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1.
Appl Radiat Isot ; 201: 110987, 2023 Nov.
Article in English | MEDLINE | ID: mdl-37660500

ABSTRACT

A method for absolute measurements of the 225Ac activity in equilibrium with its progeny was developed. Measurements were performed using the triple-to-double coincidence ratio (TDCR) method in two different TDCR counters. The activity concentration of an 225Ac solution was determined and the solution was sent to the SIR system for a comparison. The half-life of 225Ac was determined by one of the TDCR counters and found to be 9.9150(63) days.

2.
Appl Radiat Isot ; 197: 110829, 2023 Jul.
Article in English | MEDLINE | ID: mdl-37119706

ABSTRACT

The activity of the 177Lu solution has been measured by means of the CIEMAT/NIST efficiency tracing method. This result has been compared to the previous obtained results received from 4πß(LS)-γ coincidence and anticoincidence counting. The activities determined with various methods have been found to be consistent. The decay curve of the 177Lu solution has been followed in the TDCR counter to determine the half-life of this isotope. The half-life has been separately determined for double and triple coincidence events. The arithmetic mean value of these two results has been found to be T1/2 = 6.6489(52) d.

3.
Appl Radiat Isot ; 134: 385-390, 2018 Apr.
Article in English | MEDLINE | ID: mdl-29248210

ABSTRACT

An international key comparison, identifier CCRI(II)-K2.Ge-68, has been performed. The National Institute of Standards and Technology (NIST) served as the pilot laboratory, distributing aliquots of a 68Ge/68Ga solution. Results for the activity concentration, CA, of 68Ge at a reference date of 12h00 UTC 14 November 2014 were submitted by 17 laboratories, encompassing many variants of coincidence methods and liquid-scintillation counting methods. The first use of 4π(Cherenkov)ß-γ coincidence and anticoincidence methods in an international comparison is reported. One participant reported results by secondary methods only. Two results, both utilizing pure liquid-scintillation methods, were identified as outliers. Evaluation using the Power-Moderated Mean method results in a proposed Comparison Reference Value (CRV) of 621.7(11)kBqg-1, based on 14 results. The degrees of equivalence and their associated uncertainties are evaluated for each participant. Several participants submitted 3.6mL ampoules to the BIPM to link the comparison to the International Reference System (SIR) which may lead to the evaluation of a Key Comparison Reference Value and associated degrees of equivalence.

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