A construction method of the quasi-monolithic compact interferometer based on UV-adhesive bonding.

Quasi-monolithic interferometers play a crucial role in high-precision measurement experiments, including gravitational wave detection, inertial sensing, vibrometry, and seismology. Achieving high stability and accuracy in such interferometers requires a method for bonding the optical components to a baseplate. While optical contact bonding and silicate bonding are common methods, UV adhesives offer advantages such as controlled curing and low geometrical requirements for optical components and baseplates. This paper presents a detailed construction method for a quasi-monolithic compact interferometer based on UV-adhesive bonding. We built two types of interferometers using this method: a 100 × 100 × 20 mm3 Mach-Zender homodyne interferometer with unequal arm lengths of about 100 mm for laser frequency noise monitoring and a heterodyne interferometer as a displacement sensing head, sizing 20 × 30 × 20 mm3. Our Mach-Zender interferometer achieved a phase noise level of 2µradHz at 1 Hz and an equivalent laser frequency noise monitoring sensitivity of about 1kHz/Hz at 1 Hz. The compact heterodyne interferometer sensing head showed a sensitivity level of 1pm/Hz in translation and 0.2nrad/Hz in two tilts above 0.4 Hz. Our tests demonstrate that quasi-monolithic compact interferometers based on UV-adhesive bonding can achieve high sensitivity levels at the pico-meter and nano-radian scales.

Pollutants from primary sources dominate the oxidative potential of water-soluble PM2.5 in Hong Kong in terms of dithiothreitol (DTT) consumption and hydroxyl radical production.

Increasing scientific findings show that the adverse health effects of PM2.5 are related not only to its mass but also PM2.5 sources and chemical compositions. Here, we conducted a comprehensive characterization and source apportionment of oxidative potential (OP) of water-soluble PM2.5 collected in Hong Kong for one year. Two OP indicators, namely dithiothreitol (DTT) consumption and ∙OH formation, were quantified. Six PM2.5 sources, i.e. secondary sulfate, biomass burning, secondary organic aerosol (SOA), vehicle emissions, marine vessels, and a metal-related factor, were apportioned and identified to be DTT active. The four primary sources accounted for 83.5% of DTT activity of water-soluble PM2.5, with the metal-related factor and marine vessels as the leading contributors. However, only three sources, i.e. metal-related factor, vehicle emissions, and SOA, showed ∙OH generation ability, with a predominant contribution of 96.2% from the two primary sources, especially the metal-related factor (84.5%). Based on the source apportionment results, we further evaluate the intrinsic OP of water-soluble PM2.5 from each source. Marine vessels exhibited the highest intrinsic DTT activity; while metal-related factor was most effective in ∙OH generation.

Correction to: Speciation of carboxylic components in humic-like substances (HULIS) and source apportionment of HULIS in ambient fine aerosols (PM2.5) collected in Hong Kong.

The correct name of the 3rd Author is presented in this paper.

Speciation of carboxylic components in humic-like substances (HULIS) and source apportionment of HULIS in ambient fine aerosols (PM2.5) collected in Hong Kong.

Humic-like substances (HULIS) are an important mixture of organic compounds, which account for a great part of water-soluble organic compounds in ambient aerosols. In this study, individual carboxylic and hydroxylic species in HULIS extracts of PM2.5 samples collected in Hong Kong during summer were measured by gas chromatography mass spectrometry with prior chemical derivatization. Significantly higher levels of HULIS were observed on days mainly impacted by regional pollution (regional days, 4.11 ± 1.76 µg m-3) than on days under local emission influences (local days, 0.56 ± 0.30 µg m-3). Positive matrix factorization was applied to identify the major sources and apportion their contributions to HULIS. Simultaneous monitoring and analysis data from four different sampling sites showed that sources of HULIS in Hong Kong were mainly regional with small spatial variations. Secondary aerosol formation (both organic and inorganic) had a predominant contribution (52.7%) to HULIS during the whole sampling period. It accounted for 1.88 ± 0.91 µg m-3 of HULIS on regional days, which was about 5 times higher than its contribution (0.39 ± 0.34 µg m-3) on local days. Of the three identified primary sources, biomass burning had the largest contribution on both regional (34.9%) and local days (24.6%). Marine vessels were also a significant contributor, especially on local days (20.3%). Vehicle exhaust, on the other hand, showed a negligible contribution to HULIS (2.1%) in Hong Kong in this study.

Quantum expander for gravitational-wave observatories.

The quantum uncertainty of laser light limits the sensitivity of gravitational-wave observatories. Over the past 30 years, techniques for squeezing the quantum uncertainty, as well as for enhancing gravitational-wave signals with optical resonators have been invented. Resonators, however, have finite linewidths, and the high signal frequencies that are produced during the highly scientifically interesting ring-down of astrophysical compact-binary mergers still cannot be resolved. Here, we propose a purely optical approach for expanding the detection bandwidth. It uses quantum uncertainty squeezing inside one of the optical resonators, compensating for the finite resonators' linewidths while keeping the low-frequency sensitivity unchanged. This quantum expander is intended to enhance the sensitivity of future gravitational-wave detectors, and we suggest the use of this new tool in other cavity-enhanced metrological experiments.

