Temperature relaxation in strongly-coupled binary ionic mixtures.

New facilities such as the National Ignition Facility and the Linac Coherent Light Source have pushed the frontiers of high energy-density matter. These facilities offer unprecedented opportunities for exploring extreme states of matter, ranging from cryogenic solid-state systems to hot, dense plasmas, with applications to inertial-confinement fusion and astrophysics. However, significant gaps in our understanding of material properties in these rapidly evolving systems still persist. In particular, non-equilibrium transport properties of strongly-coupled Coulomb systems remain an open question. Here, we study ion-ion temperature relaxation in a binary mixture, exploiting a recently-developed dual-species ultracold neutral plasma. We compare measured relaxation rates with atomistic simulations and a range of popular theories. Our work validates the assumptions and capabilities of the simulations and invalidates theoretical models in this regime. This work illustrates an approach for precision determinations of detailed material properties in Coulomb mixtures across a wide range of conditions.

Head-on collision of compressional shocks in two-dimensional Yukawa systems.

The head-on collision of compressional shocks in two-dimensional dusty plasmas is investigated using both molecular dynamical and Langevin simulations. Two compressional shocks are generated from the inward compressional boundaries in simulations. It is found that, during the collision of shocks, there is a generally existing time delay of shocks τ, which diminishes monotonically with the increasing compressional speed of boundaries, corresponding to the time resolution of the studied system. Dispersive shock waves (DSWs) are generated around the shock front for some conditions. It is also found that the period of the DSW decreases monotonically with the inward compressional speed of boundaries, more substantially than the time delay of shocks τ. When the inward compressional speed of boundaries increases further, the DSWs gradually vanish. We speculate that, for these high compressional speeds of boundaries, the period of the DSW might be reduced to a comparable timescale of the time delay of shocks τ, i.e., the time resolution of our studied system, or even shorter, thus the DSW reasonably vanishes.

Universal relationship of compression shocks in two-dimensional Yukawa systems.

Using molecular dynamical simulations, compressional shocks in two-dimensional (2D) dusty plasmas are quantitatively investigated under various conditions. A universal relationship between the thermal and the drift velocities after shocks is discovered in 2D Yukawa systems. Using the equation of state of 2D Yukawa liquids, and the obtained pressure from the Rankine-Hugoniot relation, an analytical relation between the thermal and the drift velocities is derived, which well agrees with the discovered universal relationship for various conditions.

Erratum: Pressure and energy of compressional shocks in two-dimensional Yukawa systems [Phys. Rev. E 100, 043203 (2019)].

This corrects the article DOI: 10.1103/PhysRevE.100.043203.

Continuous and discontinuous transitions in the depinning of two-dimensional dusty plasmas on a one-dimensional periodic substrate.

Langevin dynamical simulations are performed to study the depinning dynamics of two-dimensional dusty plasmas on a one-dimensional periodic substrate. From the diagnostics of the sixfold coordinated particles P_{6} and the collective drift velocity V_{x}, three different states appear, which are the pinning, disordered plastic flow, and moving ordered states. It is found that the depth of the substrate is able to modulate the properties of the depinning phase transition, based on the results of P_{6} and V_{x}, as well as the observation of hysteresis of V_{x} while increasing and decreasing the driving force monotonically. When the depth of the substrate is shallow, there are two continuous phase transitions. When the potential well depth slightly increases, the phase transition from the pinned to the disordered plastic flow states is continuous; however, the phase transition from the disordered plastic flow to the moving ordered states is discontinuous. When the substrate is even deeper, the phase transition from the pinned to the disordered plastic flow states changes to discontinuous. When the depth of the substrate further increases, as the driving force increases, the pinned state changes to the moving ordered state directly, so that the disordered plastic flow state disappears completely.

Pressure and energy of compressional shocks in two-dimensional Yukawa systems.

