Ge. We report a synergetic effect on photosensitivity of this novel mixture.

Structural and optical properties of Nd:YAB-nanoparticle-doped PDMS elastomers for random lasers.

We report the structural and optical properties of Nd:YAB (NdxY1-x Al3(BO3)4)-nanoparticle-doped PDMS elastomer films for random lasing (RL) applications. Nanoparticles with Nd ratios of x = 0.2, 0.4, 0.6, 0.8, and 1.0 were prepared and then incorporated into the PDMS elastomer to control the optical gain density and scattering center content over a wide range. The morphology and thermal stability of the elastomer composites were studied. A systematic investigation of the lasing wavelength, threshold, and linewidth of the laser was carried out by tailoring the concentration and optical gain of the scattering centers. The minimum threshold and linewidth were found to be 0.13 mJ and 0.8 nm for x = 1 and 0.8. Furthermore, we demonstrated that the RL intensity was easily tuned by controlling the degree of mechanical stretching, with strain reaching up to 300%. A strong, repeatable lasing spectrum over ~ 50 cycles of applied strain was observed, which demonstrates the high reproducibility and robustness of the RL. In consideration for biomedical applications that require long-term RL stability, we studied the intensity fluctuation of the RL emission, and confirmed that it followed Lévy-like statistics. Our work highlights the importance of using rare-earth doped nanoparticles with polymers for RL applications.

The ROGUE: a novel, noise-generated random grating.

We propose a novel device defined as Random Optical Grating by Ultraviolet or ultrafast laser Exposure (ROGUE), a new type of fiber Bragg grating (FBG), exhibiting a weak reflection over a large bandwidth, which is independent of the length of the grating. This FBG is fabricated simply by dithering the phase randomly during the writing process. This grating has an enhanced backscatter, several orders of magnitude above typical Rayleigh backscatter of standard SMF-28 optical fiber. The grating is used in distributed sensing using optical frequency domain reflectometry (OFDR), allowing a significant increase in signal to noise ratio for strain and temperature measurement. This enhancement results in significantly lower strain or temperature noise level and accuracy error, without sacrificing the spatial resolution. Using this method, we show a sensor with a backscatter level 50 dB higher than standard unexposed SMF-28, which can thus compensate for increased loss in the system.

Spatially resolved cross-sectional refractive index profile of fs laser-written waveguides using a genetic algorithm.

Laser-written waveguides in glass have many potential applications as photonic devices. However, there is little knowledge of the actual profile of the usually asymmetric refractive index (RI) change across the femtosecond (fs) laser-written waveguides. We show, here, a new nondestructive method to measure any symmetric or asymmetric two-dimensional RI profile of fs laser-written waveguides in transparent materials. The method is also suitable for the measurement of the RI profile of any other type of waveguide. A Mach-Zehnder interferometer is used to obtain the phase shift of light propagating transversely through the RI-modified region. A genetic algorithm is then used to determine the matching cross-sectional RI profile based on the known waveguide shape and dimensions. A validation of the method with the comparison to a RNF measurement of the industry-standard SMF-28 is presented, as well as a demonstration of its versatility with measurements on fs laser-written waveguides.

Intra-Arterial Image Guidance With Optical Frequency Domain Reflectometry Shape Sensing.

Intra-arterial liver cancer therapies, such as trans-arterial chemoembolization, are the preferred therapeutic approaches for advanced hepatocellular carcinoma. However, these palliative techniques are challenging for delivering therapeutic agents selectively in the tumor without real-time 3-D visualization of the catheter within the hepatic arteries. The objective of this paper is to develop and evaluate in pre-clinical tests an advanced interventional guidance platform using a distributed strain sensing device based on optical frequency-domain reflectometry (OFDR) to track the tip and shape of a catheter. The scattering properties of a fiber triplet are enhanced by focusing an ultraviolet beam on these fibers, producing a fully distributed strain sensor, which avoids interpolation errors observed with traditional shape tracking systems. A 3-D roadmap of the hepatic arteries is obtained from a combined fully convolutional and residual networks trained on MR angiography and combined with a 4-D flow dynamic sequence enabling to map blood flow velocities. An anisotropic curvature matching method is proposed to map the sensed data onto pre-operative MR and using 3-D ultrasound to correct for non-rigid deformations. Experiments were conducted in a controlled environment setting as well as in both synthetic phantoms and in five porcine models to assess the performance for device navigation, yielding satisfactory tracking accuracy with 3-D mean errors of 2.8 ± 0.9 mm. We present the first pilot study of MR-compatible UV-exposed OFDR optical fibers for non-ionizing device guidance in intra-arterial procedures, with the potential of avoiding multiple hospitalizations required to perform invasive selective chemoembolizations.

Efficiency increase of distributed feedback Raman fiber lasers by dynamic control of the phase shift.

