Squeezed-Light Enhancement and Backaction Evasion in a High Sensitivity Optically Pumped Magnetometer.

We study the effect of optical polarization squeezing on the performance of a sensitive, quantum-noise-limited optically pumped magnetometer. We use Bell-Bloom (BB) optical pumping to excite a ^{87}Rb vapor containing 8.2×10^{12} atoms/cm^{3} and Faraday rotation to detect spin precession. The sub-pT/sqrt[Hz] sensitivity is limited by spin projection noise (photon shot noise) at low (high) frequencies. Probe polarization squeezing both improves high-frequency sensitivity and increases measurement bandwidth, with no loss of sensitivity at any frequency, a direct demonstration of the evasion of measurement backaction noise. We provide a model for the quantum noise dynamics of the BB magnetometer, including spin projection noise, probe polarization noise, and measurement backaction effects. The theory shows how polarization squeezing reduces optical noise, while measurement backaction due to the accompanying ellipticity antisqueezing is shunted into the unmeasured spin component. The method is compatible with high-density and multipass techniques that reach extreme sensitivity.

Erratum: Simple Proof of Equivalence between Adiabatic Quantum Computation and the Circuit Model [Phys. Rev. Lett. 99, 070502 (2007)].

This corrects the article DOI: 10.1103/PhysRevLett.99.070502.

Entanglement-Enhanced Phase Estimation without Prior Phase Information.

We study the generation of planar quantum squeezed (PQS) states by quantum nondemolition (QND) measurement of an ensemble of ^{87}Rb atoms with a Poisson distributed atom number. Precise calibration of the QND measurement allows us to infer the conditional covariance matrix describing the F_{y} and F_{z} components of the PQS states, revealing the dual squeezing characteristic of PQS states. PQS states have been proposed for single-shot phase estimation without prior knowledge of the likely values of the phase. We show that for an arbitrary phase, the generated PQS states can give a metrological advantage of at least 3.1 dB relative to classical states. The PQS state also beats, for most phase angles, single-component-squeezed states generated by QND measurement with the same resources and atom number statistics. Using spin squeezing inequalities, we show that spin-spin entanglement is responsible for the metrological advantage.

Entanglement-Enhanced Radio-Frequency Field Detection and Waveform Sensing.

We demonstrate a new technique for detecting the amplitude of arbitrarily chosen components of radio-frequency waveforms based on stroboscopic backaction evading measurements. We combine quantum nondemolition measurements and stroboscopic probing to detect waveform components with magnetic sensitivity beyond the standard quantum limit. Using an ensemble of 1.5×10^{6} cold rubidium atoms, we demonstrate entanglement-enhanced sensing of sinusoidal and linearly chirped waveforms, with 1.0(2) and 0.8(3) dB metrologically relevant noise reduction, respectively. We achieve volume-adjusted sensitivity of δBsqrt[V]≈3.96 fTsqrt[cm^{3}/Hz], comparable to the best rf magnetometers.

Quantum Nondemolition Measurement Enables Macroscopic Leggett-Garg Tests.

We show how a test of macroscopic realism based on Leggett-Garg inequalities (LGIs) can be performed in a macroscopic system. Using a continuous-variable approach, we consider quantum nondemolition (QND) measurements applied to atomic ensembles undergoing magnetically driven coherent oscillation. We identify measurement schemes requiring only Gaussian states as inputs and giving a significant LGI violation with realistic experimental parameters and imperfections. The predicted violation is shown to be due to true quantum effects rather than to a classical invasivity of the measurement. Using QND measurements to tighten the "clumsiness loophole" forces the stubborn macrorealist to recreate quantum backaction in his or her account of measurement.

Loophole-free Bell inequality violation using electron spins separated by 1.3 kilometres.

