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1.
Sci Rep ; 14(1): 15504, 2024 Jul 05.
Article in English | MEDLINE | ID: mdl-38969719

ABSTRACT

Time-resolved X-ray magnetic circular dichroism under the effects of ferromagnetic resonance (FMR), known as X-ray ferromagnetic resonance (XFMR) measurements, enables direct detection of precession dynamics of magnetic moment. Here we demonstrated XFMR measurements and Bayesian analyses as a quantitative probe for the precession of spin and orbital magnetic moments under the FMR effect. Magnetization precessions in two different Pt/Ni-Fe thin film samples were directly detected. Furthermore, the ratio of dynamical spin and orbital magnetic moments was evaluated quantitatively by Bayesian analyses for XFMR energy spectra around the Ni L 2 , 3 absorption edges. Our study paves the way for a microscopic investigation of the contribution of the orbital magnetic moment to magnetization dynamics.

2.
Nat Commun ; 15(1): 1999, 2024 Mar 07.
Article in English | MEDLINE | ID: mdl-38453940

ABSTRACT

Helimagnetic structures, in which the magnetic moments are spirally ordered, host an internal degree of freedom called chirality corresponding to the handedness of the helix. The chirality seems quite robust against disturbances and is therefore promising for next-generation magnetic memory. While the chirality control was recently achieved by the magnetic field sweep with the application of an electric current at low temperature in a conducting helimagnet, problems such as low working temperature and cumbersome control and detection methods have to be solved in practical applications. Here we show chirality switching by electric current pulses at room temperature in a thin-film MnAu2 helimagnetic conductor. Moreover, we have succeeded in detecting the chirality at zero magnetic fields by means of simple transverse resistance measurement utilizing the spin Berry phase in a bilayer device composed of MnAu2 and a spin Hall material Pt. These results may pave the way to helimagnet-based spintronics.

3.
Sci Adv ; 6(40)2020 Sep.
Article in English | MEDLINE | ID: mdl-32998887

ABSTRACT

Breaking of spatial inversion symmetry induces unique phenomena in condensed matter. In particular, by combining this symmetry with magnetic fields or another type of time-reversal symmetry breaking, noncentrosymmetric materials can be made to exhibit nonreciprocal responses, which are responses that differ for rightward and leftward stimuli. However, the effect of spatial inversion symmetry breaking on thermal transport in uniform media remains to be elucidated. Here, we show nonreciprocal thermal transport in the multiferroic helimagnet TbMnO3 The longitudinal thermal conductivity depends on whether the thermal current is parallel or antiparallel to the vector product of the electric polarization and magnetization. This phenomenon is thermal rectification that is controllable with external fields in a uniform crystal. This discovery may pave the way to thermal diodes with controllability and scalability.

4.
Phys Rev Lett ; 119(1): 017201, 2017 Jul 07.
Article in English | MEDLINE | ID: mdl-28731738

ABSTRACT

We investigate the magnetic dynamics in the spinel-type vanadium oxide MnV_{2}O_{4}. Inelastic neutron scattering around 10 meV and a Heisenberg model analysis have revealed that V^{3+} spin-wave modes exist at a lower-energy region than previously reported. The scattering around 20 meV cannot be reproduced with the spin-wave analysis. We propose that this scattering could originate from the spin-orbital coupled excitation. This scattering is most likely attributable to V^{3+} spin-wave modes, entangled with the orbital hybridization between t_{2g} orbitals.

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