ABSTRACT
Thermal expansion, electrical resistivity, magnetization, and specific heat measurements were performed on URu2-xFexSi2 single crystals for various values of Fe concentration x in both the hidden-order (HO) and large-moment antiferromagnetic (LMAFM) regions of the phase diagram. Our results show that the paramagnetic (PM) to HO and LMAFM phase transitions are manifested differently in the thermal expansion coefficient. The uniaxial pressure derivatives of the HO/LMAFM transition temperature T0 change dramatically when crossing from the HO to the LMAFM phase. The energy gap also changes consistently when crossing the phase boundary. In addition, for Fe concentrations at xc ≈ 0.1, we observe two features in the thermal expansion upon cooling, one that appears to be associated with the transition from the PM to the HO phase and another one at lower temperature that may be due to the transition from the HO to the LMAFM phase.
ABSTRACT
Heavy fermion compounds represent one of the most strongly correlated forms of electronic matter and give rise to low temperature states that range from small moment ordering to exotic superconductivity, both of which are often in close proximity to quantum critical points. These strong electronic correlations are associated with the transfer of entropy from the local moment degrees of freedom to the conduction electrons, and, as such, are intimately related to the low temperature degeneracy of the (originally) moment bearing ion. Here we report the discovery of six closely related Yb-based heavy fermion compounds, YbT(2)Zn(20), that are members of the larger family of dilute rare earth bearing compounds: RT(2)Zn(20) (T = Fe, Co, Ru, Rh, Os, Ir). This discovery doubles the total number of Yb-based heavy fermion materials. Given these compounds' dilute nature, systematic changes in T only weakly perturb the Yb site and allow for insight into the effects of degeneracy on the thermodynamic and transport properties of these model correlated electron systems.
