Anomalous Relativistic Emission from Self-Modulated Plasma Mirrors.

The interaction of intense laser pulses with plasma mirrors has demonstrated the ability to generate high-order harmonics, producing a bright source of extreme ultraviolet (XUV) radiation and attosecond pulses. Here, we report an unexpected transition in this process. We show that the loss of spatiotemporal coherence in the reflected high harmonics can lead to a new regime of highly efficient coherent XUV generation, with an extraordinary property where the radiation is directionally anomalous, propagating parallel to the mirror surface. With analytical calculations and numerical particle-in-cell simulations, we discover that the radiation emission is due to laser-driven oscillations of relativistic electron nanobunches that originate from a plasma surface instability.

Phase-matched high-order harmonic generation in pre-ionized noble gases.

One of the main difficulties of efficiently generating high-order harmonics in long neutral-gas targets is to reach the phase-matching conditions. The issue is that the medium cannot be sufficiently ionized by the driving laser due to plasma defocusing. We propose a method to improve the phase-matching by pre-ionizing the gas using a weak capillary discharge. We have demonstrated this mechanism, for the first time, in absorption-limited XUV generation by an 800 nm femtosecond laser in argon and krypton. The ability to control phase-mismatch is confirmed by an analytical model and numerical simulations of the entire generation process. Our method allows to increase the efficiency of the harmonic generation significantly, paving the way towards photon-hungry applications of these compact short-wavelength sources.

Two-Color Soft X-Ray Lasing in a High-Density Nickel-like Krypton Plasma.

We report evidence of strong lasing on the 4p-4s transition at 62.7 nm in nickel-like krypton occurring simultaneously with the usual 4d-4p lasing at 32.8 nm. The gain dynamics of both transitions were experimentally and numerically investigated and found comparable. The two-color amplifier was seeded by the same harmonic pulse, therefore producing a short-duration coherent two-color soft x-ray laser pulse. Both transitions offer similar prospects of pulse energy and duration and could lead to the delivery of intense and ultrashort two-color coherent soft x-ray pulses with a controllable delay.

Imaging Michelson interferometer for a low-density gas jet characterization.

A new optical probing method with increased interferometric sensitivity for a low-density gas jet characterization is presented. The proposed technique employs a Michelson interferometer with a self-imaging object arm, which enables the relay imaging of the object on itself, and in this way, the phase sensitivity of the device is increased by a double propagation of the object laser beam through the gas jet. The wavelength of 405 nm was chosen to further increase the sensitivity by increasing the probe wavenumber. A low-density argon gas jet with various backing pressures was characterized by our method and by a commonly used Mach-Zehnder interferometer setup showing the expected twofold increase in the signal to noise ratio in the double pass configuration.

High-flux source of coherent XUV pulses for user applications.

We present experimental results obtained at a user-oriented XUV beamline implemented at the ELI Beamlines facility. The coherent XUV radiation is produced via high harmonic generation in gases in a loose focusing geometry. The beamline is designed to be driven by 1 kHz, 100 mJ, 20 fs pulses centered at a wavelength of 830 nm. Results such as XUV spectra, beam wavefront and pulse energy obtained during the beamline commissioning with a commercial 1 kHz, 5 mJ, 40 fs laser system are presented. A unique XUV spectrometer for source characterization designed to reach a very high sensitivity is described in detail, and we demonstrate a novel technique for single-shot and every-shot XUV pulse energy measurement.

Pulse duration of a partially coherent soft X-ray laser estimated from far-field speckle statistics.

A novel method for estimating the pulse duration of partially coherent soft X-ray pulses from a far-field intensity pattern is presented. The method is based on intensity statistics at a single point in space and time, which allows the number of coherent longitudinal modes to be measured. Utilizing the knowledge of the coherence time of the radiation, either from the measurement of the spectral bandwidth or from numerical simulations, the duration of each individual pulse can be evaluated. This method was used to estimate the pulse duration of the laser-driven nickel-like molybdenum soft X-ray laser that is based on amplified spontaneous emission from a narrow plasma column and emits at a wavelength of 18.9 nm. By varying the length of the gain medium, a clear dependence of the number of modes caused mainly by the spectral line narrowing was observed. Supported by simulations of radiative transfer and pulse propagation, the pulse duration at the end of a 3 mm long gain medium was estimated to be 3.5 ps. The experimental data from far-field intensity patterns were also analyzed by applying the generalized van Cittert-Zernike theorem, providing a lower bound of effective source size.

Demonstration of a Circularly Polarized Plasma-Based Soft-X-Ray Laser.

We report the first experimental demonstration of a laser-driven circularly polarized soft-x-ray laser chain. It has been achieved by seeding a 32.8 nm Kr ix plasma amplifier with a high-order harmonic beam, which has been circularly polarized using a four-reflector polarizer. Our measurements testify that the amplified radiation maintains the initial polarization of the seed pulse in good agreement with our Maxwell-Bloch modeling. The resulting fully circular soft-x-ray laser beam exhibits a Gaussian profile and yields about 10^{10} photons per shot, fulfilling the requirements for laboratory-scale photon-demanding application experiments.

Extreme ultraviolet interferometry of warm dense matter in laser plasmas.

We demonstrate that interferometric probing with extreme ultraviolet (EUV) laser light enables determination of the degree of ionization of the "warm dense matter" produced between the critical and ablation surfaces of laser plasmas. Interferometry has been utilized to measure both transmission and phase information for an EUV laser beam at the photon energy of 58.5 eV, probing longitudinally through laser-irradiated plastic (parylene-N) targets (thickness 350 nm) irradiated by a 300 ps duration pulse of wavelength 438 nm and peak irradiance 10(12) W cm(-2). The transmission of the EUV probe beam provides a measure of the rate of target ablation, as ablated plasma becomes close to transparent when the photon energy is less than the ionization energy of the predominant ion species. We show that refractive indices η below the solid parylene N (η(solid) = 0.946) and expected plasma values are produced in the warm dense plasma created by laser irradiation due to bound-free absorption in C(+).

Aberration-free laser beam in the soft x-ray range.

By seeding an optical-field-ionized population-inverted plasma amplifier with the 25th harmonic of an IR laser, we have achieved what we believe to be the first aberration-free laser beam in the soft x-ray spectral range. This laser emits within a cone of 1.34 mrad(1/e(2)) at a repetition rate of 10 Hz at a central wavelength of 32.8 nm. The beam exhibits a circular profile and wavefront distortions as low as lambda/17. A theoretical analysis of these results shows that this high beam quality is due to spatial filtering of the seed beam by the plasma amplifier aperture.