Verification of the sampling procedure for radioactivity analysis of waste and industrial material.

In accordance with ISO/IEC 17025:2017, the testing laboratory needs to verify its ability to properly perform methods. For radiological testing, the sampling does not affect the results directly, but it has to ensure that sample adequately represents the tested material. To verify the procedure, a sampling of red mud and bauxite ore was conducted. All samples were measured in identical geometry by HPGe spectrometer. The counting rates per unit mass in the recorded spectra were compared. For each measurement series, the mean and standard deviations of respected peaks were calculated, as well as average and standard deviation of all series. The obtained results of each individual series were considered satisfactory, i.e. sampling procedure ensures the representativeness of the bulk material, if it is within ± two standard deviations of the average of the mean values.

Outdoor Radon as a Tool to Estimate Radon Priority Areas-A Literature Overview.

Doses from the exposure to outdoor radon are typically an order of magnitude smaller than those from indoor radon, causing a greater interest on investigation of the latter for radiation protection issues. As a consequence, assessment of radon priority areas (RPA) is mainly based on indoor radon measurements. Outdoor radon measurements might be needed to guarantee a complete estimation of radiological risk and may help to improve the estimation of RPA. Therefore, authors have analysed the available literature on outdoor radon to give an overview of outdoor radon surveys and potential correlation with indoor radon and estimation of RPA. The review has shown that outdoor radon surveys were performed at much smaller scale compared to indoor radon. Only a few outdoor radon maps were produced, with a much smaller density, covering a larger area, and therefore putting doubt on the representativeness of this data. Due to a large variety of techniques used for outdoor radon measurements and requirement to have detectors with a high sensitivity and resistance to harsh environmental conditions, a standardised measurement protocol should be derived. This is no simple endeavour since there are more applications in different scientific disciplines for outdoor radon measurements compared to indoor radon.

Radon measurements using open-faced charcoal canisters - Measurement uncertainty and method optimization.

Open-faced charcoal canisters have been used for radon measurements for over 40 years. This method is sensitive to temperature, changing radon concentrations, humidity and other parameters, but a comprehensive study dealing with the influence quantities and measurement uncertainty was not available in literature. In this paper, all the identified influence quantities are discussed in detail, uncertainty budget is developed, good practice and bad practice examples are introduced and new recommendations are proposed to optimize the method and reduce uncertainty.

Results of the first national indoor radon survey performed in Serbia.

The first step in every systematic approach to investigating population exposure to radon on a national level is to perform a comprehensive indoor radon survey. Based on general knowledge of the radon levels in Serbia and corresponding doses, the results obtained from a national indoor radon survey would allow policymakers to decide whether it is necessary to establish a national radon programme. For this reason, Serbia initiated work on a national radon action plan (RAP) in 2014 when it was decided to carry out the first national indoor radon survey. The responsibility for establishing the RAP in Serbia is that of the national regulatory body in the field of radiation protection-the Serbian Radiation and Nuclear Safety and Security Directorate (SRBATOM), formerly known as the Serbian Radiation Protection and Nuclear Safety Agency. The first national indoor radon survey was supported by the International Atomic Energy Agency (IAEA) through a Technical Cooperation Programme. Thanks to the IAEA, we received 6000 passive radon devices based on track-etched detectors. In addition, in order to ensure technical support for the project, SRBATOM formed a task force made up of expert radon representatives from national research institutions. This paper presents a thorough description of the sampling design of the first Serbian indoor radon survey. It also presents the results of the national indoor radon survey, including descriptive statistics and testing of the distribution of the obtained results for log-normality. Based on GPS coordinates, indoor radon data were projected onto a map of 10 km × 10 km grid cells. Two values were calculated for each cell to create two distinct maps. One map shows the arithmetic mean value of indoor radon concentration per grid cell, and the other map shows the number of radon detectors per grid cell used for the calculation of mean values.

Qualitative overview of indoor radon surveys in Europe.

The revised European Directive from 2013 regarding basic safety standard oblige EU Member States to establish a national action plan regarding the exposure to radon. At the same time, International Atomic Energy Agency started technical projects in order to assist countries to establish and implement national radon action. As a consequence, in recent years, in numerous countries national radon surveys were conducted and action plans established, which were not performed before. In this paper, a qualitative overview of radon surveys performed in Europe is given with a special attention to the qualitative and conceptual description of surveys, representativeness and QA/QC (quality assurance/quality control).

