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1.
Environ Geochem Health ; 40(1): 295-301, 2018 Feb.
Article in English | MEDLINE | ID: mdl-27995354

ABSTRACT

A total of 60 children (31 males and 29 females) between the ages of 3 and 12 years were randomly selected from Lanzhou City in Gansu Province, northwest China. Hand (soil/dust) SD samples from these children were collected using hand wipes. We determined the approximate amounts of hand SD and the concentrations of three tracer soil elements (Ce, Y, and V) in these samples. The approximate amounts of hand SD ranged from 42.28 to 173.76 mg, with a median value of 85.42 mg. In addition, the mean amounts of hand SD estimated using the concentrations of Ce, Y, and V in the samples were 4.63, 3.43, and 3.42 mg, respectively. The amount of hand SD varied greatly among the age groups: primary school children had more hand SD than kindergarten children, males had more hand SD than females, and children from rural areas had more hand SD than those from urban areas. The rates of daily ingestion of hand SD for kindergarten and primary school children were estimated to be 7.73 and 6.61 mg/day, respectively.


Subject(s)
Cerium/analysis , Dust , Eating , Hand , Mouth , Soil , Vanadium/analysis , Yttrium/analysis , Child , Child, Preschool , China , Dust/analysis , Female , Humans , Male , Mass Spectrometry/methods , Sex Factors , Soil/chemistry
2.
Chemosphere ; 163: 578-583, 2016 Nov.
Article in English | MEDLINE | ID: mdl-27567157

ABSTRACT

We collected and analyzed 128 surface soil samples from Xiangfen County for dichlorodiphenyltrichloroethane (DDT), dichlorodiphenyldichloroethane (DDD), and dichlorodiphenyldichloroethylene (DDE). Total DDT concentrations (DDTs; sum of p,p'-DDD, p,p'-DDE, and p,p'-DDT) ranged from ND to 427.81 ng g(-1) (dry weight, dw), with a mean of 40.26 ng g(-1) (dw). Among the three compounds, p,p'-DDD was the most dominant. The DDTs in Xiangfen County soils mainly originated from historical DDT use, but there were also new inputs likely related to dicofol use. The DDTs in Xiangfen County soils were mainly degraded under anaerobic conditions, and direct degradation to DDD was the main degradation route. Regions with relatively high concentrations of DDTs were mainly located in North and South Xiangfen County. In these regions, many soil samples contained p,p'-DDT as the predominant pollutant, suggestive of extensive new inputs of DDT. A health risk assessment revealed that there are no serious long-term health impacts of exposure to DDTs in soil, for adults or children.


Subject(s)
DDT/analysis , Dichlorodiphenyl Dichloroethylene/analysis , Dichlorodiphenyldichloroethane/analysis , Neoplasms/chemically induced , Soil Pollutants/analysis , Adult , Child , China , DDT/adverse effects , Dichlorodiphenyl Dichloroethylene/adverse effects , Dichlorodiphenyldichloroethane/adverse effects , Environmental Monitoring , Humans , Insecticides/adverse effects , Insecticides/analysis , Risk Assessment , Risk Factors , Soil/chemistry , Soil Pollutants/adverse effects
3.
Chemosphere ; 148: 248-54, 2016 Apr.
Article in English | MEDLINE | ID: mdl-26807946

ABSTRACT

The concentrations of As, Cd, Cr, Cu, Pb, Ni, Zn, and Hg in 128 surface soil samples from Xiangfen County, Shanxi Province, China were measured. The concentrations of these eight heavy metals were lower than the critical values in the national soil quality standard. However, these concentrations were found to be slightly higher than their background values in soils in Shanxi Province, indicating enrichment of these metals in soils in Xiangfen County, especially for Hg and Cd. Principal component analysis coupled with cluster analysis was used to analyze the data and identify possible sources of these heavy metals; the results showed that the eight heavy metals in soils from Xiangfen County came from three different sources. Lead, Cd, Cu and Zn mainly arose from agricultural practices and vehicle emissions. Arsenic and Ni arose mainly from parent materials. Industrial practices were the main sources of Cr and Hg. The spatial distribution of the heavy metals varied greatly, and was closely correlated to local anthropogenic activities. This study will be helpful not only for improving local soil environmental quality but will also provide a basis for effectively targeting policies to protect soils from long-term heavy metal accumulation.


Subject(s)
Agriculture , Environmental Monitoring/methods , Metals, Heavy/analysis , Soil Pollutants/analysis , Soil/chemistry , China , Cluster Analysis , Principal Component Analysis , Soil/standards , Spatial Analysis
4.
Huan Jing Ke Xue ; 35(3): 853-63, 2014 Mar.
Article in Chinese | MEDLINE | ID: mdl-24881370

ABSTRACT

The emission inventory of air pollutants from the thermal power plants in the year of 2010 was set up. Based on the inventory, the air quality of the prediction scenarios by implementation of both 2003-version emission standard and the new emission standard were simulated using Models-3/CMAQ. The concentrations of NO2, SO2, and PM2.5, and the deposition of nitrogen and sulfur in the year of 2015 and 2020 were predicted to investigate the regional air quality improvement by the new emission standard. The results showed that the new emission standard could effectively improve the air quality in China. Compared with the implementation results of the 2003-version emission standard, by 2015 and 2020, the area with NO2 concentration higher than the emission standard would be reduced by 53.9% and 55.2%, the area with SO2 concentration higher than the emission standard would be reduced by 40.0%, the area with nitrogen deposition higher than 1.0 t x km(-2) would be reduced by 75.4% and 77.9%, and the area with sulfur deposition higher than 1.6 t x km(-2) would be reduced by 37.1% and 34.3%, respectively.


Subject(s)
Air Pollutants/standards , Models, Theoretical , Power Plants/standards , Air Pollution/analysis , China , Nitric Oxide/analysis , Particulate Matter/analysis , Sulfur Dioxide/analysis
5.
Huan Jing Ke Xue ; 35(12): 4446-53, 2014 Dec.
Article in Chinese | MEDLINE | ID: mdl-25826912

ABSTRACT

Ozone concentrations obtained from 35 automatic air monitoring stations in Beijing were analyzed to investigate their temporal and spatial distribution characteristics. A process with high ozone concentration in summer was analyzed. The results showed that ozone maintained relatively high concentration from May to August while in other months, the ozone concentration was at a low level. Overall, the average concentrations of ozone in different stations in a descending order were comparison and regional station, suburban environment evaluation station, urban environmental assessment station and traffic pollution monitoring station. Ozone diurnal variation showed a single peak distribution, the peak of which appeared at 15:00 or 16:00. Ozone concentration showed obvious weekend effect, which meant ozone concentration in daytime of weekend was higher than that in weekday. Ozone concentration was lower in urban Beijing, higher in surrounding counties and the highest in northeast area with more vegetation. A high ozone concentration process occurred in Beijing on June 3, 2013. Under the effect of southwest wind in the afternoon, the concentration peaks of ozone in Yufa, Fengtaihuayuan, Olympic center and Huairou station occurred in order from south to north. Concentration peak of ozone in Huairou station occurred at 20:00 in the night. It could be concluded that significant ozone transmission characteristic was reflected in this process.


Subject(s)
Air Pollutants/analysis , Environmental Monitoring , Ozone/analysis , China , Cities , Seasons , Wind
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