Buried Depressed-Cladding Waveguides Inscribed in Nd3+ and Yb3+ Doped CLNGG Laser Crystals by Picosecond-Laser Beam Writing.

Buried depressed-cladding waveguides were fabricated in 0.7-at.% Nd:Ca3Li0.275Nb1.775Ga2.95O12 (Nd:CLNGG) and 7.28-at.% Yb:CLNGG disordered laser crystals grown by Czochralski method. Circular waveguides with 100 µm diameters were inscribed in both crystals with picosecond (ps) laser pulses at 532 nm of 0.15 µJ energy at 500 kHz repetition rate. A line-by-line writing technique at 1 mm/s scanning speed was used. Laser emission at 1.06 µm (with 0.35 mJ pulse energy) and at 1.03 µm (with 0.16 mJ pulse energy) was obtained from the waveguide inscribed in Nd:CLNGG and Yb:CLNGG, respectively, employing quasi-continuous wave pumping with fiber-coupled diode lasers. The waveguide realized in RE3+-doped CLNGG crystals using ps-laser pulses at high repetition rates could provide Q-switched or mode-locked miniaturized lasers for a large number of photonic applications.

LGYSB:Nd─High-Performance Lasing in the Near-Infrared Region.

Three incongruent melting LawNdxGdyYzSc4-w-x-y-z(BO3)4 (LGYSB:Nd) crystals with different Y concentrations (z = 0.15, 0.05, and 0.025) have been grown by the Czochralski method for the first time. The LGYSB:Nd-type crystals exhibit an acentric structure similar to that of the natural mineral huntite CaMg3(CO3)4, with space group R32. The composition of the LGYSB:Nd_3 (z = 0.025) crystal grown from the starting melt composition La0.628Gd0.547Y0.025Nd0.05Sc2.75(BO3)4 was measured by inductively coupled plasma mass spectrometry method, and it was found to be La0.6794Gd0.4105Y0.0178Nd0.0381Sc2.8542(BO3)4. The transversal spatial distribution of the refractive index in the LGYSB:Nd_3 crystal was investigated. Third-order nonlinear optical susceptibility χ(3) of the LGYSB:Nd_3 crystal was determined from third-harmonic generation experiments with ultrashort (fs) laser pulses. The optical transmission spectrum was measured in the range of 200-2000 nm. The absorption cross-section at 808 nm in σ-polarization was determined to be 1.18 × 10-19 cm2 for the LGYSB:Nd_3 crystal. The 10K absorption spectra revealed that the Nd3+ ions occupy only La3+ cationic sites in the LGYSB host matrix. The emission cross-section at 1064 nm in σ-polarization was determined to be σem(σ) = 1.74 × 10-19 cm2 for the LGYSB:Nd_3 crystal. The fluorescence lifetime was found to be τ = 115 µs for all of the LGYSB:Nd crystals. The LGYSB:Nd_3 laser was operated at an emission wavelength of 1062 nm with very high slope efficiencies of ηsa = 0.74 and ηsa = 0.64 in quasi-cw and cw regimes, respectively.

On the improvement by laser ignition of the performances of a passenger car gasoline engine.

Laser ignition was used to operate a four-stroke, four-cylinder, multipoint fuel injection gasoline passenger car engine, replacing the engine classical ignition device. The laser ignition system was compactly built with diode end-pumped Nd:YAG/Cr4+:YAG composite ceramics, each laser spark plug delivering pulses at 1.06 µm with 4 mJ energy and 0.8 ns duration at variable repetition rate, in accordance with the engine speed. The engine was operated at constant speed-constant load condition of 2000 rpm-2 bar equivalent brake mean effective pressure, and different ignition timings, thus simulating city traffic situations. Two relative air-fuel ratios have been considered: λ~1 for the stoichiometric mixture operation and λ~1.25 for the lean mixture condition. Parameters indicating engine performance, efficiency, combustion stability, and emissions have been measured and registered when groups of 500 consecutive cycles were acquired. The engine brake power, brake specific fuel consumption, coefficient of variability for indicated mean effective pressure, initial and main combustion stage durations, as well as exhaust emissions like carbon monoxide (CO) and total unburned hydrocarbons (THC) emphasized that significant improvements can be obtained for lean air-fuel mixture operation. Increases of the nitrogen oxides emission (NOx) were measured when laser ignition was used.

Passive Q-Switching by Cr4+:YAG Saturable Absorber of Buried Depressed-Cladding Waveguides Obtained in Nd-Doped Media by Femtosecond Laser Beam Writing.

We report on laser performances obtained in Q-switch mode operation from buried depressed-cladding waveguides of circular shape (100 µm diameter) that were inscribed in Nd:YAG and Nd:YVO4 media by direct writing with a femtosecond laser beam. The Q-switch operation was realized with a Cr4+:YAG saturable absorber, aiming to obtain laser pulses of moderate (few µJ) energy at high (tens to hundreds kHz) repetition rate. An average power of 0.52 W at 1.06 µm consisting of a train of pulses of 7.79 µJ energy at 67 kHz repetition rate, was obtained from a waveguide realized in a 4.8 mm long, 1.1-at % Nd:YAG ceramics; the pulse peak power reached 1.95 kW. A similar waveguide that was inscribed in a 3.4 mm long, 1.0-at % Nd:YVO4 crystal yielded laser pulses with 9.4 µJ energy at 83 kHz repetition rate (at 0.77 W average power) and 1.36 kW peak power. The laser performances obtained in continuous-wave operation were discussed for each waveguide used in the experiments. Thus, a continuous-wave output power of 1.45 W was obtained from the circular buried depressed-cladding waveguide inscribed in the 1.1-at %, 4.8 mm long Nd:YAG; the overall optical-to-optical efficiency, with respect to the absorbed pump power, was 0.21. The waveguide inscribed in the 1.0-at %, 3.4 mm long Nd:YVO4 crystal yielded 1.85 W power at 0.26 overall optical efficiency. This work shows the possibility to build compact laser systems with average-to-high peak power pulses based on waveguides realized by a femtosecond (fs) laser beam direct writing technique and that are pumped by a fiber-coupled diode laser.

