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1.
Environ Sci Technol ; 57(48): 19575-19583, 2023 Dec 05.
Article in English | MEDLINE | ID: mdl-37991894

ABSTRACT

China's civil aviation market has rapidly expanded, becoming the world's second-largest. However, the air quality and health impacts caused by its aircraft emissions have been inadequately assessed. Here, we leverage an updated emission inventory of air pollutants with improved temporal and spatial resolution based on hundreds of thousands of flight trajectories and simulate aviation-attributable contributions to ground-level air pollution in China. We find that in 2017, the annual-average aviation-attributed PM2.5 and O3 concentrations were 0.4-1.5 and 10.6-14.5 µg·m-3, respectively, suggesting that aviation emissions have become an increasingly important source of ambient air pollution. The contributions attributable to high-altitude emissions (climb/cruise/descent) were comparable to those at low altitudes (landing and takeoff). Aviation-attributed ambient PM2.5 and O3 exposures are estimated to have caused about 67,000 deaths in China in 2017, with populous coastal regions in Eastern China suffering the most due to the dense aviation activity. We recommend that industrial and policy stakeholders expedite an agenda of regulating air pollutants harmonized with decarbonization efforts for a more sustainable aviation future.


Subject(s)
Air Pollutants , Air Pollution , Aviation , Humans , Particulate Matter/analysis , Environmental Monitoring , Air Pollution/analysis , Air Pollutants/analysis , China
2.
Environ Sci Technol ; 57(44): 16989-16998, 2023 11 07.
Article in English | MEDLINE | ID: mdl-37902187

ABSTRACT

Benefiting from international economic cooperation on income, technology diffusion, and employment, China also suffers its environmental and health impacts, from both international trade (IT), as is now widely understood, and international industrial transfer (IIT), which has been largely unrecognized. Here, we develop a comprehensive framework to estimate the impacts of exporting IT and receiving IIT. We find that China's emissions of CO2 and almost all air pollutants associated with IIT and IT together grew after 1997 but then declined after 2010, with the peak shares of national total emissions ranging 18-31% for different species. These sources further accounted for 3.8% of nationwide PM2.5 concentrations and 94,610 (76,000-112,040) premature deaths in 2012, and the values declined to 2.6% and 67,370 (52,390-81,810), respectively, for 2017. Separated, the contribution of IIT to those impacts was more than twice that of IT. Scenario analyses suggest that improving emission controls in its less-developed regions would effectively reduce the impact of economic globalization, but such a benefit could be largely offset by strengthened international economic cooperation. The outcomes provide a scientific basis for adjusting China's strategic roles in the international distribution of industrial production and its formulation of relevant environmental policies from a comprehensive perspective.


Subject(s)
Air Pollutants , Air Pollution , Commerce , Internationality , Air Pollution/analysis , Industry , Air Pollutants/analysis , China , Carbon Dioxide/analysis
3.
Nat Commun ; 13(1): 3172, 2022 Jun 08.
Article in English | MEDLINE | ID: mdl-35676273

ABSTRACT

The Chinese government has set long-term carbon neutrality and renewable energy (RE) development goals for the power sector. Despite a precipitous decline in the costs of RE technologies, the external costs of renewable intermittency and the massive investments in new RE capacities would increase electricity costs. Here, we develop a power system expansion model to comprehensively evaluate changes in the electricity supply costs over a 30-year transition to carbon neutrality. RE supply curves, operating security constraints, and the characteristics of various generation units are modelled in detail to assess the cost variations accurately. According to our results, approximately 5.8 TW of wind and solar photovoltaic capacity would be required to achieve carbon neutrality in the power system by 2050. The electricity supply costs would increase by 9.6 CNY¢/kWh. The major cost shift would result from the substantial investments in RE capacities, flexible generation resources, and network expansion.

