Signatures of a surface spin-orbital chiral metal.

The relation between crystal symmetries, electron correlations and electronic structure steers the formation of a large array of unconventional phases of matter, including magneto-electric loop currents and chiral magnetism1-6. The detection of such hidden orders is an important goal in condensed-matter physics. However, until now, non-standard forms of magnetism with chiral electronic ordering have been difficult to detect experimentally7. Here we develop a theory for symmetry-broken chiral ground states and propose a methodology based on circularly polarized, spin-selective, angular-resolved photoelectron spectroscopy to study them. We use the archetypal quantum material Sr2RuO4 and reveal spectroscopic signatures that, despite being subtle, can be reconciled with the formation of spin-orbital chiral currents at the surface of the material8-10. As we shed light on these chiral regimes, our findings pave the way for a deeper understanding of ordering phenomena and unconventional magnetism.

Designing spin and orbital sources of Berry curvature at oxide interfaces.

Quantum materials can display physical phenomena rooted in the geometry of electronic wavefunctions. The corresponding geometric tensor is characterized by an emergent field known as the Berry curvature (BC). Large BCs typically arise when electronic states with different spin, orbital or sublattice quantum numbers hybridize at finite crystal momentum. In all the materials known to date, the BC is triggered by the hybridization of a single type of quantum number. Here we report the discovery of the first material system having both spin- and orbital-sourced BC: LaAlO3/SrTiO3 interfaces grown along the [111] direction. We independently detect these two sources and probe the BC associated to the spin quantum number through the measurements of an anomalous planar Hall effect. The observation of a nonlinear Hall effect with time-reversal symmetry signals large orbital-mediated BC dipoles. The coexistence of different forms of BC enables the combination of spintronic and optoelectronic functionalities in a single material.

Colossal Orbital Edelstein Effect in Noncentrosymmetric Superconductors.

In superconductors that lack inversion symmetry, the flow of supercurrent can induce a nonvanishing magnetization, a phenomenon which is at the heart of nondissipative magnetoelectric effects, also known as Edelstein effects. For electrons carrying spin and orbital moments, a question of fundamental relevance deals with the orbital nature of magnetoelectric effects in conventional spin-singlet superconductors with Rashba coupling. Remarkably, we find that the supercurrent-induced orbital magnetization is more than 1 order of magnitude greater than that due to the spin, giving rise to a colossal magnetoelectric effect. The induced orbital magnetization is shown to be sign tunable, with the sign change occurring for the Fermi level lying in proximity of avoiding crossing points in the Brillouin zone. In the presence of superconducting phase inhomogeneities, a modulation of the Edelstein signal on the scale of the superconducting coherence length appears, leading to domains with opposite orbital moment orientations. These hallmarks are robust to real-space self-consistent treatment of the superconducting order parameter. The orbital-dominated magnetoelectric phenomena, hence, have clear-cut marks for detection both in the bulk and at the edge of the system and are expected to be a general feature of multiorbital superconductors with inversion symmetry breaking.

Gate Control of the Current-Flux Relation of a Josephson Quantum Interferometer Based on Proximitized Metallic Nanojuntions.

We demonstrate an Al superconducting quantum interference device in which the Josephson junctions are implemented through gate-controlled proximity Cu mesoscopic weak links. This specific kind of metallic weak links behaves analogously to genuine superconducting metals in terms of the response to electrostatic gating and provides a good performance in terms of current-modulation visibility. We show that through the application of a static gate voltage we can modify the interferometer current-flux relation in a fashion that seems compatible with the introduction of π-channels within the gated weak link. Our results suggest that the microscopic mechanism at the origin of the suppression of the switching current in the interferometer is apparently phase coherent, resulting in an overall damping of the superconducting phase rigidity. We finally tackle the performance of the interferometer in terms of responsivity to magnetic flux variations in the dissipative regime and discuss the practical relevance of gated proximity-based all-metallic SQUIDs for magnetometry at the nanoscale.

Synthetic Weyl Points and Chiral Anomaly in Majorana Devices with Nonstandard Andreev-Bound-State Spectra.

We demonstrate how to design various nonstandard types of Andreev-bound-state (ABS) dispersions, via a composite construction relying on Majorana bound states (MBSs). Here, the MBSs appear at the interface of a Josephson junction consisting of two topological superconductors (TSCs). Each TSC harbors multiple MBSs per edge by virtue of a chiral or unitary symmetry. We find that, while the ABS dispersions are 2π periodic, they still contain multiple crossings which are protected by the conservation of fermion parity. A single junction with four interface MBSs and all MBS couplings fully controllable, or networks of such coupled junctions with partial coupling tunability, open the door for topological band structures with Weyl points or nodes in synthetic dimensions, which in turn allow for fermion-parity (FP) pumping with a cycle set by the ABS-dispersion details. In fact, in the case of nodes, the FP pumping is a manifestation of chiral anomaly in 2D synthetic spacetime. The possible experimental demonstration of ABS engineering in these devices further promises to unveil new paths for the detection of MBSs and higher-dimensional chiral anomaly.