ABSTRACT
We use a rotating magnetic field to assemble an oblate cluster of paramagnetic colloidal particles. If the field is rotating about a horizontal axis, the cluster acts as a colloidal wheel rolling across the supporting glass surface. The motion is reversible upon switching the direction of rotation. Surprisingly, the reversibility is lost if the axis of field rotation is tilted with respect to the surface. The wheel then rolls in a direction that is not perpendicular to the field rotation axis. We explain the skewed rotation with an interplay between a magnetic driving torque, magnetic anisotropy and an anisotropy in the hydrodynamic mobility tensor in the vicinity of a surface. The opposing forward and backward drive induce opposite chirality in the degrees of freedom of the mechanically achiral colloidal wheel.
ABSTRACT
Isotropic magnetic field modulations cause the formation and coarsening of transient two dimensional paramagnetic colloidal networks. We show that the virgin transient network consists of sub- and supercritical meshes. In the initial coarsening process subcritical meshes shrink while supercritical meshes grow. While the coarsening is a truly non-equilibrium process, the critical nucleation size is independent of transport coefficients and can be theoretically described by the competition of first order long range collective dipolar interactions and short range second order dipolar pair correlations.