4.
Nat Commun ; 13(1): 1008, 2022 02 23.
Article in English | MEDLINE | ID: mdl-35197466

ABSTRACT

Recent evidence shows that carbon emissions in China are likely to peak ahead of 2030. However, the social and economic impacts of such an early carbon peak have rarely been assessed. Here we focus on the economic costs and health benefits of different carbon mitigation pathways, considering both possible socio-economic futures and varying ambitions of climate policies. We find that an early peak before 2030 in line with the 1.5 °C target could avoid ~118,000 and ~614,000 PM2.5 attributable deaths under the Shared Socioeconomic Pathway 1, in 2030 and 2050, respectively. Under the 2 °C target, carbon mitigation costs could be more than offset by health co-benefits in 2050, bringing a net benefit of $393-$3,017 billion (in 2017 USD value). This study not only provides insight into potential health benefits of an early peak in China, but also suggests that similar benefits may result from more ambitious climate targets in other countries.


Subject(s)
Air Pollutants , Air Pollution , Air Pollutants/analysis , Air Pollution/analysis , Air Pollution/prevention & control , Carbon Dioxide/analysis , China , Climate Change , Particulate Matter/analysis
5.
Environ Int ; 158: 106909, 2022 01.
Article in English | MEDLINE | ID: mdl-34619531

ABSTRACT

This study investigates the contribution of formaldehyde from residential building materials to ambient air in mainland China. Based on 265 indoor field tests in 9 provinces, we estimate that indoor residential sources are responsible for 6.66% of the total anthropogenic formaldehyde in China's ambient air (range for 31 provinces: 1.88-18.79%). Residential building materials rank 6th among 81 anthropogenic sources (range: 2nd-10th for 31 provinces). Emission intensities show large spatial variability between and within regions due to different residential densities, emission characteristics of building materials, and indoor thermal conditions. Our findings indicate that formaldehyde from the indoor environment is a significant source of ambient formaldehyde, especially in urban areas. This study will help to more accurately evaluate exposure to ambient formaldehyde and its related pollutants, and will assist in formulating policies to protect air quality and public health.


Subject(s)
Air Pollutants , Air Pollution, Indoor , Air Pollution , Air Pollutants/analysis , Air Pollution/analysis , Air Pollution, Indoor/analysis , China , Formaldehyde/analysis
6.
Nat Commun ; 12(1): 6953, 2021 Nov 29.
Article in English | MEDLINE | ID: mdl-34845233

ABSTRACT

The Japanese government has announced a commitment to net-zero greenhouse gas emissions by 2050. It envisages an important role for hydrogen in the nation's future energy economy. This paper explores the possibility that a significant source for this hydrogen could be produced by electrolysis fueled by power generated from offshore wind in China. Hydrogen could be delivered to Japan either as liquid, or bound to a chemical carrier such as toluene, or as a component of ammonia. The paper presents an analysis of factors determining the ultimate cost for this hydrogen, including expenses for production, storage, conversion, transport, and treatment at the destination. It concludes that the Chinese source could be delivered at a volume and cost consistent with Japan's idealized future projections.

7.
Proc Natl Acad Sci U S A ; 118(42)2021 10 19.
Article in English | MEDLINE | ID: mdl-34635590

ABSTRACT

As the world's largest CO2 emitter, China's ability to decarbonize its energy system strongly affects the prospect of achieving the 1.5 °C limit in global, average surface-temperature rise. Understanding technically feasible, cost-competitive, and grid-compatible solar photovoltaic (PV) power potentials spatiotemporally is critical for China's future energy pathway. This study develops an integrated model to evaluate the spatiotemporal evolution of the technology-economic-grid PV potentials in China during 2020 to 2060 under the assumption of continued cost degression in line with the trends of the past decade. The model considers the spatialized technical constraints, up-to-date economic parameters, and dynamic hourly interactions with the power grid. In contrast to the PV production of 0.26 PWh in 2020, results suggest that China's technical potential will increase from 99.2 PWh in 2020 to 146.1 PWh in 2060 along with technical advances, and the national average power price could decrease from 4.9 to 0.4 US cents/kWh during the same period. About 78.6% (79.7 PWh) of China's technical potential will realize price parity to coal-fired power in 2021, with price parity achieved nationwide by 2023. The cost advantage of solar PV allows for coupling with storage to generate cost-competitive and grid-compatible electricity. The combined systems potentially could supply 7.2 PWh of grid-compatible electricity in 2060 to meet 43.2% of the country's electricity demand at a price below 2.5 US cents/kWh. The findings highlight a crucial energy transition point, not only for China but for other countries, at which combined solar power and storage systems become a cheaper alternative to coal-fired electricity and a more grid-compatible option.

