On-Axis Optical Trapping with Vortex Beams: The Role of the Multipolar Decomposition.

Optical trapping is a well-established, decades old technology with applications in several fields of research. The most common scenario deals with particles that tend to be centered on the brightest part of the optical trap. Consequently, the optical forces keep the particle away from the dark zones of the beam. However, this is not the case when a focused doughnut-shaped beam generates on-axis trapping. In this system, the particle is centered on the intensity minima of the laser beam and the bright annular part lies on the periphery of the particle. Researchers have shown great interest in this phenomenon due to its advantage of reducing light interaction with trapped particles and the intriguing increase in the trapping strength. This work presents experimental and theoretical results that extend the analysis of on-axis trapping with light vortex beams. Specifically, in our experiments, we trap micron-sized spherical silica (SiO2) particles in water and we measure, through the power spectrum density method, the trap stiffness constant κ generated by vortex beams with different topological charge orders. The optical forces are calculated from the exact solutions of the electromagnetic fields provided by the generalized Lorentz-Mie theory. We show a remarkable agreement between the theoretical prediction and the experimental measurements of κ. Moreover, our numerical model gives us information about the electromagnetic fields inside the particle, offering valuable insights into the influence of the electromagnetic fields present in the vortex beam trapping scenario.

Kerker Conditions upon Lossless, Absorption, and Optical Gain Regimes.

The directionality and polarization of light show peculiar properties when the scattering by a dielectric sphere can be described exclusively by electric and magnetic dipolar modes. Particularly, when these modes oscillate in phase with equal amplitude, at the so-called first Kerker condition, the zero optical backscattering condition emerges for nondissipating spheres. However, the role of absorption and optical gain in the first Kerker condition remains unexplored. In this work, we demonstrate that either absorption or optical gain precludes the first Kerker condition and, hence, the absence of backscattered radiation light, regardless of the particle's size, incident wavelength, and incoming polarization. Finally, we derive the necessary prerequisites of the second Kerker condition of the zero forward light scattering, finding that optical gain is a compulsory requirement.

Lens-axicon separation to tailor aberration free focused Bessel-Gaussian beams in the paraxial regime.

Lens-axicon doublets have been used to produce Bessel-Gaussian beams, a narrow non-diffracting beam of relatively constant width. One problem of using Bessel-Gaussian beams is that there is a compromise between achieving a long effective focal length with a small central core radius and distributing the beam intensity between the central core and the off-axis rings. Here, we explore the advantage of tuning the lens-axicon separation, which allows us to have an additional degree of freedom to tailor the beam profile. Moreover, the separation between the lens and the axicon reduces the spherical aberrations in the beam profile, which can then be modeled within the paraxial regime. We study the detrimental effects of the spherical aberrations and provide several options to minimize them. We examine both sharp and shallow axicons used in combination with different converging lenses. We perform a series of detailed experiments to image the structure of the beam through the Bessel region. The spatial light distribution of the lens-axicon system is analyzed by using high dynamic range imaging and complemented with consistent theoretical calculations within the paraxial regime.

Symmetry Protection of Photonic Entanglement in the Interaction with a Single Nanoaperture.

In this work, we experimentally show that quantum entanglement can be symmetry protected in the interaction with a single subwavelength plasmonic nanoaperture, with a total volume of V∼0.2λ^{3}. In particular, we experimentally demonstrate that two-photon entanglement can be either completely preserved or completely lost after the interaction with the nanoaperture, solely depending on the relative phase between the quantum states. We achieve this effect by using specially engineered two-photon states to match the properties of the nanoaperture. In this way we can access a symmetry protected state, i.e., a state constrained by the geometry of the interaction to retain its entanglement. In spite of the small volume of interaction, we show that the symmetry protected entangled state retains its main properties. This connection between nanophotonics and quantum optics probes the fundamental limits of the phenomenon of quantum interference.

OAM interferometry: the detection of the rotational Doppler shift.

In this paper, we propose a new type of rotational Doppler shift measurement based on the OAM of light which is capable of measuring the rotation of a point source in the plane orthogonal to the observer line of sight. By analysing the correlations between OAM states of light emitted by rotating sources, the rotational Doppler shift, and hence the rate of rotation, can be measured. We demonstrate that an OAM interferometer capable of extracting the rotational Doppler shift from OAM correlations can be constructed from a standard OAM modesorter combined with a phase filter.

Quantum optical rotatory dispersion.

