Modeling electric-field-sensitive scanning probe measurements for a tip of arbitrary shape.

We present a numerical method to model electric-field-sensitive scanning probe microscopy measurements which allows for a tip of arbitrary shape and invokes image charges to exactly account for a sample dielectric overlayer. The method is applied to calculate the spatial resolution of a subsurface charge accumulation imaging system, achieving reasonable agreement with experiment.

Transition between quantum states in a parallel-coupled double quantum dot.

Strong electron and spin correlations in a double quantum dot (DQD) can give rise to different quantum states. We observe a continuous transition from a Kondo state exhibiting a single-peak Kondo resonance to another exhibiting a double peak by increasing the interdot coupling (t) in a parallel-coupled DQD. The transition into the double-peak state provides evidence for spin entanglement between the excess electrons on each dot. Toward the transition, the peak splitting merges and becomes substantially smaller than t because of strong Coulomb effects. Our device tunability bodes well for future quantum computation applications.

Time-dependent speckle in holographic optical coherence imaging and the health of tumor tissue.

Holographic optical coherence imaging acquires en face images from successive depths inside scattering tissue. In a study of multicellular tumor spheroids the holographic features recorded from a fixed depth are observed to be time dependent, and they may be classified as variable or persistent. The ratio of variable to persistent features, as well as speckle correlation times, provides quantitative measures of the health of the tissue. Studies of rat osteogenic sarcoma tumor spheroids that have been subjected to metabolic and cross-polymerizing poisons provide quantitative differentiation among healthy, necrotic, and poisoned tissue. Organelle motility in healthy tissue appears as super-Brownian laser speckle, whereas chemically fixed tissue exhibits static speckle.

Ultrasound detection through turbid media.

Optical coherence-domain reflectometry and laser-based ultrasound detection have been combined with the use of adaptive optics to detect ultrasound through turbid media. The dynamic hologram in a photorefractive quantum-well device performs as a coherence gate that eliminates multiply scattered background. Quadrature homodyne detection conditions are selected by the choice of center wavelength of the pulse spectrum, requiring no active stabilization or feedback. A depth resolution of 30 microm was achieved, with a pulse duration of nominally 120 fs for ultrasound detection through turbid media up to optical thicknesses of 11 mean free scattering lengths.

High-speed adaptive interferometer for optical coherence-domain reflectometry through turbid media.

Two-wave mixing in a dynamic holographic film acts as the adaptive beam combiner in a short-coherence interferometer that performs optical coherence-domain reflectometry (OCDR) through turbid media. This approach combines the high spatial resolution and sensitivity of coherence-domain reflectometry with photorefractive quantum-well-based adaptive homodyne detection. A depth resolution of 28 microm and penetration through 16 mean free paths in a turbid medium have been obtained in this adaptive OCDR application.

The Kondo effect in an artificial quantum dot molecule.

Double quantum dots provide an ideal model system for studying interactions between localized impurity spins. We report on the transport properties of a series-coupled double quantum dot as electrons are added one by one onto the dots. When the many-body molecular states are formed, we observe a splitting of the Kondo resonance peak in the differential conductance. This splitting reflects the energy difference between the bonding and antibonding states formed by the coherent superposition of the Kondo states of each dot. The occurrence of the Kondo resonance and its magnetic field dependence agree with a simple interpretation of the spin status of a double quantum dot.

Elimination of beam walk-off in low-coherence off-axis photorefractive holography.

Whole-field photorefractive holography can be combined with low-coherence interferometry for three-dimensional imaging and other applications, including imaging through turbid media, but the off-axis holographic recording geometry results in a limited field of view when light of low temporal coherence is used. We show that tilting the energy fronts with respect to the wave fronts by use of prisms can eliminate this problem and point out that this approach will be useful for many linear and nonlinear wave-mixing experiments.

Generation and characterization of terahertz pulse trains from biased, large-aperture photoconductors.

The saturation properties of terahertz emission from biased, large-aperture photoconductors excited by trains of amplified femtosecond optical pulses are presented. A direct comparison is made of the multiple-pulse saturation properties of terahertz emission from semi-insulating GaAs and low-temperature-grown GaAs emitters with different carrier lifetimes. When the carrier lifetime is less than or comparable with the interpulse spacing, a significant enhancement of the narrow-band terahertz output is observed. The enhancement is not observed for emitters with long carrier lifetimes, consistent with the results of a previously derived saturation theory [Opt. Lett. 18, 1340 (1993)].

Oscillatory mode coupling and electrically strobed gratings in photorefractive quantum-well diodes.

Oscillatory mode coupling between two coherent laser beams is produced when an interference pattern moves against a quasi-static electrically strobed grating in a photorefractive AlGaAs/GaAs multiple-quantum-well diode operated in the quantum-confined Stark geometry. The oscillation frequency is equal to the frequency difference between the two laser beams and provides a method to measure high-frequency Doppler shifts or large surface displacements for laser-based ultrasound. Combined photorefractive gains (normally forbidden by symmetry in the Stark geometry) and absorptive gains approach 1200cm(-1)during two-wave mixing using moving gratings.

Direct-to-video holographic readout in quantum wells for three-dimensional imaging through turbid media.

Customized photorefractive quantum-well devices have been developed for real-time video acquisition of coherence-gated, three-dimensional images in turbid media. Large-field-of-view holographic imaging with direct video capture is now possible. We have evaluated the role of intensity-limited device performance in Fourier-plane and image-plane holography in such devices and, using near-infrared light, have imaged through turbid phantoms of 13 mean free paths' scattering depth with 50-microm transverse and 60-microm depth resolution.

Real-time edge enhancement of femtosecond time-domain images by use of photorefractive quantum wells.

Dynamic holograms written in a photorefractive multiple quantum well placed inside a Fourier femtosecond pulse shaper convert a space-domain image into the time domain. We demonstrate that edge-enhancement processing of the time-domain image can be performed by controlling hologram-writing intensities.

Femtosecond pulse shaping by dynamic holograms in photorefractive multiple quantum wells.

Femtosecond pulses can be shaped in the time domain by diffraction from dynamic holograms in a photorefractive multiple quantum well placed inside a Fourier pulse shaper. We present several examples of shaped pulses obtained by controlling the amplitude or the phase of the hologram writing beams, which modifies the complex spectrum of the femtosecond output.

Reflection-geometry photorefractive quantum wells.

We present what is to our knowledge the first demonstration of photorefractive AlGaAs/GaAs quantum wells operated in the reflection geometry, using the quantum-confined Stark effect. This photorefractive geometry relies on volume reflection gratings of a small number of periods written in a nonstoichiometric multiple-quantum-well layer with counterpropagating beams. Combined absorptive and photorefractive twowave mixing gains as large as 1500 cm(-1) are observed under reverse bias of the diode.

Spatial-harmonic gratings at high modulation depths in photorefractive quantum wells.

High-order spatial harmonics of photorefractive gratings are detected directly in multi wave mixing experiments in photorefractive AlGaAs/GaAs quantum wells operating in the Franz-Keldysh geometry. We have observed diffraction signals from the first-, second-, and third-harmonic refractive-index gratings. The quadratic electro-optic effect in the quantum wells second-spatial-harmonic grating.