8.
Environ Int ; 152: 106482, 2021 07.
Article in English | MEDLINE | ID: mdl-33706036

ABSTRACT

Facing the dual challenges of climate change and air pollution, China has made great efforts to explore the co-control strategies for the both. We assessed the benefits of carbon and pollution control policies on air quality and human health, with an integrated framework combining an energy-economic model, an air quality model and a concentration-response model. With a base year 2015, seven combined scenarios were developed for 2030 based on three energy scenarios and three end-of-pipe control ones. Policy-specific benefits were then evaluated, indicated by the reduced emissions, surface concentrations of major pollutants, and premature deaths between scenarios. Compared to the 2030 baseline scenario, the nationwide PM2.5- and O3-related mortality was expected to decline 23% or 289 (95% confidence interval: 220-360) thousand in the most stringent scenario, and three quarters of the avoided deaths were attributed to the end-of-pipe control measures. Provinces in heavily polluted and densely populated regions would benefit more from carbon and pollution control strategies. The population fractions with PM2.5 exposure under the national air quality standard (35 µg/m3) and WHO guideline (10 µg/m3) would be doubled from 2015 to 2030 (the most stringent scenario), while still very few people would live in areas with the WHO guideline achieved for O3 (100 µg/m3). Increased health impact of O3 suggested a great significance of joint control of PM2.5 and O3 in future policy-making.


Subject(s)
Air Pollutants , Air Pollution , Air Pollutants/analysis , Air Pollution/analysis , Air Pollution/prevention & control , Carbon , China , Humans , Particulate Matter/analysis , Policy
9.
Nat Commun ; 12(1): 1698, 2021 03 16.
Article in English | MEDLINE | ID: mdl-33727563

ABSTRACT

Recognizing that bioenergy with carbon capture and storage (BECCS) may still take years to mature, this study focuses on another photosynthesis-based, negative-carbon technology that is readier to implement in China: biomass intermediate pyrolysis poly-generation (BIPP). Here we find that a BIPP system can be profitable without subsidies, while its national deployment could contribute to a 61% reduction of carbon emissions per unit of gross domestic product in 2030 compared to 2005 and result additionally in a reduction in air pollutant emissions. With 73% of national crop residues used between 2020 and 2030, the cumulative greenhouse gas (GHG) reduction could reach up to 8620 Mt CO2-eq by 2050, contributing 13-31% of the global GHG emission reduction goal for BECCS, and nearly 4555 Mt more than that projected for BECCS alone in China. Thus, China's BIPP deployment could have an important influence on achieving both national and global GHG emissions reduction targets.

10.
Proc Natl Acad Sci U S A ; 117(41): 25370-25377, 2020 10 13.
Article in English | MEDLINE | ID: mdl-32968019

ABSTRACT

China started to implement comprehensive measures to mitigate traffic pollution at the end of 1990s, but the comprehensive effects, especially on ambient air quality and public health, have not yet been systematically evaluated. In this study, we analyze the effects of vehicle emission control measures on ambient air pollution and associated deaths attributable to long-term exposures of fine particulate matter (PM2.5) and O3 based on an integrated research framework that combines scenario analysis, air quality modeling, and population health risk assessment. We find that the total impact of these control measures was substantial. Vehicular emissions during 1998-2015 would have been 2-3 times as large as they actually were, had those measures not been implemented. The national population-weighted annual average concentrations of PM2.5 and O3 in 2015 would have been higher by 11.7 µg/m3 and 8.3 parts per billion, respectively, and the number of deaths attributable to 2015 air pollution would have been higher by 510 thousand (95% confidence interval: 360 thousand to 730 thousand) without these controls. Our analysis shows a concentration of mortality impacts in densely populated urban areas, motivating local policymakers to design stringent vehicle emission control policies. The results imply that vehicle emission control will require policy designs that are more multifaceted than traditional controls, primarily represented by the strict emission standards, with careful consideration of the challenges in coordinated mitigation of both PM2.5 and O3 in different regions, to sustain improvement in air quality and public health given continuing swift growth in China's vehicle population.