π-phase-shifted distributed feedback, ultralong fiber Bragg gratings (FBGs) with Raman gain have been shown to be excellent ultranarrow single-frequency lasers that can be operated at any wavelength. However, these lasers have shown unusually low slope efficiency (1%-10%), while theoretical simulations predict a much higher (30%-60%) number. We believe this poor performance is due to a thermally induced phase shift inside the FBG due to absorption of the high intensity of the signal oscillating in the cavity. To compensate for this, a thermally controlled dynamic phase shift is proposed to increase efficiency after lasing first occurs. We show here an increase in the slope efficiency of a factor of 4 and an increase in the total output efficiency by a factor of 6.5 with 6 W of pump power by reducing the phase shift once the laser begins oscillating.

Single-frequency low-threshold linearly polarized DFB Raman fiber lasers.

Distributed feedback (DFB) fiber lasers have been demonstrated to be excellent narrow-linewidth (kilohertz range) single-frequency laser sources. However, this type of laser is normally limited to rare-earth-doped fibers. Raman gain offers an alternative, operating at any arbitrary wavelength. We demonstrate here linearly polarized, single-frequency, DFB fiber Bragg grating Raman lasers with, to the best of our knowledge, the lowest pump threshold of 350 mW, an output power of up to 50 mW at 1120 nm, an 8.5% slope efficiency, and 300 mW of output power at 1178 nm. In the high-power regime, stimulated Brillouin scattering plays an important role in the laser dynamics. We also report the characterization of the power profile inside the fiber along its axis through a novel side-scatter technique.

Enhancement of accuracy in shape sensing of surgical needles using optical frequency domain reflectometry in optical fibers.

We demonstrate a novel approach to enhance the precision of surgical needle shape tracking based on distributed strain sensing using optical frequency domain reflectometry (OFDR). The precision enhancement is provided by using optical fibers with high scattering properties. Shape tracking of surgical tools using strain sensing properties of optical fibers has seen increased attention in recent years. Most of the investigations made in this field use fiber Bragg gratings (FBG), which can be used as discrete or quasi-distributed strain sensors. By using a truly distributed sensing approach (OFDR), preliminary results show that the attainable accuracy is comparable to accuracies reported in the literature using FBG sensors for tracking applications (~1mm). We propose a technique that enhanced our accuracy by 47% using UV exposed fibers, which have higher light scattering compared to un-exposed standard single mode fibers. Improving the experimental setup will enhance the accuracy provided by shape tracking using OFDR and will contribute significantly to clinical applications.

Are optical fibers really uniform? Measurement of refractive index on a centimeter scale.

Many applications of optical fiber, such as specialized fiber Bragg gratings (FBGs), require high uniformity of a fiber's refractive index (RI) along its length. We show here that the mode effective index of most fibers is not constant, even on a short length scale. To help improve fiber manufacturing and selection, we demonstrate a technique for characterizing a meter length single-mode optical fiber's effective RI over a centimeter scale with a precision of 3×10-6 RI units (RIUs) and an absolute accuracy of 2×10-4 RIU. By writing several weak probe FBGs as frequency references and then measuring the frequency deviation of these probe FBGs along the length of the fiber with an optical frequency domain reflectometer, the RI distribution of the effective mode index may be found. We validate our measurements on reference and fibers under test with theoretical simulations.

Stimulated Brillouin scattering in ultra-long distributed feedback Bragg gratings in standard optical fiber.

Distributed feedback (DFB) fiber Bragg gratings (FBG) are widely used as narrow-band filters and single-mode cavities for lasers. Recently, a nonlinear generation has been shown in 10-20 cm DFB gratings in a highly nonlinear fiber. First, we show in this Letter a novel fabrication technique of ultra-long DFBs in a standard fiber (SMF-28). Second, we demonstrate nonlinear generation in such gratings. A particular inscription technique was used to fabricate all-in-phase ultra-long FBG and to implement reproducible phase shift to form a DFB mode. We demonstrate stimulated Brillouin scattering (SBS) emission from this DFB mode and characterize the resulting laser. It seems that such a SBS based DFB laser stabilizes a pump's jittering and reduces its linewidth.

3D printed long period gratings for optical fibers.

We demonstrate a simple technique for implementing long period grating (LPG) structures by the use of a 3D printer. This Letter shows a way of manipulating the mode coupling within an optical fiber by applying stress through an external 3D printed periodic structure. Different LPG lengths and periods have been studied, as well as the effect of the applied stress on the coupling efficiency from the fundamental mode to cladding modes. The technique is very simple, highly flexible, affordable, and easy to implement without the need of altering the optical fiber. This Letter is part of a growing line of interest in the use of 3D printers for optical applications.

Fabrication of ultrafast laser written low-loss waveguides in flexible As2S3 chalcogenide glass tape.

