Colorimetry characterization of molecular reorientation transition in thin nematic cells.

The characterization of equilibria and their transition is fundamental in dynamic systems. Experimentally, the characterization of transitions is complex due to time scales separation, the effect of thermal fluctuations, and inherent experimental imperfections. Liquid crystal devices are derived from the manipulation of the molecular reorientation and transition between them by employing external electrical and magnetic fields. Here, we investigate and determine the Fréedericksz transition using hue measurements of the transmitted light in thin nematic liquid crystal cells. Based on birefringent retardation experienced by transmitted light due to molecular reorientation, the color adjustment of the nematic liquid crystal cells under white light illumination is characterized. By monitoring the hue of the transmitted light, the bifurcation diagram is determined. As a function of the voltage frequency, the critical transition voltage is characterized. The critical voltage increases with the applied frequency.

Dissipative structures induced by photoisomerization in a dye-doped nematic liquid crystal layer.

Order-disorder phase transitions driven by temperature or light in soft matter materials exhibit complex dissipative structures. Here, we investigate the spatio-temporal phenomena induced by light in a dye-doped nematic liquid crystal layer. Experimentally, for planar anchoring of the nematic layer and high enough input power, photoisomerization processes induce a nematic-isotropic phase transition mediated by interface propagation between the two phases. In the case of a twisted nematic layer and for intermediate input power, the light induces a spatially modulated phase, which exhibits stripe patterns. The pattern originates as an instability mediated by interface propagation between the modulated and the homogeneous nematic states. Theoretically, the phase transition, emergence of stripe patterns and front dynamics are described on the basis of a proposed model for the dopant concentration coupled with the nematic order parameter. Numerical simulations show quite a fair agreement with the experimental observations.This article is part of the theme issue 'Dissipative structures in matter out of equilibrium: from chemistry, photonics and biology (part 2)'.

Light-matter interaction induces a shadow vortex.

By sending a light beam on a homeotropic nematic liquid-crystal cell subjected to a voltage with a photosensitive wall, a stable matter vortex can be induced at the center of the beam. When the applied voltage is decreased, the vortex disappears from the illuminated region; however, the system shows a stationary molecular texture. Based on a forced Ginzburg-Landau amplitude equation, we show that the vortex with a core of exponentially suppressed amplitude always remains in a shadow region below instability threshold and that the observed texture is induced by its phase distribution. This is a different type of vortex phase singularity solution. Numerical simulations and experimental observations show a quite fair agreement.

Control and generation of drifting patterns by asymmetrical Fourier filtering.

We report the theoretical and experimental demonstration of one-dimensional drifting patterns generated by asymmetrical Fourier filtering in the transverse plane of an optical feedback system with a Kerr type nonlinearity. We show, with good agreement between our theoretical (analytics and numerics) calculations and experimental observations that at the primary instability threshold the group velocity is always different from zero. Consequently, the system is convective at this threshold, then exhibits drifting patterns.

Light-matter interaction induces a single positive vortex with swirling arms.

Homeotropic nematic liquid crystal cells with a photosensitive wall and negative dielectric anisotropy exhibit, under the influence of local illumination, stable vortexes with swirling arms that are trapped at the illuminated area. Close to the Fréedericksz transition an amplitude equation is derived, which allows us to understand the origin of the induced vortex and the competition between the illuminating profile and the elastic anisotropy generating the swirling of the arms.

Chaoticon: localized pattern with permanent dynamics.

An analytical mechanism that support localized spatio-temporal chaos is provided. We consider a simple model-the Nagumo Kuramoto model-which contains the crucial ingredients for observing localized spatio-temporal chaos, namely, the spatio-temporal chaotic pattern and its coexistence with a uniform state. This model allows us to unveil the front dynamics and to show that it can be described by a chaotic motor corresponding to the deterministic counterpart of a Brownian motor. Front interaction is identified as the mechanism at the origin of the localized spatio-temporal chaotic structures.

Photo-isomerization fronts in dye-doped nematic liquid crystals.

An experimental study of the photo-isomerization dynamics in dye-doped nematic crystals is reported, which shows that, when the sample is illuminated by a Gaussian beam, and for high enough input power, a transition from the nematic to the isotropic phase takes place in the illuminated area. The two phases are spatially connected via a front propagating outward from the center of the beam and following the local intensity profile and thus inducing a photo-controlled optical aperture. The optical intensity and temperature fields on the sample follow the same dynamical profile. The front dynamics is described by a phenomenological bi-stable model with an inhomogeneous control parameter, directly related to the beam intensity profile.

Slow and stored light by photo-isomerization induced transparency in dye doped chiral nematics.

Decelerating and stopping light is fundamental for optical processing, high performance sensor technologies and digital signal treatment, many of these applications relying on the ability of controlling the amplitude and phase of coherent light pulses. In this context, slow-light has been achieved by various methods, as coupling light into resonant media, Brillouin scattering in optical fibers, beam coupling in photorefractive and liquid crystal media or engineered dispersion in photonic crystals. Here, we present a different mechanism for slowing and storing light, which is based on photo-isomerization induced transparency of azo-dye molecules hosted in a chiral liquid crystal structure. Sharp spectral features of the medium absorption/dispersion, and the long population lifetime of the dye metastable state, enable the storage of light pulses with a significant retrieval after times much longer than the medium response time.

Harnessing optical vortex lattices in nematic liquid crystals.