Subject(s)
Air Pollutants/chemistry , Air Pollution/prevention & control , Ozone , Particulate Matter , Transportation , Vehicle Emissions/analysis , China , Environmental Exposure/prevention & control , Environmental Monitoring/methods , Humans , Risk Assessment
11.
Environ Sci Technol ; 53(18): 11013-11022, 2019 Sep 17.
Article in English | MEDLINE | ID: mdl-31415163

ABSTRACT

Mass adoption of electric vehicles (EVs) is widely viewed as essential to address climate change and requires a compelling case for ownership worldwide. While the manufacturing costs and technical capabilities of EVs are similar across regions, customer needs and economic contexts vary widely. Assessments of the all-electric-range required to cover day-to-day driving demand, and the climate and economic benefits of EVs, need to account for differences in regional characteristics and individual travel patterns. To meet this need travel profiles for 1681 light-duty passenger vehicles in China, the U.S., and Germany were used to make the first consistent multiregional comparison of customer and greenhouse gas (GHG) emission benefits of EVs. We show that despite differences in fuel prices, driving patterns, and subsidies, the economic benefits/challenges of EVs are generally similar across regions. Individuals who are economically most likely to adopt EVs have GHG benefits that are substantially greater than for average drivers. Such "priority" EV customers have large (32%-63%) reductions in cradle-to-grave GHG emissions. It is shown that low battery costs (below approximately $100/kWh) and a portfolio of EV offerings are required for mass adoption of electric vehicles.


Subject(s)
Gasoline , Vehicle Emissions , China , Germany , Greenhouse Effect , Humans , Motor Vehicles , United States
12.
Environ Pollut ; 251: 415-424, 2019 Aug.
Article in English | MEDLINE | ID: mdl-31103001

ABSTRACT

Emission inventories are critical to understanding the sources of air pollutants, but have high uncertainties in China due in part to insufficient on-site measurements. In this study, we developed a method of examining, screening and applying online data from the country's improving continuous emission monitoring systems (CEMS) to reevaluate a "bottom-up" emission inventory of China's coal-fired power sector. The benefits of China's current national emission standards and ultra-low emission policy for the sector were quantified assuming their full implementation. The derived national average emission factors of SO2, NOx and particulate matter (PM) were 1.00, 1.00 and 0.25 kg/t-coal respectively for 2015 based on CEMS data, smaller than those of previous studies that may not fully recognize improved emission controls in recent years. The annual emissions of SO2, NOx and PM from the sector were recalculated at 1321, 1430 and 334 Gg respectively, 75%, 63% and 76% smaller than our estimates based on a previous approach without the benefit of CEMS data. The results imply that online measurement with proper data screening can better track the recent progress of emission controls. The emission intensity (the ratio of emissions to economic output) of Northwest China was larger than that of other regions, attributed mainly to its less intensive economy and industry. Transmission of electricity to more-developed eastern provinces raised the energy consumption and emissions of less-developed regions. Judged by 95 percentiles of flue-gas concentrations measured by CEMS, most power plants met the current national emission standards in 2015 except for those in Northwest and Northeast China, while plants that met the ultra-low emission policy were much scarcer. National SO2, NOx and PM emissions would further decline by 68%, 55% and 81% respectively if the ultra-low emission policy can be strictly implemented, implying the great potential of the policy for emission abatement.