The propagation of compressional shocks in two-dimensional (2D) dusty plasmas is investigated using MD simulations under various conditions. The shock Hugoniot curves of the relationship between the shock front speed D and the mean particle speed v[over ¯] after shocks are obtained and analytically fit to parabolic expressions. As the screening parameter increases, the weaker Yukawa interparticle interaction cause the shock Hugoniot curves to be more linear. Combining the obtained shock Hugoniot curves with the Rankine-Hugoniot jump relations, analytic expressions of pressure and energy after the shocks in 2D Yukawa systems are obtained, which are functions of the observable quantities, like the shock front speed D or the mean particle speed v[over ¯] or the specific volume.

Depinning dynamics of two-dimensional dusty plasmas on a one-dimensional periodic substrate.

We investigate the depinning dynamics of two-dimensional dusty plasmas driven over one-dimensional periodic substrates using Langevin dynamical simulations. We find that, for a specific range of substrate strengths, as the external driving force increases from zero, there are three different states, which are the pinned, the disordered plastic flow, and the moving ordered states, respectively. These three states are clearly observed using different diagnostics, including the collective drift velocity, static structural measures, the particle trajectories, the mean-squared displacements, and the kinetic temperature. We compare the observed depinning dynamics here with the depinning dynamics in other systems.

Erratum: Extremely Low Electron-ion Temperature Relaxation Rates in Warm Dense Hydrogen: Interplay between Quantum Electrons and Coupled Ions [Phys. Rev. Lett. 122, 015001 (2019)].

This corrects the article DOI: 10.1103/PhysRevLett.122.015001.

Extremely Low Electron-ion Temperature Relaxation Rates in Warm Dense Hydrogen: Interplay between Quantum Electrons and Coupled Ions.

Theoretical and computational modeling of nonequilibrium processes in warm dense matter represents a significant challenge. The electron-ion relaxation process in warm dense hydrogen is investigated here by nonequilibrium molecular dynamics using the constrained electron force field (CEFF) method. CEFF evolves wave packets that incorporate dynamic quantum diffraction that obviates the Coulomb catastrophe. Predictions from this model reveal temperature relaxation times as much as three times longer than prior molecular dynamics results based on quantum statistical potentials. Through analyses of energy distributions and mean free paths, this result can be traced to delocalization. Finally, an improved GMS [Gericke, Murillo, and Schlanges, Phys. Rev. E 78, 025401 (2008)PRESCM1539-375510.1103/PhysRevE.78.025401] model is proposed, in which the Coulomb logarithms are in good agreement with CEFF results.

Thermodynamic and Kinetic Properties of Shocks in Two-Dimensional Yukawa Systems.

Particle-level simulations of shocked plasmas are carried out to examine kinetic properties not captured by hydrodynamic models. In particular, molecular dynamics simulations of 2D Yukawa plasmas with variable couplings and screening lengths are used to examine shock features unique to plasmas, including the presence of dispersive shock structures for weak shocks. A phase-space analysis reveals several kinetic properties, including anisotropic velocity distributions, non-Maxwellian tails, and the presence of fast particles ahead of the shock, even for moderately low Mach numbers. We also examine the thermodynamics (Rankine-Hugoniot relations) of recent experiments [Phys. Rev. Lett. 111, 015002 (2013)PRLTAO0031-900710.1103/PhysRevLett.111.015002] and find no anomalies in their equations of state.

Viscosity of two-dimensional strongly coupled dusty plasma modified by a perpendicular magnetic field.

Transport properties of two-dimensional (2D) strongly coupled dusty plasmas have been investigated in detail, but never for viscosity with a strong perpendicular magnetic field; here, we examine this scenario using Langevin dynamics simulations of 2D liquids with a binary Yukawa interparticle interaction. The shear viscosity η of 2D liquid dusty plasma is estimated from the simulation data using the Green-Kubo relation, which is the integration of the shear stress autocorrelation function. It is found that, when a perpendicular magnetic field is applied, the shear viscosity of 2D liquid dusty plasma is modified substantially. When the magnetic field is increased, its viscosity increases at low temperatures, while at high temperatures its viscosity diminishes. It is determined that these different variational trends of η arise from the different behaviors of the kinetic and potential parts of the shear stress under external magnetic fields.

