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1.
ACS Appl Mater Interfaces ; 16(22): 29188-29197, 2024 Jun 05.
Article in English | MEDLINE | ID: mdl-38775355

ABSTRACT

Noncontact sensors have demonstrated significant potential in human-machine interactions (HMIs) in terms of hygiene and less wear and tear. The development of soft, stable, and simply structured noncontact sensors is highly desired for their practical applications in HMIs. This work reports on electret-based self-powered noncontact sensors that are soft, transparent, stable, and easy to manufacture. The sensors contain a three-layer structure with a thickness of 0.34 mm that is fabricated by simply stacking a polymeric electret layer, an electrode layer, and a substrate layer together. The fabricated sensors show high charge-retention capability, keeping over 98% of the initial surface potential even after 90 h, and can accurately and repeatedly sense external approaching objects with impressive durability. The intensity of the detected signal shows a strong dependence on the distance between the object and the sensor, capable of sensing a distance as small as 2 mm. Furthermore, the sensors can report stable signals in response to external objects over 3000 cycles. By virtue of the signal dependence on distance, an intelligent noncontact positioning system is developed that can precisely detect the location of an approaching object. Finally, by integrating with eyeglasses, the transparent sensor successfully captures the movements of blinks for information translation. This work may contribute to the development of stable and easily manufactured noncontact soft sensors for HMI applications, for instance, assisting with communication for locked-in syndrome patients.

2.
Adv Mater ; : e2400657, 2024 May 08.
Article in English | MEDLINE | ID: mdl-38719210

ABSTRACT

The growing demand for wearable devices has sparked a significant interest in ferroelectret films. They possess flexibility and exceptional piezoelectric properties due to strong macroscopic dipoles formed by charges trapped at the interface of their internal cavities. This review of ferroelectrets focuses on the latest progress in fabrication techniques for high temperature resistant ferroelectrets with regular and engineered cavities, strategies for optimizing their piezoelectric performance, and novel applications. The charging mechanisms of bipolar and unipolar ferroelectrets with closed and open-cavity structures are explained first. Next, the preparation and piezoelectric behavior of ferroelectret films with closed, open, and regular cavity structures using various materials are discussed. Three widely used models for predicting the piezoelectric coefficients (d33) are outlined. Methods for enhancing the piezoelectric performance such as optimized cavity design, utilization of fabric electrodes, injection of additional ions, application of DC bias voltage, and synergy of foam structure and ferroelectric effect are illustrated. A variety of applications of ferroelectret films in acoustic devices, wearable monitors, pressure sensors, and energy harvesters are presented. Finally, the future development trends of ferroelectrets toward fabrication and performance optimization are summarized along with its potential for integration with intelligent systems and large-scale preparation.

3.
Angew Chem Int Ed Engl ; 62(51): e202315143, 2023 Dec 18.
Article in English | MEDLINE | ID: mdl-37964724

ABSTRACT

With the rapid development of integrated circuits towards miniaturization and complexity, there is an urgent need for materials with low dielectric constant/loss and high processing temperatures to effectively prevent signal delay and crosstalk. With high porosity, thermal stability, and easy structural modulation, covalent organic frameworks have great potential in the field of low dielectric materials. However, the optimization of dielectric properties by modulating the conjugated/plane curvature structure of covalent organic frameworks (COFs) has rarely been reported. Accordingly, we herein innovatively prepare COF films with adjustable planar curvature, hence possessing ultralow dielectric constant (1.9 at 1 kHz), ultralow dielectric loss at 1 kHz (0.0029 at room temperature, 0.0052 at 200 °C), high thermal decomposition temperature (5 % weight loss temperature, 473 °C) and good hydrophobicity (water contact angle, 105.3°). Also, to the best of our knowledge, we are the first to report that the resulting COF film enables high surface potential (≈320 V) for one week, attributing to its intrinsic high porosity, thus presenting great potential in electret applications. Accordingly, this innovative work provides a readily available and scalable idea to prepare materials with comprehensively excellent dielectric and electret properties as well as high processing temperatures simultaneously for advanced electronic device applications.

4.
Sensors (Basel) ; 23(4)2023 Feb 11.
Article in English | MEDLINE | ID: mdl-36850649

ABSTRACT

Most imaging methods based on ultrasonic Lamb waves in structural health monitoring requires reference signals, recorded in the intact state. This paper focuses on a novel baseline-free method for damage localization using Lamb waves based on a hyperbolic algorithm. This method employs a special array with a relatively small number of transducers and only one branch of the hyperbola. The novel symmetrical array was arranged on plate structures to eliminate the direct waves. The time difference between the received signals at symmetrical sensors was obtained from the damage-scattered waves. The sequence of time difference for constructing the hyperbolic trajectory was calculated by the cross-correlation method. Numerical simulation and experimental measurements were implemented on an aluminum plate with a through-thickness hole in the current state. The imaging results show that both the damages outside and inside the diamond-shaped arrays can be localized, and the positioning error reaches the maximum for the diamond-shaped array with the minimum size. The results indicate that the position of the through-hole in the aluminum plate can be identified and localized by the proposed baseline-free method.