Subject(s)
Air Pollutants/analysis , Air Pollution/prevention & control , Coal , Environmental Monitoring/methods , Power Plants/legislation & jurisprudence , Air Pollution/legislation & jurisprudence , China , Industry , Nitrogen Oxides/analysis , Particulate Matter/analysis , Power Plants/standards , Sulfur Dioxide/analysis
13.
Proc Natl Acad Sci U S A ; 116(17): 8206-8213, 2019 04 23.
Article in English | MEDLINE | ID: mdl-30962380

ABSTRACT

Realizing the goal of the Paris Agreement to limit global warming to 2 °C by the end of this century will most likely require deployment of carbon-negative technologies. It is particularly important that China, as the world's top carbon emitter, avoids being locked into carbon-intensive, coal-fired power-generation technologies and undertakes a smooth transition from high- to negative-carbon electricity production. We focus here on deploying a combination of coal and biomass energy to produce electricity in China using an integrated gasification cycle system combined with carbon capture and storage (CBECCS). Such a system will also reduce air pollutant emissions, thus contributing to China's near-term goal of improving air quality. We evaluate the bus-bar electricity-generation prices for CBECCS with mixing ratios of crop residues varying from 0 to 100%, as well as associated costs for carbon mitigation and cobenefits for air quality. We find that CBECCS systems employing a crop residue ratio of 35% could produce electricity with net-zero life-cycle emissions of greenhouse gases, with a levelized cost of electricity of no more than 9.2 US cents per kilowatt hour. A carbon price of approximately $52.0 per ton would make CBECCS cost-competitive with pulverized coal power plants. Therefore, our results provide critical insights for designing a CBECCS strategy in China to harness near-term air-quality cobenefits while laying the foundation for achieving negative carbon emissions in the long run.

14.
Environ Int ; 121(Pt 1): 250-259, 2018 12.
Article in English | MEDLINE | ID: mdl-30223201

ABSTRACT

Emissions from power plants in China and India contain a myriad of fine particulate matter (PM2.5, PM ≤ 2.5 µm in diameter) precursors, posing significant health risks among large, densely settled populations. Studies isolating the contributions of various source classes and geographic regions are limited in China and India, but such information could be helpful for policy makers attempting to identify efficient mitigation strategies. We quantified the impact of power generation emissions on annual mean PM2.5 concentrations using the state-of-the-art atmospheric chemistry model WRF-Chem (Weather Research Forecasting model coupled with Chemistry) in China and India. Evaluations using nationwide surface measurements show the model performs reasonably well. We calculated province-specific annual changes in mortality and life expectancy due to power generation emissions generated PM2.5 using the Integrated Exposure Response (IER) model, recently updated IER parameters from Global Burden of Disease (GBD) 2015, population data, and the World Health Organization (WHO) life tables for China and India. We estimate that 15 million (95% Confidence Interval (CI): 10 to 21 million) years of life lost can be avoided in China each year and 11 million (95% CI: 7 to 15 million) in India by eliminating power generation emissions. Priorities in upgrading existing power generating technologies should be given to Shandong, Henan, and Sichuan provinces in China, and Uttar Pradesh state in India due to their dominant contributions to the current health risks.


Subject(s)
Air Pollutants/analysis , Models, Theoretical , Particulate Matter/analysis , Power Plants , Air Pollution/analysis , China , Environmental Monitoring , Forecasting , Humans , India , Mortality, Premature
15.
Nat Commun ; 8(1): 738, 2017 09 29.
Article in English | MEDLINE | ID: mdl-28963511

ABSTRACT

Recent studies show that international trade affects global distributions of air pollution and public health. Domestic interprovincial trade has similar effects within countries, but has not been comprehensively investigated previously. Here we link four models to evaluate the effects of both international exports and interprovincial trade on PM2.5 pollution and public health across China. We show that 50-60% of China's air pollutant emissions in 2007 were associated with goods and services consumed outside of the provinces where they were produced. Of an estimated 1.10 million premature deaths caused by PM2.5 pollution throughout China, nearly 19% (208,500 deaths) are attributable to international exports. In contrast, interprovincial trade leads to improved air quality in developed coastal provinces with a net effect of 78,500 avoided deaths nationwide. However, both international export and interprovincial trade exacerbate the health burdens of air pollution in China's less developed interior provinces. Our results reveal trade to be a critical but largely overlooked consideration in effective regional air quality planning for China.International and domestic interprovincial trade of China are entangled, but their health impacts have been treated separately in earlier studies. Here Wang. quantify the complex impacts of trade on public health across China within an integrative framework.


