Global iron connections between desert dust, ocean biogeochemistry, and climate.

The environmental conditions of Earth, including the climate, are determined by physical, chemical, biological, and human interactions that transform and transport materials and energy. This is the "Earth system": a highly complex entity characterized by multiple nonlinear responses and thresholds, with linkages between disparate components. One important part of this system is the iron cycle, in which iron-containing soil dust is transported from land through the atmosphere to the oceans, affecting ocean biogeochemistry and hence having feedback effects on climate and dust production. Here we review the key components of this cycle, identifying critical uncertainties and priorities for future research.

Long-range transport of mineral dust in the global atmosphere: impact of African dust on the environment of the southeastern United States.

Soil dust is a major constituent of airborne particles in the global atmosphere. Dust plumes frequently cover huge areas of the earth; they are one of the most prominent and commonly visible features in satellite imagery. Dust is believed to play a role in many biogeochemical processes, but the importance of dust in these processes is not well understood because of the dearth of information about the global distribution of dust and its physical, chemical, and mineralogical properties. This paper describes some features of the large-scale distribution of dust and identifies some of the geological characteristics of important source areas. The transport of dust from North Africa is presented as an example of possible long-range dust effects, and the impact of African dust on environmental processes in the western North Atlantic and the southeastern United States is assessed. Dust transported over long distances usually has a mass median diameter <10 microm. Small wind-borne soil particles show signs of extensive weathering; consequently, the physical and chemical properties of the particles will greatly depend on the weathering history in the source region and on the subsequent modifications that occur during transit in the atmosphere (typically a period of a week or more). To fully understand the role of dust in the environment and in human health, mineralogists will have to work closely with scientists in other disciplines to characterize the properties of mineral particles as an ensemble and as individual particles especially with regard to surface characteristics.

Long-range atmospheric transport of soil dust from Asia to the tropical north pacific: temporal variability.

The concentration of airborne soil dust at Enewetak Atoll(11 degrees N, 162 degrees E) in April 1979 was 2.3 micrograms per cubic meter but decreased steadily to 0.02 microgram per cubic meter over the next 5 months. The spring dust is probably derived from China; its deposition rate ( approximately 0.3 millimeter per 1000 years) suggests that it may be a significant contributor to the deep-sea sediments of the North Pacific.

Dust concentration in the atmosphere of the equatorial north atlantic: possible relationship to the sahelian drought.

The concentration of insoluble mineral aerosol in the lower troposphere of the western equatorial North Atlantic Ocean has increased by a factor of 3 over the last decade. This increase may be related to the drought in the Sahelian zone of North Africa.

Radon-222 in the North Atlantic trade winds: its relationship to dust transport from Africa.

The concentration of radon-222 in air was measured during a flight from Miami to Barbados to Dakar and return; concentrations ranged from 1 to 55 picocuries per standard cubic meter of air and were highest in areas of dense haze, which were present along most of the flight path across the Atlantic Ocean. The haze is attributed to dust originating from the arid regions of western Africa. Radon-222 may be useful as a tracer for African air parcels over the equatorial Atlantic.

Beryllium-7 in ocean water.

Concentration of the radio nuclide beryllium-7, produced by cosmic rays, was measured in waters collected from both the Atlantic and Pacific oceans. This short-lived nuclide is well suited as a tracer for interactions at the air-sea interface and for the measurement of rapid mixing processes in the surface layer of the ocean.