More than 50 years ago, John Bell proved that no theory of nature that obeys locality and realism can reproduce all the predictions of quantum theory: in any local-realist theory, the correlations between outcomes of measurements on distant particles satisfy an inequality that can be violated if the particles are entangled. Numerous Bell inequality tests have been reported; however, all experiments reported so far required additional assumptions to obtain a contradiction with local realism, resulting in 'loopholes'. Here we report a Bell experiment that is free of any such additional assumption and thus directly tests the principles underlying Bell's inequality. We use an event-ready scheme that enables the generation of robust entanglement between distant electron spins (estimated state fidelity of 0.92 ± 0.03). Efficient spin read-out avoids the fair-sampling assumption (detection loophole), while the use of fast random-basis selection and spin read-out combined with a spatial separation of 1.3 kilometres ensure the required locality conditions. We performed 245 trials that tested the CHSH-Bell inequality S ≤ 2 and found S = 2.42 ± 0.20 (where S quantifies the correlation between measurement outcomes). A null-hypothesis test yields a probability of at most P = 0.039 that a local-realist model for space-like separated sites could produce data with a violation at least as large as we observe, even when allowing for memory in the devices. Our data hence imply statistically significant rejection of the local-realist null hypothesis. This conclusion may be further consolidated in future experiments; for instance, reaching a value of P = 0.001 would require approximately 700 trials for an observed S = 2.4. With improvements, our experiment could be used for testing less-conventional theories, and for implementing device-independent quantum-secure communication and randomness certification.

Generation of macroscopic singlet states in a cold atomic ensemble.

We report the generation of a macroscopic singlet state in a cold atomic sample via quantum nondemolition measurement-induced spin squeezing. We observe 3 dB of spin squeezing and detect entanglement with 5σ statistical significance using a generalized spin-squeezing inequality. The degree of squeezing implies at least 50% of the atoms have formed singlets.

Ultra-fast quantum randomness generation by accelerated phase diffusion in a pulsed laser diode.

We demonstrate a high bit-rate quantum random number generator by interferometric detection of phase diffusion in a gain-switched DFB laser diode. Gain switching at few-GHz frequencies produces a train of bright pulses with nearly equal amplitudes and random phases. An unbalanced Mach-Zehnder interferometer is used to interfere subsequent pulses and thereby generate strong random-amplitude pulses, which are detected and digitized to produce a high-rate random bit string. Using established models of semiconductor laser field dynamics, we predict a regime of high visibility interference and nearly complete vacuum-fluctuation-induced phase diffusion between pulses. These are confirmed by measurement of pulse power statistics at the output of the interferometer. Using a 5.825 GHz excitation rate and 14-bit digitization, we observe 43 Gbps quantum randomness generation.

Simulation of non-Abelian gauge theories with optical lattices.

Many phenomena occurring in strongly correlated quantum systems still await conclusive explanations. The absence of isolated free quarks in nature is an example. It is attributed to quark confinement, whose origin is not yet understood. The phase diagram for nuclear matter at general temperatures and densities, studied in heavy-ion collisions, is not settled. Finally, we have no definitive theory of high-temperature superconductivity. Though we have theories that could underlie such physics, we lack the tools to determine the experimental consequences of these theories. Quantum simulators may provide such tools. Here we show how to engineer quantum simulators of non-Abelian lattice gauge theories. The systems we consider have several applications: they can be used to mimic quark confinement or to study dimer and valence-bond states (which may be relevant for high-temperature superconductors).

Feedback cooling of an atomic spin ensemble.

We apply entropy removal by measurement and feedback to a cold atomic spin ensemble. Using quantum nondemolition probing by Faraday rotation measurement, and feedback by weak optical pumping, we drive the initially random collective spin variable F toward the origin F=0. We use input-output relations and ensemble quantum noise models to describe this quantum control process and identify an optimal two-round control procedure. We observe 12 dB of spin noise reduction, or a factor-of-63 reduction in phase-space volume. The method offers a nonthermal route to generation of exotic entangled states in ultracold gases, including macroscopic singlet states and strongly correlated states of quantum lattice gases.

Fast beam steering with full polarization control using a galvanometric optical scanner and polarization controller.

Optical beam steering is a key element in many industrial and scientific applications like in material processing, information technologies, medical imaging and laser display. Even though galvanometer-based scanners offer flexibility, speed and accuracy at a relatively low cost, they still lack the necessary control over the polarization required for certain applications. We report on the development of a polarization steerable system assembled with a fiber polarization controller and a galvanometric scanner, both controlled by a digital signal processor board. The system implements control of the polarization decoupled from the pointing direction through a feed-forward control scheme. This enables to direct optical beams to a desired direction without affecting its initial polarization state. When considering the full working field of view, we are able to compensate polarization angle errors larger than 0.2 rad, in a temporal window of less than ∼ 20 ms. Given the unification of components to fully control any polarization state while steering an optical beam, the proposed system is potentially integrable and robust.