Subject(s)
Air Pollution , Commerce , Mortality, Premature , Public Health , China , Humans , Particulate Matter
16.
Environ Int ; 97: 180-186, 2016 Dec.
Article in English | MEDLINE | ID: mdl-27614532

ABSTRACT

With rapid economic growth, China has witnessed increasingly frequent and severe haze and smog episodes over the past decade, posing serious health impacts to the Chinese population, especially those in densely populated city clusters. Quantification of the spatial and temporal variation of health impacts attributable to ambient fine particulate matter (PM2.5) has important implications for China's policies on air pollution control. In this study, we evaluated the spatial distribution of premature deaths in China between 2000 and 2010 attributable to ambient PM2.5 in accord with the Global Burden of Disease based on a high resolution population density map of China, satellite retrieved PM2.5 concentrations, and provincial health data. Our results suggest that China's anthropogenic ambient PM2.5 led to 1,255,400 premature deaths in 2010, 42% higher than the level in 2000. Besides increased PM2.5 concentration, rapid urbanization has attracted large population migration into the more developed eastern coastal urban areas, intensifying the overall health impact. In addition, our analysis implies that health burdens were exacerbated in some developing inner provinces with high population density (e.g. Henan, Anhui, Sichuan) because of the relocation of more polluting and resource-intensive industries into these regions. In order to avoid such national level environmental inequities, China's regulations on PM2.5 should not be loosened in inner provinces. Furthermore policies should create incentive mechanisms that can promote transfer of advanced production and emissions control technologies from the coastal regions to the interior regions.


Subject(s)
Air Pollutants/toxicity , Mortality, Premature/trends , Particulate Matter/toxicity , China/epidemiology , Cities , Environmental Pollution/adverse effects , Humans , Urbanization
17.
Environ Sci Technol ; 48(3): 2016-24, 2014.
Article in English | MEDLINE | ID: mdl-24383490

ABSTRACT

Demands for electricity and energy to supply heat are expected to expand by 71% and 47%, respectively, for Beijing in 2020 relative to 2009. If the additional electricity and heat are supplied solely by coal as is the current situation, annual emissions of CO2 may be expected to increase by 59.6% or 99 million tons over this interval. Assessed against this business as usual (BAU) background, the present study indicates that significant reductions in emissions could be realized using wind-generated electricity to provide a source of heat, employed either with heat pumps or with electric thermal storage (ETS) devices. Relative to BAU, reductions in CO2 with heat pumps assuming 20% wind penetration could be as large as 48.5% and could be obtained at a cost for abatement of as little as $15.6 per ton of avoided CO2. Even greater reductions, 64.5%, could be realized at a wind penetration level of 40% but at a higher cost, $29.4 per ton. Costs for reduction of CO2 using ETS systems are significantly higher, reflecting the relatively low efficiency for conversion of coal to power to heat.


Subject(s)
Air Pollution/prevention & control , Electricity , Heating , Wind , Carbon Dioxide , China , Cities , Coal , Hot Temperature , Models, Theoretical , Power Plants , Renewable Energy/economics
18.
Environ Sci Technol ; 46(14): 7882-9, 2012 Jul 17.
Article in English | MEDLINE | ID: mdl-22724530

ABSTRACT

Emissions of sulfur dioxide (SO(2)) from the U.S. power sector decreased by 24% in 2009 relative to 2008. The Logarithmic Mean Divisia Index (LMDI) approach was applied to isolate the factors responsible for this decrease. It is concluded that 15% of the decrease can be attributed to the drop in demand for electricity triggered by the economic recession, and 28% can be attributed to switching of fuel from coal to gas responding to the decrease in prices for the latter. The largest factor in the decrease, close to 57%, resulted from an overall decline in emissions per unit of power generated from coal. This is attributed in part to selective idling of older, less efficient coal plants that generally do not incorporate technology for sulfur removal, and in part to continued investments by the power sector in removal equipment in response to the requirements limiting emissions imposed by the U.S. Environmental Protection Agency (U.S. EPA). The paper argues further that imposition of a modest tax on emissions of carbon would have ancillary benefits in terms of emissions of SO(2).