Natural radionuclides in waste water discharged from coal-fired power plants in Serbia.

Investigation of the natural radioactivity levels in water around power plants, as well as in plants, coal, ash, slag and soil, and to assess the associated radiation hazard is becoming an emerging and interesting topic. This paper is focused on the results of the radioactivity analysis in waste water samples from five coal-fired power plants in Serbia (Nikola Tesla A, Nikola Tesla B, Kolubara, Morava and Kostolac), which were analyzed in the period 2003-2015. River water samples taken upstream and downstream from the power plants, drain water and overflow water were analyzed. In the water samples gamma spectrometry analysis was performed as well as determination of gross alpha and beta activity. Natural radionuclide 40K was detected by gamma spectrometry, while the concentrations of other radionuclides, 226Ra, 235U and 238U, usually were below the minimum detection activity (MDA). 232Th and artificial radionuclide 137Cs were not detected in these samples. Gross alpha and beta activities were determined by the α/ß low level proportional counter Thermo Eberline FHT 770 T. In the analyzed samples, gross alpha activity ranged from MDA to 0.47 Bq L-1, while the gross beta activity ranged from MDA to 1.55 Bq L-1.

137Cs and 40K in some traditional herbal teas collected in the mountain regions of Serbia.

Herbal teas are an important part of traditional medicine in Serbia. The objective of the present study was to determine the activity concentrations of (40)K and (137)Cs in herbal tea, using the gamma spectroscopy method. The samples were collected during the period 2011-2012 in three mountain regions in Western and Central Serbia. The activity concentrations of (40)K and (137)Cs were found to be in the range of 130-1160 and 0.7-124 Bq kg(-1), respectively. The average annual effective dose equivalents from ingestion of (40)K and (137)Cs for an adult person consuming one cup of herbal tea daily were found to be 588.4-5250.2 nSv for (40)K and 4.0-706.1 nSv for (137)Cs. Our investigation showed that the herbal teas originating from Maljen, Zlatibor and Tara mountains are radiologically safe for human consumption.

Comparative study of (137)Cs distribution in broilers and pheasants and possibilities for protection.

The aim of the present study was to investigate distribution of (137)Cs in leg and breast meat of broilers and pheasants following single alimentary contamination and administration of two protectors (AFCF and clinoptilolite). The birds were administered a single dose of (137)CsCl, with an activity of 750 Bq. Protectors were given via gastric tube or mixed in the forage pellets. AFCF given via gastric tube decreased the (137)Cs concentration by a factor of 7.8 in broilers leg meat and 7.4 in broilers breast meat. When AFCF was mixed in pellets, the (137)Cs concentration was 19.5 times lower in broilers leg meat and 22.1 times lower in broilers breast meat, than in the control group. In pheasants, AFCF administered via gastric tube decreased the (137)Cs concentration by a factor of 12.4 in leg meat and by a factor of 13.7 in breast meat, respectively. In group 4, where pheasants were administered AFCF mixed in pellets, the (137)Cs concentration was 3.7 times lower in leg and breast meat, than in the control group. For comparison, clinoptilolite administered via gastric tube decreased the (137)Cs concentration 1.8 times in broilers leg meat and 2.0 times in breast meat, compared to the control group. In pheasants, (137)Cs concentration was 2.9 times lower in leg meat and 2.6 times lower in breast meat. Clinoptilolite mixed in the feed had relatively low efficiency of protection in broilers ((137)Cs concentration was 1.4 times lower in leg meat and 1.6 lower in breast meat). A similar trend was observed in pheasants ((137)Cs concentration was 1.6 lower in leg and breast meat).

Identification of Metals (Heavy and Radioactive) in Drinking Water by an Indirect Analysis Method Based on Scale Tests.

The analysis of water quality, regarding the content of metals, especially heavy and radioactive ones, has been carried out in an indirect way, by testing scale formed in a hot-water heater, using water from the water-supply network of the city of Belgrade - the district of New Belgrade. The determination of the composition and the structure of the scale has resulted in its complete identification, and its crystallochemical formula has been defined. It has unequivocally been established that the obtained results are within the tolerance boundary with the results acquired by a conventional analysis of water, when it is a matter of very low concentrations. The presence of radioactive elements of uranium and strontium in a scale sample has been found and the way of their penetrating its composition and structure has been explained. Applying the fractional extraction method, uranium has been established to be of an anthropogenic origin.