Efficient quantification of non-gaussian spin distributions.

We study theoretically and experimentally the quantification of non-gaussian distributions via nondestructive measurements. Using the theory of cumulants, their unbiased estimators, and the uncertainties of these estimators, we describe a quantification which is simultaneously efficient, unbiased by measurement noise, and suitable for hypothesis tests, e.g., to detect nonclassical states. The theory is applied to cold 87Rb spin ensembles prepared in non-gaussian states by optical pumping and measured by nondestructive Faraday rotation probing. We find an optimal use of measurement resources under realistic conditions, e.g., in atomic ensemble quantum memories.

Magnetic sensitivity beyond the projection noise limit by spin squeezing.

We report the generation of spin squeezing and entanglement in a magnetically sensitive atomic ensemble, and entanglement-enhanced field measurements with this system. A maximal m(f) = ± 1 Raman coherence is prepared in an ensemble of 8.5 × 10(5) laser-cooled (87)Rb atoms in the f = 1 hyperfine ground state, and the collective spin is squeezed by synthesized optical quantum nondemolition measurement. This prepares a state with large spin alignment and noise below the projection-noise level in a mixed alignment-orientation variable. 3.2 dB of noise reduction is observed and 2.0 dB of squeezing by the Wineland criterion, implying both entanglement and metrological advantage. Enhanced sensitivity is demonstrated in field measurements using alignment-to-orientation conversion.

True random numbers from amplified quantum vacuum.

Random numbers are essential for applications ranging from secure communications to numerical simulation and quantitative finance. Algorithms can rapidly produce pseudo-random outcomes, series of numbers that mimic most properties of true random numbers while quantum random number generators (QRNGs) exploit intrinsic quantum randomness to produce true random numbers. Single-photon QRNGs are conceptually simple but produce few random bits per detection. In contrast, vacuum fluctuations are a vast resource for QRNGs: they are broad-band and thus can encode many random bits per second. Direct recording of vacuum fluctuations is possible, but requires shot-noise-limited detectors, at the cost of bandwidth. We demonstrate efficient conversion of vacuum fluctuations to true random bits using optical amplification of vacuum and interferometry. Using commercially-available optical components we demonstrate a QRNG at a bit rate of 1.11 Gbps. The proposed scheme has the potential to be extended to 10 Gbps and even up to 100 Gbps by taking advantage of high speed modulation sources and detectors for optical fiber telecommunication devices.

Fast optical source for quantum key distribution based on semiconductor optical amplifiers.

A novel integrated optical source capable of emitting faint pulses with different polarization states and with different intensity levels at 100 MHz has been developed. The source relies on a single laser diode followed by four semiconductor optical amplifiers and thin film polarizers, connected through a fiber network. The use of a single laser ensures high level of indistinguishability in time and spectrum of the pulses for the four different polarizations and three different levels of intensity. The applicability of the source is demonstrated in the lab through a free space quantum key distribution experiment which makes use of the decoy state BB84 protocol. We achieved a lower bound secure key rate of the order of 3.64 Mbps and a quantum bit error ratio as low as 1.14×10⁻² while the lower bound secure key rate became 187 bps for an equivalent attenuation of 35 dB. To our knowledge, this is the fastest polarization encoded QKD system which has been reported so far. The performance, reduced size, low power consumption and the fact that the components used can be space qualified make the source particularly suitable for secure satellite communication.

Interaction-based quantum metrology showing scaling beyond the Heisenberg limit.