5.
Nanotechnology ; 33(32)2022 May 20.
Article in English | MEDLINE | ID: mdl-35439735

ABSTRACT

In recent years, flexible pressure sensors have caused widespread concern for their extensive applications in human activity and health monitoring, robotics and prosthesis, as well as human-machine interface. Flexible pressure sensors in these applications are required to have a high sensitivity, large detective limit, linear response, fast response time, and mechanical stability. The mechanisms of capacitive, piezoresistive, and piezoelectric pressure sensors and the strategies to improve their performance are introduced. Sensing layers with microstructures have shown capability to significantly improve the performances of pressure sensors. Various fabrication methods for these structures are reviewed in terms of their pros and cons. Besides, the interference caused by environmental stimuli and internal stress from different directions leads to the infidelity of the signal transmission. Therefore, the anti-interference ability of flexible pressure sensors is highly desired. Several potential applications for flexible pressure sensors are also briefly discussed. Last, we conclude the future challenges for facilely fabricating flexible pressure sensors with high performance and anti-interference ability.

6.
Ultrasonics ; 119: 106606, 2022 Feb.
Article in English | MEDLINE | ID: mdl-34627027

ABSTRACT

The combination of air-coupled ultrasonic testing (ACUT) and ultrasonic Lamb wave is featured with long-distance propagation and high sensitivity to discontinuities, which is a promising method for rapid and accurate inspection of plate-like materials and lightweighted structures. However, dispersive nature of Lamb wave, signal attenuation plus inevitable noises would lead to low signal-to-noise ratio (SNR). To address this problem, phase coded excitation and pulse compression technique are proposed in this paper to achieve higher SNR by over 10 dB in received signals. 13-bit and 1-carrier-period Barker code is employed as both main lobe peak and Peak Side-lobe Level (PSL) are relatively high. It is demonstrated that A0 mode Lamb wave has good localization ability for defects based on these SNR-enhanced signals. Furthermore, Damage Index (DI) and modified Reconstruction Algorithm for the Probabilistic Inspection of Damage (RAPID) are applied to realize ultrasonic imaging based defect evaluation. Results show that the imaging results agree well with the actual artificial defects in terms of size and shape. Lamb-wave-based air-coupled ultrasonic testing, combined with DI and ultrasonic imaging algorithm, could be a potential way in the NDT of lightweighted structures.

7.
Sensors (Basel) ; 23(1)2022 Dec 22.
Article in English | MEDLINE | ID: mdl-36616695

ABSTRACT

This article proposes an electromagnetic acoustic transducer (EMAT) for selectively improving the purity and amplitude of ultrasonic Lamb waves in non-ferromagnetic plates. The developed EMAT consists of a racetrack coil and a group of periodic permanent magnets (PPMs). Two-dimensional finite element simulations and experiments are implemented to analyze the working mechanism and performance of the PPM EMAT. Thanks to the specific design, the eddy currents increase with increasing wire density and the directions of the magnetic fields and Lorentz forces alternate according to the polarities of the magnet units. Wires laid uniformly beneath the magnets, and the gaps between adjacent magnets generate tangential and normal Lorentz forces, resulting in-plane (IP) and out-of-plane (OP) displacements, respectively. The constructive interference occurs when the wavelength of the generated Lamb wave is twice the spacing of the magnets, leading to large amplitudes of the targeted ultrasonic Lamb waves. Therefore, the PPM EMAT is capable of generating pure symmetric or antisymmetric mode Lamb waves at respective frequencies. The results prove that the developed PPM EMAT can generate pure either S0 or A0 mode Lamb waves at respective frequencies. The increase in wire width and wire density further increases the signal amplitudes. Compared with the case of conventional meander-line-coil (MLC) EMAT, the amplitudes of the A0 and S0 mode Lamb waves of our PPM EMAT are increased to 880% and 328%, respectively.

8.
Adv Mater ; 33(8): e2006437, 2021 Feb.
Article in English | MEDLINE | ID: mdl-33458893

ABSTRACT

The trend to a world with ubiquitous electronics has the need for novel concepts for sensors and actuators that are lightweight, flexible, low-cost, and also sustainable. Piezoelectric transducers on the basis of functional polymers can meet these expectations. In this work, a novel concept for paper-embedded large-area piezoelectric devices realized solely by means of roll-to-roll (R2R) mass printing and post printing technologies including inline poling are introduced. The device set-up, as well as the process technology, offers the great opportunity for a cost-efficient and environmentally friendly mass production of thin and flexible organic large-area piezoelectric devices. As the functional layers are embedded into paper by the hot lamination of two poly(vinylidene fluoride-co-trifluoroethylene) P(VDF-TrFE) layers, the printed electronics is protected and invisible. The paper gives insights to the R2R printing of a 500 m long web including R2R post printing processes and electrical and acoustic inline characterization. Fully R2R processed devices show a high remnant polarization of up to 78 mC m-2 and can be realized with high yield of >90%. Finally, a 360° surround-sound installation realized with a 387 cm long paper web consisting of 56 piezoelectric speakers including wiring is presented.

9.
Nat Commun ; 5: 4293, 2014 Jul 01.
Article in English | MEDLINE | ID: mdl-24980606

ABSTRACT

Fast actuation speed, large-shape deformation and robust responsiveness are critical to synthetic soft actuators. A simultaneous optimization of all these aspects without trade-offs remains unresolved. Here we describe porous polymer actuators that bend in response to acetone vapour (24 kPa, 20 °C) at a speed of an order of magnitude faster than the state-of-the-art, coupled with a large-scale locomotion. They are meanwhile multi-responsive towards a variety of organic vapours in both the dry and wet states, thus distinctive from the traditional gel actuation systems that become inactive when dried. The actuator is easy-to-make and survives even after hydrothermal processing (200 °C, 24 h) and pressing-pressure (100 MPa) treatments. In addition, the beneficial responsiveness is transferable, being able to turn 'inert' objects into actuators through surface coating. This advanced actuator arises from the unique combination of porous morphology, gradient structure and the interaction between solvent molecules and actuator materials.

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