Subject(s)
Air Pollutants/analysis , Air Pollution/economics , Air Pollution/prevention & control , Natural Gas/economics , Power Plants/economics , Sulfur Dioxide/analysis , Carbon/economics , Coal/economics , Electricity , Sulfur/analysis , Taxes/economics , United States
19.
Sci Total Environ ; 409(24): 5177-87, 2011 Nov 15.
Article in English | MEDLINE | ID: mdl-21944199

ABSTRACT

Policies to control emissions of criteria pollutants in China may have conflicting impacts on public health, soil acidification, and climate. Two scenarios for 2020, a base case without anticipated control measures and a more realistic case including such controls, are evaluated to quantify the effects of the policies on emissions and resulting environmental outcomes. Large benefits to public health can be expected from the controls, attributed mainly to reduced emissions of primary PM and gaseous PM precursors, and thus lower ambient concentrations of PM2.5. Approximately 4% of all-cause mortality in the country can be avoided (95% confidence interval: 1-7%), particularly in eastern and north-central China, regions with large population densities and high levels of PM2.5. Surface ozone levels, however, are estimated to increase in parts of those regions, despite NOX reductions. This implies VOC-limited conditions. Even with significant reduction of SO2 and NOX emissions, the controls will not significantly mitigate risks of soil acidification, judged by the exceedance levels of critical load (CL). This is due to the decrease in primary PM emissions, with the consequent reduction in deposition of alkaline base cations. Compared to 2005, even larger CL exceedances are found for both scenarios in 2020, implying that PM control may negate any recovery from soil acidification due to SO2 reductions. Noting large uncertainties, current polices to control emissions of criteria pollutants in China will not reduce climate warming, since controlling SO2 emissions also reduces reflective secondary aerosols. Black carbon emission is an important source of uncertainty concerning the effects of Chinese control policies on global temperature change. Given these conflicts, greater consideration should be paid to reconciling varied environmental objectives, and emission control strategies should target not only criteria pollutants but also species such as VOCs and CO2.


Subject(s)
Air Pollutants/analysis , Air Pollutants/chemistry , Air Pollution/prevention & control , Acids/chemistry , China , Computer Simulation , Environmental Policy , Government Regulation , Models, Chemical , Models, Theoretical , Nitrogen Oxides/analysis , Nitrogen Oxides/chemistry , Particulate Matter/analysis , Particulate Matter/chemistry , Public Health , Soil/chemistry , Sulfur Dioxide/analysis , Sulfur Dioxide/chemistry , Temperature
20.
Environ Pollut ; 159(10): 2726-32, 2011 Oct.
Article in English | MEDLINE | ID: mdl-21676509

ABSTRACT

China's strategies to control acidifying pollutants and particulate matter (PM) may be in conflict for soil acidification abatement. Acidifying pollutant emissions are estimated for 2005 and 2020 with anticipated control policies. PM emissions including base cations (BCs) are evaluated with two scenarios, a base case applying existing policy to 2020, and a control case including anticipated tightened measures. Depositions of sulfur (S), nitrogen (N) and BCs are simulated and their acidification risks are evaluated with critical load (CL). In 2005, the area exceeding CL covered 15.6% of mainland China, with total exceedance of 2.2 Mt S. These values decrease in the base scenario 2020, implying partial recovery from acidification. Under more realistic PM control, the respective estimates are 17.9% and 2.4 Mt S, indicating increased acidification risks due to abatement of acid-neutralizing BCs. China's anthropogenic PM abatement will have potentially stronger chemical implications for acidification than developed countries.


Subject(s)
Air Pollution/prevention & control , Particulate Matter/analysis , Soil/chemistry , Air Pollution/legislation & jurisprudence , Air Pollution/statistics & numerical data , China , Environmental Monitoring , Environmental Policy , Hydrogen-Ion Concentration , Nitrogen/analysis , Sulfur/analysis
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