Satellite testing of a gravitationally induced quantum decoherence model.

Quantum mechanics and the general theory of relativity are two pillars of modern physics. However, a coherent unified framework of the two theories remains an open problem. Attempts to quantize general relativity have led to many rival models of quantum gravity, which, however, generally lack experimental foundations. We report a quantum optical experimental test of event formalism of quantum fields, a theory that attempts to present a coherent description of quantum fields in exotic spacetimes containing closed timelike curves and ordinary spacetime. We experimentally test a prediction of the theory with the quantum satellite Micius that a pair of time-energy-entangled particles probabilistically decorrelate passing through different regions of the gravitational potential of Earth. Our measurement results are consistent with the standard quantum theory and hence do not support the prediction of event formalism.

Optical properties, source apportionment and redox activity of humic-like substances (HULIS) in airborne fine particulates in Hong Kong.

Humic-like substances (HULIS) account for a considerable fraction of water-soluble organic matter (WSOM) in ambient fine particulates (PM2.5) over the world. However, systemic studies regarding the chemical characteristics, sources and redox activity of HULIS are still limited. In this study, the mass concentration, optical properties, and reactive oxygen species (ROS)-generation potential of HULIS were investigated in PM2.5 samples collected in Hong Kong during 2011-2012, and they all showed higher levels on days under regional pollution than on days under long range transport (LRT) pollution and local emissions. Positive matrix factorization (PMF) analysis was conducted regarding the mass concentration and dithiothreitol (DTT) activity of HULIS. Four primary sources (i.e. marine vessels, industrial exhaust, biomass burning, and vehicle emissions), and two secondary sources (i.e. secondary organic aerosol formation and secondary sulfate) were identified. Most sources showed higher contributions to both the mass concentration and DTT activity of HULIS on regional days than on LRT and local days, except that marine vessels had a higher contribution on local days than the other two synoptic conditions. Secondary processes were the major contributor to HULIS (54.9%) throughout the year, followed by biomass burning (27.4%) and industrial exhaust (14.7%). As for the DTT activity of HULIS, biomass burning (62.9%) and secondary processes (25.4%) were found to be the top two contributors. Intrinsic ROS-generation potential of HULIS was also investigated by normalizing the DTT activity by HULIS mass in each source. HULIS from biomass burning were the most DTT-active, followed by marine vessels; while HULIS formed through secondary processes were the least DTT-active. For the optical properties of HULIS, multiple linear regression model was adopted to evaluate the contributions of various sources to the light absorbing ability of HULIS. Biomass burning was found to be the only source significantly associated with the light absorbing property of HULIS.

Towards the Fundamental Quantum Limit of Linear Measurements of Classical Signals.

The quantum Cramér-Rao bound (QCRB) sets a fundamental limit for the measurement of classical signals with detectors operating in the quantum regime. Using linear-response theory and the Heisenberg uncertainty relation, we derive a general condition for achieving such a fundamental limit. When applied to classical displacement measurements with a test mass, this condition leads to an explicit connection between the QCRB and the standard quantum limit that arises from a tradeoff between the measurement imprecision and quantum backaction; the QCRB can be viewed as an outcome of a quantum nondemolition measurement with the backaction evaded. Additionally, we show that the test mass is more a resource for improving measurement sensitivity than a victim of the quantum backaction, which suggests a new approach to enhancing the sensitivity of a broad class of sensors. We illustrate these points with laser interferometric gravitational-wave detectors.

A quantitative assessment of source contributions to fine particulate matter (PM2.5)-bound polycyclic aromatic hydrocarbons (PAHs) and their nitrated and hydroxylated derivatives in Hong Kong.

Atmospheric polycyclic aromatic hydrocarbons (PAHs) and their derivatives are of great concern due to their adverse health effects. However, source identification and apportionment of these compounds, particularly their nitrated and hydroxylated derivatives (i.e., NPAHs and OHPAHs), in fine particulate matter (PM2.5) in Hong Kong are still lacking. In this study, we conducted a 1-year observation at an urban site in Hong Kong. PM2.5-bound PAHs and their derivatives were measured, with median concentrations of 4590, 44.4 and 31.6 pg m-3 for ∑21PAHs, ∑13NPAHs, and ∑12OHPAHs, respectively. Higher levels were observed on regional pollution days than on long regional transport (LRT) or local emission days. Based on positive matrix factorization analysis, four sources were determined: marine vessels, vehicle emissions, biomass burning, and a mixed source of coal combustion and NPAHs secondary formation. Coal combustion and biomass burning were the major sources of PAHs, contributing over 85% of PAHs on regional and LRT days. Biomass burning was the predominant source of OHPAHs throughout the year, while NPAHs mainly originated from secondary formation and fuel combustion. For benzo[a]pyrene (BaP)-based PM2.5 toxicity, the mixed source of coal combustion and NPAHs secondary formation was the major contributor, followed by biomass burning and vehicle emissions.