The phenomenon of molecular optical activity manifests itself as the rotation of the plane of linear polarization when light passes through chiral media. Measurements of optical activity and its wavelength dependence, that is, optical rotatory dispersion, can reveal information about intricate properties of molecules, such as the three-dimensional arrangement of atoms comprising a molecule. Given a limited probe power, quantum metrology offers the possibility of outperforming classical measurements. This has particular appeal when samples may be damaged by high power, which is a potential concern for chiroptical studies. We present the first experiment in which multiwavelength polarization-entangled photon pairs are used to measure the optical activity and optical rotatory dispersion exhibited by a solution of chiral molecules. Our work paves the way for quantum-enhanced measurements of chirality, with potential applications in chemistry, biology, materials science, and the pharmaceutical industry. The scheme that we use for probing wavelength dependence not only allows one to surpass the information extracted per photon in a classical measurement but also can be used for more general differential measurements.

Measurement and limitations of optical orbital angular momentum through corrected atmospheric turbulence.

In recent years, there have been a series of proposals to exploit the orbital angular momentum (OAM) of light for astronomical applications. The OAM of light potentially represents a new way in which to probe the universe. The study of this property of light entails the development of new instrumentation and problems which must be addressed. One of the key issues is whether we can overcome the loss of the information carried by OAM due to atmospheric turbulence. We experimentally analyze the effect of atmospheric turbulence on the OAM content of a signal over a range of realistic turbulence strengths typical for astronomical observations. With an adaptive optics system we are able to recover up to 89% power in an initial non-zero OAM mode (ℓ = 1) at low turbulence strengths (0.30" FWHM seeing). However, for poorer seeing conditions (1.1" FWHM seeing), the amount of power recovered is significantly lower (5%), showing that for the terrestrial detection of astronomical OAM, a careful design of the adaptive optics system is needed.

Far-field measurements of vortex beams interacting with nanoholes.

We measure the far-field intensity of vortex beams going through nanoholes. The process is analyzed in terms of helicity and total angular momentum. It is seen that the total angular momentum is preserved in the process, and helicity is not. We compute the ratio between the two transmitted helicity components, γm,p. We observe that this ratio is highly dependent on the helicity (p) and the angular momentum (m) of the incident vortex beam in consideration. Due to the mirror symmetry of the nanoholes, we are able to relate the transmission properties of vortex beams with a certain helicity and angular momentum, with the ones with opposite helicity and angular momentum. Interestingly, vortex beams enhance the γm,p ratio as compared to those obtained by Gaussian beams.

Quantum Emulation of Gravitational Waves.

Gravitational waves, as predicted by Einstein's general relativity theory, appear as ripples in the fabric of spacetime traveling at the speed of light. We prove that the propagation of small amplitude gravitational waves in a curved spacetime is equivalent to the propagation of a subspace of electromagnetic states. We use this result to propose the use of entangled photons to emulate the evolution of gravitational waves in curved spacetimes by means of experimental electromagnetic setups featuring metamaterials.

Isotropically polarized speckle patterns.

The polarization of the light scattered by an optically dense and random solution of dielectric nanoparticles shows peculiar properties when the scatterers exhibit strong electric and magnetic polarizabilities. While the distribution of the scattering intensity in these systems shows the typical irregular speckle patterns, the helicity of the incident light can be fully conserved when the electric and magnetic polarizabilities of the scatterers are equal. We show that the multiple scattering of helical beams by a random dispersion of "dual" dipolar nanospheres leads to a speckle pattern exhibiting a perfect isotropic constant polarization, a situation that could be useful in coherent control of light as well as in lasing in random media.

Angular momentum-induced circular dichroism in non-chiral nanostructures.

Circular dichroism, that is, the differential absorption of a system to left and right circularly polarized light, is one of the only techniques capable of providing morphological information of certain samples. In biology, for instance, circular dichroism spectroscopy is widely used to study the structure of proteins. More recently, it has also been used to characterize metamaterials and plasmonic structures. Typically, circular dichorism can only be observed in chiral objects. Here we present experimental results showing that a non-chiral sample such as a subwavelength circular nanoaperture can produce giant circular dichroism when a vortex beam is used to excite it. These measurements can be understood by studying the symmetries of the sample and the total angular momentum that vortex beams carry. Our results show that circular dichroism can provide a wealth of information about the sample when combined with the control of the total angular momentum of the input field.

Correcting vortex splitting in higher order vortex beams.