Quantum metrology aims to use entanglement and other quantum resources to improve precision measurement. An interferometer using N independent particles to measure a parameter χ can achieve at best the standard quantum limit of sensitivity, δχ ∝ N(-1/2). However, using N entangled particles and exotic states, such an interferometer can in principle achieve the Heisenberg limit, δχ ∝ N(-1). Recent theoretical work has argued that interactions among particles may be a valuable resource for quantum metrology, allowing scaling beyond the Heisenberg limit. Specifically, a k-particle interaction will produce sensitivity δχ ∝ N(-k) with appropriate entangled states and δχ ∝ N(-(k-1/2)) even without entanglement. Here we demonstrate 'super-Heisenberg' scaling of δχ ∝ N(-3/2) in a nonlinear, non-destructive measurement of the magnetization of an atomic ensemble. We use fast optical nonlinearities to generate a pairwise photon-photon interaction (corresponding to k = 2) while preserving quantum-noise-limited performance. We observe super-Heisenberg scaling over two orders of magnitude in N, limited at large numbers by higher-order nonlinear effects, in good agreement with theory. For a measurement of limited duration, super-Heisenberg scaling allows the nonlinear measurement to overtake in sensitivity a comparable linear measurement with the same number of photons. In other situations, however, higher-order nonlinearities prevent this crossover from occurring, reflecting the subtle relationship between scaling and sensitivity in nonlinear systems. Our work shows that interparticle interactions can improve sensitivity in a quantum-limited measurement, and experimentally demonstrates a new resource for quantum metrology.

Quantum nondemolition measurement of large-spin ensembles by dynamical decoupling.

Quantum nondemolition (QND) measurement of collective variables by off-resonant optical probing has the ability to create entanglement and squeezing in atomic ensembles. Until now, this technique has been applied to real or effective spin one-half systems. We show theoretically that the buildup of Raman coherence prevents the naive application of this technique to larger spin atoms, but that dynamical decoupling can be used to recover the ideal QND behavior. We experimentally demonstrate dynamical decoupling by using a two-polarization probing technique. The decoupled QND measurement achieves a sensitivity 5.7(6) dB better than the spin projection noise.

Sub-projection-noise sensitivity in broadband atomic magnetometry.

We demonstrate sub-projection-noise sensitivity of a broadband atomic magnetometer using quantum nondemolition spin measurements. A cold, dipole-trapped sample of rubidium atoms provides a long-lived spin system in a nonmagnetic environment, and is probed nondestructively by paramagnetic Faraday rotation. The calibration procedure employs as known reference state, the maximum-entropy or "thermal" spin state, and quantitative imaging-based atom counting to identify electronic, quantum, and technical noise in both the probe and spin system. The measurement achieves a sensitivity 1.6 dB (2.8 dB) better than projection-noise (thermal state quantum noise) and will enable squeezing-enhanced broadband magnetometry.

Acceleration of purine degradation by periodontal diseases.

Periodontal diseases, such as gingivitis and periodontitis, are characterized by bacterial plaque accumulation around the gingival crevice and the subsequent inflammation and destruction of host tissues. To test the hypothesis that cellular metabolism is altered as a result of host-bacteria interaction, we performed an unbiased metabolomic profiling of gingival crevicular fluid (GCF) collected from healthy, gingivitis, and periodontitis sites in humans, by liquid and gas chromatography mass spectrometry. The purine degradation pathway, a major biochemical source for reactive oxygen species (ROS) production, was significantly accelerated at the disease sites. This suggests that periodontal-disease-induced oxidative stress and inflammation are mediated through this pathway. The complex host-bacterial interaction was further highlighted by depletion of anti-oxidants, degradation of host cellular components, and accumulation of bacterial products in GCF. These findings provide new mechanistic insights and a panel of comprehensive biomarkers for periodontal disease progression.

Bright filter-free source of indistinguishable photon pairs.

We demonstrate a high-brightness source of pairs of indistinguishable photons based on a type-II phase-matched doubly-resonant optical parametric oscillator operated far below threshold. The cavityenhanced down-conversion output of a PPKTP crystal is coupled into two single-mode fibers with a mode coupling efficiency of 58%. The high degree of indistinguishability between the photons of a pair is demonstrated by a Hong-Ou-Mandel interference visibility of higher than 90% without any filtering at an instantaneous coincidence rate of 450,000 pairs/s per mW of pump power per nm of down-conversion bandwidth. For the degenerate spectral mode with a linewidth of 7 MHz at 795 nm a rate of 70 pairs/(s mW MHz) is estimated, increasing the spectral brightness for indistinguishable photons by two orders of magnitude compared to similar previous sources.