ABSTRACT
This paper is devoted to reviewing the latest results achieved in solid-state lasers based on thulium-doped mixed-sesquioxide ceramics, i.e., (Lu,Sc,Y)2O3. The near- and mid-infrared regions are of interest for many applications, from medicine to remote sensing, as they match molecular fingerprints and cover several atmospheric transparency windows. These matrices are characterized by a strong electron-phonon interaction-which results in a large splitting of the ground state-and by a spectral broadening of the optical transition suitable for developing tunable and short-pulse lasers. In particular, the manuscript reports on the trivalent thulium laser transitions at 1.5, 1.9, and 2.3 µm, along with the thermal and optical characteristics of the (Lu,Sc,Y)2O3 ceramics, including the fabrication techniques, spectroscopic and optical properties, and laser performances achieved in different pumping regimes, such as continuous-wave (CW), quasi-CW, and pulsed modes. A comparison of the performance obtained with these mixed-sesquioxide ceramics and with the corresponding crystals is reported.
ABSTRACT
Samples of magnesium aluminum spinel ceramics doped with manganese ions were prepared by a high-temperature solid-state reaction method; their potential as red-emitting phosphors was analyzed using a time-resolved luminescence spectroscopy technique, from room temperature to 10 K. It was found that in the red spectral range, the luminescence spectra of manganese ions in the MgAl2O4 spinel showed a narrow band peaking at 651 nm due to the emission of Mn4+ and a broader emission band in the region of 675 ÷ 720 nm; the ratio of intensities for these bands depends on the synthesis conditions. By applying a special multi-step annealing procedure, the MgAl2O4:Mn4+ phosphor containing only tetravalent manganese ions, Mn4+, was synthesized. Broad-band far-red emission observed from MgAl2O4:Mn and Mg1.25Al1.75O3.75F0.25:Mn phosphors, prepared by a conventional method of a solid-state reaction, was interpreted as coming from Mn3+ ions.
ABSTRACT
We report a comprehensive characterization of a 10 at.% Yb3+-doped YSAG (Yb:Y3ScxAl(5-x)O12, x = 1.5) ceramic, including microstructural, spectroscopic and laser properties. Moreover, we illustrate and discuss the fabrication technique. Yb3+ in YSAG features a broader absorption and emission band than in traditional YAG, which is advantageous for laser applications (i.e., tunable laser sources, ultrafast pulse generation). Pumping in a quasi continuous wave regime at 936 nm, the ceramic has shown good laser performance as the maximum output power was 6.3 W with a corresponding slope efficiency (ηs) of 67.8%. In continuous wave regime instead, the maximum output power was 5 W with ηs = 52.7%. The laser emission wavelengths in free running were λL = 1051 nm and λL = 1031 nm, depending on the output coupler transmission. Finally, by a tunable cavity we obtained laser emission spanning from 991.5 to 1073 nm, i.e., 81.5 nm, which is the broadest tuning range ever reported for this material, to the best of our knowledge.
ABSTRACT
We report a broad comparative analysis of the spectroscopic and laser properties of solid solution Lutetium-Yttrium Aluminum Garnet (LuYAG, (LuxY1-x)3Al5O12) ceramics doped with Yb. The investigation was mainly aimed to assess the impact of the Lu/Y ratio on the Yb optical and laser properties. Therefore we analyzed a set of samples with different Y/Lu balance, namely 25/75, 50/50 and 75/25, with 15% Yb doping. We found that the Yb absorption and emission spectra changed from YAG to LuAG when gradually increasing in Lu content. Regarding the laser emission, remarkable results were achieved with all samples. Maximum output power was 8.2 W, 7.3 W and 8.7 W for Y/Lu balance 25/75, 50/50 and 75/25 respectively, at 1030 nm; the slope efficiency and the optical-to-optical efficiencies approached or exceeded 60% and 50% respectively. The tuning range was investigated using an intracavity ZnSe prism. The broadest tuning range (998 nm to 1063 nm) was obtained with Y/Lu balance 75/25, whereas the emission of the other two samples extended from 1000 nm to 1058 nm. To the best of our knowledge, this is the first comparative analysis of Yb:LuYAG ceramics or crystals as laser host across such a broad range of Y/Lu ratios.
ABSTRACT
We report the first laser oscillation on Yb0.15:(Lu0.5Y0.5)3Al12 ceramics at room temperature. At 1030 nm we measured a maximum output power of 7.3 W with a corresponding slope efficiency of 55.4% by using an output coupler with a transmission of T = 39.2%. The spectroscopic properties are compared with those of the two parent garnets Yb:YAG and Yb:LuAG. To the best of our knowledge these are the first measurements reported in literature achieved with this new host.
ABSTRACT
The laser performance of a 5% Yb doped Lu2SiO5 (Yb:LSO) has been investigated in quasi continuous-wave pumping regime along the three principal dielectric axes of the crystal, to obtain a complete characterization of its laser properties. The comparison among the obtained results for differently polarized lasers, in term of relative slope efficiency and absolute efficiency, allows the exploitability of different orientations of the material in order to be determined to obtain efficient laser sources. The laser slope efficiency and the energy conversion efficiency were similar for emission polarized along the three indicatrix axes, with noticeable maximum values of slope efficiency around 90% for polarization along the Y and Z axes. Tunable laser action has been obtained in the range 990 nm - 1084 nm, with sizeable differences in the shape of the tuning curve for polarization along the X, Y and Z axes. In particular, the tuning for polarization along the Z axis is relatively flat and uniform in the range 1023 nm - 1083 nm.
