ABSTRACT
A single quantum emitter can possess a very strong intrinsic nonlinearity, but its overall promise for nonlinear effects is hampered by the challenge of efficient coupling to incident photons. Common nonlinear optical materials, on the other hand, are easy to couple to but are bulky, imposing a severe limitation on the miniaturization of photonic systems. In this Letter, we show that a single organic molecule acts as an extremely efficient nonlinear optical element in the strong coupling regime of cavity quantum electrodynamics. We report on single-photon sensitivity in nonlinear signal generation and all-optical switching. Our work promotes the use of molecules for applications such as integrated photonic circuits operating at very low powers.
ABSTRACT
We present a computer algorithm capable of simulating the photon stream and the corresponding temporal photon statistics of thermal light sources. The algorithm implements realistic experimental conditions, incorporating the relevant parameters of the source as well as of the detection process. The code is verified by comparing the temporal photon autocorrelation function computed from the simulations to the one measured with a real thermal light source. In view of the renewed interest for intensity interferometry in astronomy and the life sciences, such simulations become increasingly relevant.
