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1.
ACS Mater Lett ; 3(12): 1826-1831, 2021 Dec 06.
Article in English | MEDLINE | ID: mdl-34901872

ABSTRACT

Graphene oxide (GO) is widely used as a component in thin film optoelectronic device structures for practical reasons because its electronic and optical properties can be controlled. Progress critically depends on elucidating the nanoscale electronic structure of GO. However, direct experimental access is challenging because of its disordered and nonconductive character. Here, we quantitatively mapped the nanoscopic charge distribution and charge dynamics of an individual GO sheet by using Kelvin probe force microscopy (KPFM). Charge domains are identified, presenting important charge interactions below distances of 20 nm. Charge dynamics with very long relaxation times of at least several hours and a logarithmic decay of the time correlation function are in excellent agreement with Monte Carlo simulations, revealing an universal hopping transport mechanism best described by Efros-Shklovskii's law.

2.
Sci Rep ; 8(1): 15460, 2018 Oct 18.
Article in English | MEDLINE | ID: mdl-30337558

ABSTRACT

Proliferation of topological defects like vortices and dislocations plays a key role in the physics of systems with long-range order, particularly, superconductivity and superfluidity in thin films, plasticity of solids, and melting of atomic monolayers. Topological defects are characterized by their topological charge reflecting fundamental symmetries and conservation laws of the system. Conservation of topological charge manifests itself in extreme stability of static topological defects because destruction of a single defect requires overcoming a huge energy barrier proportional to the system size. However, the stability of driven topological defects remains largely unexplored. Here we address this issue and investigate numerically a dynamic instability of moving vortices in planar arrays of Josephson junctions. We show that a single vortex driven by sufficiently strong current becomes unstable and destroys superconductivity by triggering a chain reaction of self-replicating vortex-antivortex pairs forming linear of branching expanding patterns. This process can be described in terms of propagating phase cracks in long-range order with far-reaching implications for dynamic systems of interacting spins and atoms hosting magnetic vortices and dislocations.

3.
Sci Rep ; 6: 21647, 2016 Feb 25.
Article in English | MEDLINE | ID: mdl-26911652

ABSTRACT

The surface potential of conducting polymers has been studied with scanning Kelvin probe microscopy. The results show that this technique can become an excellent tool to really 'see' interesting surface charge interaction effects at the nanoscale. The electron glass model, which assumes that charges are localized by the disorder and that interactions between them are relevant, is employed to understand the complex behavior of conducting polymers. At equilibrium, we find surface potential domains with a typical lateral size of 50 nm, basically uncorrelated with the topography and strongly fluctuating in time. These fluctuations are about three times larger than thermal energy. The charge dynamics is characterized by an exponentially broad time distribution. When the conducting polymers are excited with light the surface potential relaxes logarithmically with time, as usually observed in electron glasses. In addition, the relaxation for different illumination times can be scaled within the full aging model.

4.
Phys Rev Lett ; 116(1): 010404, 2016 Jan 08.
Article in English | MEDLINE | ID: mdl-26799005

ABSTRACT

Recently, it has been suggested that the many-body localized phase can be characterized by local integrals of motion. Here we introduce a Hilbert-space-preserving renormalization scheme that iteratively finds such integrals of motion exactly. Our method is based on the consecutive action of a similarity transformation using displacement operators. We show, as a proof of principle, localization and the delocalization transition in interacting fermion chains with random on-site potentials. Our scheme of consecutive displacement transformations can be used to study many-body localization in any dimension, as well as disorder-free Hamiltonians.

5.
Phys Rev Lett ; 102(21): 216601, 2009 May 29.
Article in English | MEDLINE | ID: mdl-19519122

ABSTRACT

Motivated by anomalously large conductivity anisotropy in layered materials, we propose a simple model of randomly spaced potential barriers (mimicking stacking faults) with isotropic impurities in between the barriers. We solve this model both numerically and analytically by utilizing an exact solution for the conductivity of a one-dimensional disordered system. In the absence of bulk disorder, electron motion in the out-of-plane direction is localized. Bulk disorder destroys one-dimensional localization. As a result, the out-of-plane conductivity is finite and scales linearly with the scattering rate by bulk impurities until planar and bulk disorder become comparable. The ac out-of-plane conductivity is of a manifestly non-Drude form: the real part starts from finite value at zero frequency and has a maximum at the frequency corresponding to the scattering rate by potential barriers.

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