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1.
ACS Appl Mater Interfaces ; 13(17): 20788-20795, 2021 May 05.
Article in English | MEDLINE | ID: mdl-33877796

ABSTRACT

All-oxide-based synthetic antiferromagnets (SAFs) are attracting intense research interest due to their superior tunability and great potentials for antiferromagnetic spintronic devices. In this work, using the La2/3Ca1/3MnO3/CaRu1/2Ti1/2O3 (LCMO/CRTO) superlattice as a model SAF, we investigated the layer-resolved magnetic reversal mechanism by polarized neutron reflectivity. We found that the reversal of LCMO layer moments is mediated by nucleation, expansion, and shrinkage of a magnetic soliton. This unique magnetic reversal process creates a reversed magnetic configuration of the SAF after a simple field cycling. Therefore, it can enable vertical data transfer from the bottom to the top of the superlattice. The physical origin of this intriguing magnetic reversal process could be attributed to the cooperation of the surface spin-flop effect and enhanced uniaxial magnetic anisotropy of the bottom LCMO layer. This work may pave a way to utilize all-oxide-based SAFs for three-dimensional spintronic devices with vertical data transfer and high-density data storage.

2.
Beilstein J Nanotechnol ; 11: 1254-1263, 2020.
Article in English | MEDLINE | ID: mdl-32874825

ABSTRACT

We have investigated the structural, magnetic and superconduction properties of [Nb(1.5 nm)/Fe(x)]10 superlattices deposited on a thick Nb(50 nm) layer. Our investigation showed that the Nb(50 nm) layer grows epitaxially at 800 °C on the Al2O3(1-102) substrate. Samples grown at this condition possess a high residual resistivity ratio of 15-20. By using neutron reflectometry we show that Fe/Nb superlattices with x < 4 nm form a depth-modulated FeNb alloy with concentration of iron varying between 60% and 90%. This alloy has weak ferromagnetic properties. The proximity of this weak ferromagnetic layer to a thick superconductor leads to an intermediate phase that is characterized by a suppressed but still finite resistance of structure in a temperature interval of about 1 K below the superconducting transition of thick Nb. By increasing the thickness of the Fe layer to x = 4 nm the intermediate phase disappears. We attribute the intermediate state to proximity induced non-homogeneous superconductivity in the structure.

3.
Small ; 3(5): 880-9, 2007 May.
Article in English | MEDLINE | ID: mdl-17410621

ABSTRACT

In this work, we present the size-controlled preparation of silica-filled micelle cores and their self-assembly behavior, which is dependent on the block lengths, different coating techniques, and substrates. Furthermore, we present a way to use these structures as templates for highly ordered magnetic nanostructures, revealed by Ar-ion milling. The resulting structures were characterized by different imaging and scattering techniques and model simulations were performed. The characterization of the obtained nanostructured surfaces has be performed with atomic force microscopy, by scanning electron microscopy, grazing-incidence X-ray small-angle scattering, and X-ray reflectivity measurements. The magneto-optical Kerr effect was utilized to investigate magnetic properties.


Subject(s)
Colloids/chemistry , Crystallization/methods , Nanostructures/chemistry , Nanostructures/ultrastructure , Nanotechnology/methods , Polymers/chemistry , Silicon Dioxide/chemistry , Macromolecular Substances/chemistry , Materials Testing , Micelles , Molecular Conformation , Particle Size , Surface Properties
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