Publisher's Note: Generalized hydrodynamics model for strongly coupled plasmas [Phys. Rev. E 92, 013107 (2015)].

This corrects the article DOI: 10.1103/PhysRevE.92.013107.

Strongly-coupled plasmas formed from laser-heated solids.

We present an analysis of ion temperatures in laser-produced plasmas formed from solids with different initial lattice structures. We show that the equilibrium ion temperature is limited by a mismatch between the initial crystallographic configuration and the close-packed configuration of a strongly-coupled plasma, similar to experiments in ultracold neutral plasmas. We propose experiments to demonstrate and exploit this crystallographic heating in order to produce a strongly coupled plasma with a coupling parameter of several hundred.

Generalized hydrodynamics model for strongly coupled plasmas.

Beginning with the exact equations of the Bogoliubov-Born-Green-Kirkwood-Yvon hierarchy, we obtain the density, momentum, and stress tensor-moment equations. We close the moment equations with two closures, one that guarantees an equilibrium state given by density-functional theory and another that includes collisions in the relaxation of the stress tensor. The introduction of a density functional-theory closure ensures self-consistency in the equation-of-state properties of the plasma (ideal and excess pressure, electric fields, and correlations). The resulting generalized hydrodynamics thus includes all impacts of Coulomb coupling, viscous damping, and the high-frequency (viscoelastic) response. We compare our results with those of several known models, including generalized hydrodynamic theory and models obtained using the Singwi-Tosi-Land-Sjolander approximation and the quasilocalized charge approximation. We find that the viscoelastic response, including both the high-frequency elastic generalization and viscous wave damping, is important for correctly describing ion-acoustic waves. We illustrate this result by considering three very different systems: ultracold plasmas, dusty plasmas, and dense plasmas. The new model is validated by comparing its results with those of the current autocorrelation function obtained from molecular-dynamics simulations of Yukawa plasmas, and the agreement is excellent. Generalizations of this model to mixtures and quantum systems should be straightforward.

Using higher ionization states to increase Coulomb coupling in an ultracold neutral plasma.

We report measurements and simulations of the time-evolving rms velocity distribution in an ultracold neutral plasma. A strongly coupled ultracold neutral Ca+ plasma is generated by photoionizing laser-cooled atoms close to threshold. A fraction of these ions is then promoted to the second ionization state to form a mixed Ca+-Ca2+ plasma. By varying the time delay between the first and the second ionization events, a minimum in ion heating is achieved. We show that the Coulomb strong-coupling parameter Γ increases by a factor of 1.4 to a maximum value of 3.6. A pure Ca2+ plasma would have Γ=6.8, moving these strongly coupled systems closer to the regime of liquid-like correlations.

Unified description of linear screening in dense plasmas.

Electron screening of ions is among the most fundamental properties of plasmas, determining the effective ionic interactions that impact all properties of a plasma. With the development of new experimental facilities that probe high-energy-density physics regimes ranging from warm dense matter to hot dense matter, a unified framework for describing dense plasma screening has become essential. Such a unified framework is presented here based on finite-temperature orbital-free density functional theory, including gradient corrections and exchange-correlation effects. We find a new analytic pair potential for the ion-ion interaction that incorporates moderate electronic coupling, quantum degeneracy, gradient corrections to the free energy, and finite temperatures. This potential can be used in large-scale "classical" molecular dynamics simulations, as well as in simpler theoretical models (e.g., integral equations and Monte Carlo), with no additional computational complexity. The new potential theoretically connects limits of Debye-Hückel-Yukawa, Lindhard, Thomas-Fermi, and Bohmian quantum hydrodynamics descriptions. Based on this new potential, we predict ionic static structure factors that can be validated using x-ray Thomson scattering data.

Kinetic theory molecular dynamics and hot dense matter: theoretical foundations.