We demonstrate a general method for the first order compensation of singularity splitting in a vortex beam at a single plane. By superimposing multiple forked holograms on the SLM used to generate the vortex beam, we are able to compensate vortex splitting and generate beams with desired phase singularities of order ℓ = 0, 1, 2, and 3 in one plane. We then extend this method by application of a radial phase, in order to simultaneously compensate the observed vortex splitting at two planes (near and far field) for an ℓ = 2 beam.

Dual and anti-dual modes in dielectric spheres.

We present how the angular momentum of light can play an important role to induce a dual or anti-dual behaviour on a dielectric particle. Although the material the particle is made of is not dual, i.e. a dielectric does not interact with an electrical field in the same way as it does with a magnetic one, a spherical particle can behave as a dual system when the correct excitation beam is chosen. We study the conditions under which this dual or anti-dual behaviour can be induced.

Electromagnetic duality symmetry and helicity conservation for the macroscopic Maxwell's equations.

In this Letter, we show that the electromagnetic duality symmetry, broken in the microscopic Maxwell's equations by the presence of charges, can be restored for the macroscopic Maxwell's equations. The restoration of this symmetry is shown to be independent of the geometry of the problem. These results provide a tool for the study of light-matter interactions within the framework of symmetries and conservation laws. We illustrate its use by determining the helicity content of the natural modes of structures possessing spatial inversion symmetries and by elucidating the root causes for some surprising effects in the scattering off magnetic spheres.

Necessary symmetry conditions for the rotation of light.

Two conditions on symmetries are identified as necessary for a linear scattering system to be able to rotate the linear polarization of light: Lack of at least one mirror plane of symmetry and electromagnetic duality symmetry. Duality symmetry is equivalent to the conservation of the helicity of light in the same way that rotational symmetry is equivalent to the conservation of angular momentum. When the system is a solution of a single species of particles, the lack of at least one mirror plane of symmetry leads to the familiar requirement of chirality of the individual particle. With respect to helicity preservation, according to the analytical and numerical evidence presented in this paper, the solution preserves helicity if and only if the individual particle itself preserves helicity. However, only in the particular case of forward scattering the helicity preservation condition on the particle is relaxed: We show that the random orientation of the molecules endows the solution with an effective rotational symmetry; at its turn, this leads to helicity preservation in the forward scattering direction independently of any property of the particle. This is not the case for a general scattering direction. These results advance the current understanding of the phenomena of molecular optical activity and provide insight for the design of polarization control devices at the nanoscale.

Excitation of single multipolar modes with engineered cylindrically symmetric fields.

We present a new method to address multipolar resonances and to control the scattered field of a spherical scatterer. This method is based on the engineering of the multipolar content of the incident beam. We propose experimentally feasible techniques to generate light beams which contain only a few multipolar modes. The technique uses incident beams with a well defined component of the angular momentum and appropriate focusing with aplanatic lenses. The control of the multipolar content of light beams allow for the excitation of single Mie resonances and unprecedented control of the scattered field from spherical particles.

Characterization of dielectric spheres by spiral imaging.

We study the spiral spectra scattered off transparent dielectric spheres when probed by different Laguerre-Gaussian light beams, carrying nested topological wavefront dislocations. We show that such scattering data may be employed to determine geometrical properties of the spheres, such as their position. The technique is a generalization of standard Mie scattering, and it can be extended to study and to characterize nanospheres.

Polarization change induced by a galvanometric optical scanner.

We study the optical properties of a two-axis galvanometric optical scanner constituted by a pair of rotating planar mirrors, focusing our attention on the transformation induced on the polarization state of the input beam. We obtain the matrix that defines the transformation of the propagation direction of the beam and the Jones matrix that defines the transformation of the polarization state. Both matrices are expressed in terms of the rotation angles of two mirrors. Finally, we calculate the parameters of the general rotation in the Poincaré sphere that describes the change in the polarization state for each mutual orientation of the mirrors.

Deterministic subwavelength control of light confinement in nanostructures.

We propose a novel deterministic protocol, based on continuous light flows, that enables us to control the concentration of light in generic plasmonic nanostructures. Based on an exact inversion of the response tensor of the nanosystem, the so-called deterministic optical inversion protocol provides a physical solution for the incident field leading to a desired near-field pattern, expressed in the form of a coherent superposition of high-order beams. We demonstrate the high degree of control achieved on complex plasmonic architectures and quantify its efficiency and accuracy.