As2S3 glass has a unique combination of optical properties, such as wide transparency in the infrared region and a high nonlinear coefficient. Recently, intense research has been conducted to improve photonic devices using thin materials. In this Letter, highly uniform rectangular single-index and 2 dB/m loss step-index optical tapes have been drawn by the crucible technique. Low-loss (<0.15 dB/cm) single-mode waveguides in chalcogenide glass tapes have been fabricated using femtosecond laser writing. Optical backscatter reflectometry has been used to study the origin of the optical losses. A detailed study of the laser writing process in thin glass is also presented to facilitate a repeatable waveguide inscription recipe.

Toward the integration of optical sensors in smartphone screens using femtosecond laser writing.

We demonstrate a new type of sensor incorporated directly into Corning Gorilla glass, an ultraresistant glass widely used in the screen of popular devices such as smartphones, tablets, and smart watches. Although physical space is limited in portable devices, the screens have been so far neglected in regard to functionalization. Our proof-of-concept shows a new niche for photonics device development, in which the screen becomes an active component integrated into the device. The sensor itself is a near-surface waveguide, sensitive to refractive index changes, enabling the analysis of liquids directly on the screen of a smartphone, without the need for any add-ons, thus opening this part of the device to advanced functionalization. The primary function of the screen is unaffected, since the sensor and waveguide are effectively invisible to the naked eye. We fabricated a waveguide just below the glass surface, directly written without any surface preparation, in which the change in refractive index on the surface-air interface changes the light guidance, thus the transmission of light. This work reports on sensor fabrication, using a femtosecond pulsed laser, and the light-interaction model of the beam propagating at the surface is discussed and compared with experimental measurement for refractive indexes in the range 1.3-1.7. A new and improved model, including input and output reflections due to the effective mode index change, is also proposed and yields a better match with our experimental measurements and also with previous measurements reported in the literature.

Rayleigh scatter based order of magnitude increase in distributed temperature and strain sensing by simple UV exposure of optical fibre.

We present a technique to improve signal strength, and therefore sensitivity in distributed temperature and strain sensing (DTSS) using Frequency domain Rayleigh scatter. A simple UV exposure of a hydrogen loaded standard SMF-28 fibre core is shown to enhance the Rayleigh back-scattered light dramatically by ten-fold, independent of the presence of a Bragg grating, and is therefore created by the UV exposure alone. This increase in Rayleigh back-scatter allows an order-of-magnitude increase in temperature and strain resolution for DTSS compared to un-exposed SMF-28 fibre used as a sensing element. This enhancement in sensitivity is effective for cm range or more sensor gauge length, below which is the theoretical cross-correlation limit. The detection of a 20 mK temperature rise with a spatial resolution of 2 cm is demonstrated. This gain in sensitivity for SMF-28 is compared with a high Ge doped photosensitive fibre with a characteristically high NA. For the latter, the UV enhancement is also present although of lower amplitude, and enables an even lower noise level for sensing, due to the fibre's intrinsically higher Rayleigh scatter signal.

Capacitors go optical: wavelength independent broadband mode cavity.

Fabry-Perot resonators or interferometers (FPI) have existed for a long time and act as light accumulators. However, their applications have been limited to the allowed resonance modes in the cavity, which are defined by the specific free-spectral range of the FPI. We show here a novel concept involving a light "capacitor" capable of accumulating light over a wide spectral range, at any given repetition frequency. This device is actually an FPI in which a high chirped mirror (chirped fiber Bragg grating or chirp multi-layer coated mirror) is added to remove the wavelength dependence of the mode resonances, enabling a single very large broad-band mode. This "modification" does not affect the amount of light which can be accumulated, i.e. it does not reduce the Q-factor of the cavity. We show here the theoretical concept of such a device and experimental results demonstrating this principle.

High-sensitivity temperature sensing using higher-order Stokes stimulated Brillouin scattering in optical fiber.

In an effort to reduce the cost of sensing systems and make them more compact and flexible, Brillouin scattering has been demonstrated as a useful tool, especially for distributed temperature and strain sensing (DTSS), with a resolution of a few centimeters over several tens of kilometers of fiber. However, sensing is limited by the Brillouin frequency shift's sensitivity to these parameters, which are of the order of ~1.3 MHz/°C and of ~0.05 MHz/µÎµ for standard fiber. In this Letter, we demonstrate a new and simple technique for enhancing the sensitivity of sensing by using higher-orders Stokes shifts with stimulated Brillouin scattering (SBS). By this method, we multiply the sensitivity of the sensor by the number of the Stokes order used, enhanced by six-fold, therefore reaching a sensitivity of ~7 MHz/°C, and potentially ~0.30 MHz/µÎµ. To do this, we place the test fiber within a cavity to produce a frequency comb. Based on a reference multiorder SBS source for heterodyning, this system should provide a new distributed sensing technology with significantly better resolution at a potentially lower cost than currently available DTSS systems.