Electrons are weakly coupled in hot, dense matter that is created in high-energy-density experiments. They are also mildly quantum mechanical and the ions associated with them are classical and may be strongly coupled. In addition, the dynamical evolution of plasmas under these hot, dense matter conditions involve a variety of transport and energy exchange processes. Quantum kinetic theory is an ideal tool for treating the electrons but it is not adequate for treating the ions. Molecular dynamics is perfectly suited to describe the classical, strongly coupled ions but not the electrons. We develop a method that combines a Wigner kinetic treatment of the electrons with classical molecular dynamics for the ions. We refer to this hybrid method as "kinetic theory molecular dynamics," or KTMD. The purpose of this paper is to derive KTMD from first principles and place it on a firm theoretical foundation. The framework that KTMD provides for simulating plasmas in the hot, dense regime is particularly useful since current computational methods are generally limited by their inability to treat the dynamical quantum evolution of the electronic component. Using the N-body von Neumann equation for the electron-proton plasma, three variations of KTMD are obtained. Each variant is determined by the physical state of the plasma (e.g., collisional versus collisionless). The first variant of KTMD yields a closed set of equations consisting of a mean-field quantum kinetic equation for the electron one-particle distribution function coupled to a classical Liouville equation for the protons. The latter equation includes both proton-proton Coulombic interactions and an effective electron-proton interaction that involves the convolution of the electron density with the electron-proton Coulomb potential. The mean-field approach is then extended to incorporate equilibrium electron-proton correlations through the Singwi-Tosi-Land-Sjolander (STLS) ansatz. This is the second variant of KTMD. The STLS contribution produces an effective electron-proton interaction that involves the electron-proton structure factor, thereby extending the usual mean-field theory to correlated but near equilibrium systems. Finally, a third variant of KTMD is derived. It includes dynamical electrons and their correlations coupled to a MD description for the ions. A set of coupled equations for the one-particle electron Wigner function and the electron-electron and electron-proton correlation functions are coupled to a classical Liouville equation for the protons. This latter variation has both time and momentum dependent correlations.

Superdiffusion of two-dimensional Yukawa liquids due to a perpendicular magnetic field.

Stochastic transport of a two-dimensional (2D) dusty plasma liquid with a perpendicular magnetic field is studied. Superdiffusion is found to occur especially at higher magnetic fields with ß of order unity. Here, ß = ω(c)/ω(pd) is the ratio of the cyclotron and plasma frequencies for dust particles. The mean-square displacement MSD = 4D(α)t(α) is found to have an exponent α > 1, indicating superdiffusion, with α increasing monotonically to 1.1 as ß increases to unity. The 2D Langevin molecular dynamics simulation used here also reveals that another indicator of random particle motion, the velocity autocorrelation function, has a dominant peak frequency ω(peak) that empirically obeys ω(peak)(2) = ω(c)(2) + ω(pd)(2)/4.

Molecular dynamics simulations of temperature equilibration in dense hydrogen.

The temperature equilibration rate between electrons and protons in dense hydrogen has been calculated with molecular dynamics simulations for temperatures between 10 and 600eV and densities between 10;{20}cm;{-3}to10;{24}cm;{-3} . Careful attention has been devoted to convergence of the simulations, including the role of semiclassical potentials. We find that for Coulomb logarithms L greater, similar1 , a model by Gericke-Murillo-Schlanges (GMS) [D. O. Gericke, Phys. Rev. E 65, 036418 (2002)] based on a T -matrix method and the approach by Brown-Preston-Singleton [L. S. Brown, Phys. Rep. 410, 237 (2005)] agrees with the simulation data to within the error bars of the simulation. For smaller Coulomb logarithms, the GMS model is consistent with the simulation results. Landau-Spitzer models are consistent with the simulation data for L>4 .

Gibbs-Bogolyubov inequality and transport properties for strongly coupled Yukawa fluids.

The Gibbs-Bogolyubov inequality is used to establish a mapping between the Yukawa system and both the hard-sphere and the one-component reference systems. The transport coefficients of self-diffusion, shear viscosity, and thermal conductivity are computed for the Yukawa fluid using known properties of the reference systems. Comparisons are made with simulation results. For sufficiently strong screening, the hard-sphere reference system yields a lower upper bound of the Yukawa Helmholtz free energy and a better estimate of the Yukawa transport coefficients.