ABSTRACT
We report a rigorous study of the spectroscopic, laser and thermal properties of a 10at.% and a 15at.% Yb:LuAG crystals. A loss mechanism is observed in the medium with the highest doping, pumped at 936 nm and 968 nm, as a sharp and dramatic decrease of the laser output power is measured at higher excitation densities. The nonlinearity of the loss mechanism is confirmed by the fluorescence data and by the thermal lens. In particular, the dioptric power of the thermal lens acquired at different pumping levels shows a strong deviation of the expected linear trend. Here we report the influence of both the concentration and the ion excitation density of Yb3+ on the output powers, the slope efficiencies and the thresholds. Conversely excellent results are achieved with the 10at.%, which does not show any loss mechanism as at 1046 nm it delivers 11.8 W with a slope efficiency of η(s) = 82%, which is, to the best of our knowledge, the highest value reported in literature for this material.
ABSTRACT
We report the spectroscopic characteristics and the laser performances of a low-doped 1% at. Yb:Sc(2)O(3) ceramic sample. Under end- pumping at 933 nm and 968 nm in quasi-CW mode, at 1040.5 nm the laser delivers a maximum output power of 4.3 W and 1.77 W, respectively with a corresponding slope efficiency of 74% and 80%, which are, to the best of our knowledge, the highest value reported in literature for ceramics. We explored the tuning range of the sample, which spans from 1005 nm to 1050.5 nm, and finally we characterized the low losses tunable cavity at 1032 nm.
Subject(s)
Ceramics , Lasers, Solid-State , Energy Transfer , Equipment Design , Equipment Failure AnalysisABSTRACT
We report the first oscillation achieved on 1 at. % Yb-doped Sc2O3 and Lu2O3 ceramics under quasi-CW pumping at 968 nm. With Sc2O3 we measured a maximum output power of 2.2 W with a slope efficiency of 59% at 1040.5 nm. Comparable results are obtained with Lu2O3 at 1032.5 nm, i.e., 1.8 W with a corresponding slope of 45%, while at 1078 nm we measured 1.5 W with 34% of slope efficiency. Finally, we present the range of tunability, which exceeds 41 nm for both samples. To the best of our knowledge, these are the first measurements reported in literature either in terms of laser emission or continuous tunability range achieved with 1 at. % doping level.
ABSTRACT
We report the behavior of two Yb(3+) doped ceramics (i.e. 10% at. and 20% at.) under quasi-continuous wave laser pumping. Two different behaviors are found depending on the density of Yb(3+) in the excited level. Experimental results show that at low population inversion density, the maximum output power and the efficiency are almost independent on the doping concentration. In particular, an output power as high as 8.9 W with a corresponding slope efficiency of 52% with respect to the injected pump power was reached with the 20% at. sample. Conversely, at high population inversion densities, the 20% doped sample shows a sudden decrease of the laser output for increasing pump power, due to the onset of a nonlinear loss mechanism. Finally, we report a comparison of the experimental results with numerical simulations for the evaluation of the inversion density and of the temperature distribution.
Subject(s)
Ceramics , Lasers, Solid-State , Light , Cold TemperatureABSTRACT
We present a comprehensive characterization of a laser, based on a high-quality heavily doped Yb:YLF crystal. The analysis includes the comparison of the laser efficiency in respect of the absorbed pump for both pi and sigma-polarization. In particular, for the tunable laser, we report an enhancement of the tuning range obtained by adapting the output coupler transmission in respect of the lasing wavelength. The experimental results obtained for various output coupling have also been compared with a numerical model in order to give information for a further enlargement of the tuning range.
ABSTRACT
We report an extensive comparison of the laser performances of diode-pumped Yb(3+):YLF (30% at.) and Yb(3+):CaF(2) (5% at.) crystals, lasing at room-temperature and operating in two different operation mode, i.e. Continuous Wave (CW) and quasi-CW. An in-depth investigation of the crystals behavior by changing the pump power, clearly shows the crystal absorption depends on the lasing conditions. Therefore, we report an unambiguous definition of the slope efficiency calculated taken into account the real measured crystal absorption under laser action. Finally, we present a study of problems related to thermally induced losses which are expected influencing the laser performance.
Subject(s)
Lasers, Solid-State , Computer-Aided Design , Equipment Design , Equipment Failure Analysis , Reproducibility of Results , Sensitivity and Specificity , TemperatureABSTRACT
We present a high-power, high-efficiency and low threshold laser prototype based on doped ceramic Yb(3+):YAG. We achieved an output power of 9 W with a slope efficiency of 73% and a threshold of 1 W at 1030 nm in quasi-Continuous Wave (QCW). Moreover, we obtained an output power 7.7 W with a slope efficiency of 60% in Continuous Wave (CW). Finally, a characterization of a low losses tunable cavity for several laser wavelengths with an output power exceeding 5 W is reported.
Subject(s)
Ceramics/chemistry , Lasers, Solid-State , Computer-Aided Design , Equipment Design , Equipment Failure AnalysisABSTRACT
We report the first direct measurements of the atomic dipole phase in the process of high-order harmonic generation. Differently from previously reported studies based on frequency chirp measurements, we use extreme ultraviolet interferometry as the most natural and direct way to measure phase shifts. Our approach has the important advantage of allowing us to investigate the effects associated to both the main quantum paths involved in the emission of a particular harmonic, thus offering a particularly clear and simple picture of the underlying electronic dynamics.