Association of polycyclic aromatic hydrocarbons in housewives' hair with hypertension.

The relationship between polycyclic aromatic hydrocarbons (PAHs) and hypertension remains a subject of debate. The aims of this study were to determine an association of concentrations of PAHs in housewives' hair with hypertension risk and the modification effect of single nucleotide polymorphisms (SNPs) related to Phase I metabolism of PAHs. We recruited 405 women for a cross-sectional study in Shanxi Province, China, including 170 with hypertension (the case group) and 235 without hypertension (the control group). We analyzed 26 individual PAHs in hair samples and the SNPs of the genes including cytochrome P450, family 1, subfamily A, polypeptide 1 (CYP1A1), CYP1A2, CYP1B1 and CYP2E1. Our results showed that seven PAHs in hair samples were measured with detection rate >70%. Only acenaphthylene was found to be associated with an increased risk of hypertension with adjustment for the potential confounders following Bonferroni correction, whereas others not. No SNPs of the concerned genes were found to be associated with the risk of hypertension. A multiple interaction effect of PAHs in housewives' hair and SNPs on hypertension risk was not observed. It was concluded that PAHs tended to contribute to the formation of hypertension.

Enhancing the Bandwidth of Gravitational-Wave Detectors with Unstable Optomechanical Filters.

Advanced interferometric gravitational-wave detectors use optical cavities to resonantly enhance their shot-noise-limited sensitivity. Because of positive dispersion of these cavities-signals at different frequencies pick up different phases, there is a tradeoff between the detector bandwidth and peak sensitivity, which is a universal feature for quantum measurement devices having resonant cavities. We consider embedding an active unstable filter inside the interferometer to compensate the phase, and using feedback control to stabilize the entire system. We show that this scheme in principle can enhance the bandwidth without sacrificing the peak sensitivity. However, the unstable filter under our current consideration is a cavity-assisted optomechanical device operating in the instability regime, and the thermal fluctuation of the mechanical oscillator puts a very stringent requirement on the environmental temperature and the mechanical quality factor.

Linear negative dispersion with a gain doublet via optomechanical interactions.

Optical cavities containing a negative dispersion medium have been proposed as a means of improving the sensitivity of laser interferometric gravitational wave detectors through the creation of white-light signal recycling cavities. Here we demonstrate that negative dispersion can be realized using an optomechanical cavity pumped by a blue detuned doublet. We used an 85-mm cavity with an intracavity silicon nitride membrane. Tunable negative dispersion is demonstrated, with a phase derivative dφ/df from -0.14 Deg·Hz(-1) to -4.2×10(-3) Deg·Hz(-1).

Concentrations and spatial distribution of polycyclic aromatic hydrocarbons (PAHs) and nitrated PAHs (NPAHs) in the atmosphere of North China, and the transformation from PAHs to NPAHs.

The occurrence of polycyclic aromatic hydrocarbons (PAHs) and nitrated derivatives (NPAHs), as well as their transformation may have significant health impacts on humans. To investigate the level, spatial distribution and the transformation process of PAHs and NPAHs in North China, we performed a griddedfield passive air sampling campaign in summer of 2011. The median concentration of 25 PAH congeners and 13 NPAHs was 294 ng m(-3) (or 26.7 mg sample(-1)) and 203 ng sample(-1), respectively. Relative higher level of PAHs in Shanxi Province and NPAHs in megacities was observed. In North China, coal/biomass combustion and photochemical formation was the predominant source of PAHs and NPAHs, respectively.To investigate the relationship between these pollutants, a model incorporating NPAHs, PAHs and NO(2) was established, and the result indicated that NO(2) will promote the transformation processes from PAHs to NPAHs, which may increase the total toxicity of PAH-NPAH mixtures.

Narrowing the filter-cavity bandwidth in gravitational-wave detectors via optomechanical interaction.

We propose using optomechanical interaction to narrow the bandwidth of filter cavities for achieving frequency-dependent squeezing in advanced gravitational-wave detectors, inspired by the idea of optomechanically induced transparency. This can allow us to achieve a cavity bandwidth on the order of 100 Hz using small-scale cavities. Additionally, in contrast to a passive Fabry-Pérot cavity, the resulting cavity bandwidth can be dynamically tuned, which is useful for adaptively optimizing the detector sensitivity when switching amongst different operational modes. The experimental challenge for its implementation is a stringent requirement for very low thermal noise of the mechanical oscillator, which would need a superb mechanical quality factor and a very low temperature. We consider one possible setup to relieve this requirement by using optical dilution to enhance the mechanical quality factor.