Ignition of an automobile engine by high-peak power Nd:YAG/Cr4⁺:YAG laser-spark devices.

Laser sparks that were built with high-peak power passively Q-switched Nd:YAG/Cr(4+):YAG lasers have been used to operate a Renault automobile engine. The design of such a laser spark igniter is discussed. The Nd:YAG/Cr(4+):YAG laser delivered pulses with energy of 4 mJ and 0.8-ns duration, corresponding to pulse peak power of 5 MW. The coefficients of variability of maximum pressure (COV(Pmax)) and of indicated mean effective pressure (COV(IMEP)) and specific emissions like hydrocarbons (HC), carbon monoxide (CO), nitrogen oxides (NO(x)) and carbon dioxide (CO2) were measured at various engine speeds and high loads. Improved engine stability in terms of COV(Pmax) and COV(Pmax) and decreased emissions of CO and HC were obtained for the engine that was run by laser sparks in comparison with classical ignition by electrical spark plugs.

Diode-laser pumping into the emitting level for efficient lasing of depressed cladding waveguides realized in Nd:YVO4 by the direct femtosecond-laser writing technique.

Depressed cladding waveguides have been realized in Nd:YVO(4) employing direct writing technique with a femtosecond-laser beam. It was shown that the output performances of such laser devices are improved by the reduction of the quantum defect between the pump wavelength and the laser wavelength. Thus, under the classical pump at 808 nm (i.e. into the (4)F(5/2) level), a 100-µm diameter circular waveguide inscribed in a 0.7-at.% Nd:YVO(4) outputted 1.06-µm laser pulses with 3.0-mJ energy, at 0.30 optical efficiency and slope efficiency of 0.32. The pump at 880 nm (i.e.directly into the (4)F(3/2) emitting level) increased the pulse energy at 3.8 mJ and improved both optical efficiency and slope efficiency at 0.36 and 0.39, respectively. The same waveguide yielded continuous-wave 1.5-W output power at 1.06 µm under the pump at 880 nm. Laser emission at 1.34 µm was also improved using the pump into the (4)F(3/2) emitting level of Nd:YVO(4).

Laser emission from diode-pumped Nd:YAG ceramic waveguide lasers realized by direct femtosecond-laser writing technique.

We report on realization of buried waveguides in Nd:YAG ceramic media by direct femtosecond-laser writing technique and investigate the waveguides laser emission characteristics under the pump with fiber-coupled diode lasers. Laser pulses at 1.06 µm with energy of 2.8 mJ for the pump with pulses of 13.1-mJ energy and continuous-wave output power of 0.49 W with overall optical efficiency of 0.13 were obtained from a 100-µm diameter circular cladding waveguide realized in a 0.7-at.% Nd:YAG ceramic. A circular waveguide of 50-µm diameter yielded laser pulses at 1.3 µm with 1.2-mJ energy.

Composite, all-ceramics, high-peak power Nd:YAG/Cr(4+):YAG monolithic micro-laser with multiple-beam output for engine ignition.

A passively Q-switched Nd:YAG/Cr(4+):YAG micro-laser with three-beam output was realized. A single active laser source made of a composite, all-ceramics Nd:YAG/Cr(4+):YAG monolithic cavity was pumped by three independent lines. At 5 Hz repetition rate, each line delivered laser pulses with ~2.4 mJ energy and 2.8-MW peak power. The M(2) factor of a laser beam was 3.7, and stable air breakdowns were realized. The increase of pump repetition rate up to 100 Hz improved the laser pulse energy by 6% and required ~6% increase of the pump pulse energy. Pulse timing of the laser-array beams can by adjusted by less than 5% tuning of an individual line pump energy, and therefore simultaneous multi-point ignition is possible. This kind of laser can be used for multi-point ignition of an automobile engine.

Multipass pumped Nd-based thin-disk lasers: continuous-wave laser operation at 1.06 and 0.9 microm with intracavity frequency doubling.

The laser performances of the 1.06 microm (4)F(3/2) --> (4)I(11/2) four-level transition and of the 0.9 microm (4)F(3/2) --> I(9/2)4 quasi-three-level transition were investigated using multipass pumped Nd-based media in thin-disk geometry. When pumping at 0.81 microm into the (4)F(5/2) level, continuous-wave laser operation was obtained with powers in excess of 10 W at 1.06 microm, in the multiwatt region at 0.91 microm in Nd:YVO(4) and Nd:GdVO(4), and at 0.95 microm in Nd:YAG. Intracavity frequency-doubled Nd:YVO(4) thin-disk lasers with output powers of 6.4 W at 532 nm and of 1.6 W at 457 nm were realized at this pumping wavelength. The pumping at 0.88 microm, which is directed into the (4)F(3/2) emitting level, was also employed, and Nd:YVO(4) and Nd:GdVO(4) thin-disk lasers with ~9 W output power at 1.06 microm and visible laser radiation at 0.53 microm with output power in excess of 4 W were realized. Frequency-doubled Nd:vanadate thin-disk lasers with deep blue emission at 0.46 microm were obtained under pumping directly into the (4)F(3/2) emitting level.