By creating self-induced vortexlike defects in the nematic liquid crystal layer of a light valve, we demonstrate the realization of programable lattices of optical vortices with arbitrary distribution in space. On each lattice site, every matter vortex acts as a photonic spin-to-orbital momentum coupler and an array of circularly polarized input beams is converted into an output array of vortex beams with topological charges consistent with the matter lattice. The vortex arrangements are explained on the basis of light-induced matter defects of both signs and consistent topological rules.

Spatiotemporal chaotic localized state in liquid crystal light valve experiments with optical feedback.

The existence, stability properties, and dynamical evolution of localized spatiotemporal chaos are studied. We provide evidence of spatiotemporal chaotic localized structures in a liquid crystal light valve experiment with optical feedback. The observations are supported by numerical simulations of the Lifshitz model describing the system. This model exhibits coexistence between a uniform state and a spatiotemporal chaotic pattern, which emerge as the necessary ingredients to obtain localized spatiotemporal chaos. In addition, we have derived a simplified model that allows us to unveil the front interaction mechanism at the origin of the localized spatiotemporal chaotic structures.

Golden spirals as phyllotactic arrangements of optical patterns.

A nonlinear optical medium with nonlocal feedback is shown to have all the necessary ingredients to simulate a growthlike process that generates golden spirals and phyllotactic patterns. Elementary droplets of light are generated by the optical nonlinearity whereas the combination of rotation and translation in the feedback loop geometrically distributes them on spiraling patterns. The symmetry of the geometrical arrangements is described with the help of a simple replication algorithm.

Phase conjugation and slow light in dye-doped chiral nematics.

Optical phase conjugation and slow light are obtained in dye-doped chiral nematics via degenerate four-wave mixing. The creation of the light-induced dynamical grating is described and the amplitude of the phase-conjugate wave is shown to follow the changes of the input signal, hence providing efficient distortion correction. Associated to these capabilities, slowing down of light pulses is obtained thanks to the dispersive properties of the wave mixing occurring in the cholesteric liquid crystals, opening the way to applications in interferometry and imaging through highly scattering media.

Vortex induction via anisotropy stabilized light-matter interaction.

By sending circularly polarized light beams onto a homeotropic nematic liquid crystal cell with a photosensitive wall, we are able to locally induce spontaneous matter vortices that remain, each, stable and trapped at the chosen location. We discuss the dual light-matter nature of the created vortices and demonstrate the ability of the system to create optical vortices with opposite topological charges that, consistent with angular momentum conservation, both derive from the same defect created in the liquid crystal texture. Theoretically, we identify a self-stabilizing mechanism for the matter vortex, which is provided by the concurrency of light-induced gradients and anisotropy of the elastic constants that characterize the deformation of the liquid crystal medium.

Effects of translational coupling on dissipative localized states.

Nonequilibrium localized states under the influence of translational coupling are studied experimentally and theoretically. We show that localized structures are deformed and advected in the direction of the coupling, thus undergoing different instabilities. Experimentally, localized structures are obtained in a light valve with optical feedback. By introducing a tilt of one mirror in the feedback loop, localized structures acquire a translational coupling. To understand the phenomenon in a universal framework we consider a prototypical model of localized states with translational coupling in one and two spatial dimensions. The model allows us to analytically characterize the propagation speed and the deformation exhibited by the localized state profiles as well as to figure out different mechanisms of destabilization of these dissipative structures. The results are in good qualitative agreement with the experimental and numerical observations.

High resolution wavefront correction with photocontrolled deformable mirror.

We demonstrate that a novel actuation scheme, employed in an optical control deformable mirror, can be more convenient than the conventional discrete fixed actuators approach. The Photo-Controlled Deformable Mirror (PCDM) mirror leverages consumer LCD display technology in the wavefront forming control, enabling flexible programmable configuration of the actuation geometry. This new approach simplifies the driving electronics, relaxing the per channel cost of high spatial control of the wavefront forming surface. In our experiment we tested the PCDM by applying the equivalent of 36, 76 and 201 actuators, this by just changing the light driving pattern. We demonstrated the effectiveness of this technique in a closed loop setup, which showed performances superior to the state of the art for similar DM, while providing a significant reduction in the hardware complexity.

Optical pulsing in a resonator with a highly dispersive nonlinearity.

By introducing an intracavity Doppler shift in a resonator with a highly dispersive nonlinear medium, a train of optical pulses is generated whose features are related to the slow/fast-light response of the medium. The cavity transmission is asymmetric and the pulse shape is modified differently depending on the direction of the Doppler shift, hence, on the sign of the group delay provided by the dispersive process.

Two-wave mixing in chiral dye-doped nematic liquid crystals.

Two-wave mixing in nematic liquid crystals doped with dyes and chiral agents is studied. The photo-induced spatial modulation of the chiral structure, together with the diffusion anisotropy of the mixture, determine a relatively fast response time, a spatial resolution of 1 µm, and a maximum gain for circularly polarized interacting beams. The gain is insensitive to changes in linear polarization, while it varies with the grating period and with the pump-to-signal intensity ratio.

Granularity and inhomogeneity are the joint generators of optical rogue waves.

In the presence of many waves, giant events can occur with a probability higher than expected for random dynamics. By studying linear light propagation in a glass fiber, we show that optical rogue waves originate from two key ingredients: granularity, or a minimal size of the light speckles at the fiber exit, and inhomogeneity, that is, speckles clustering into separate domains with different average intensities. These two features characterize also rogue waves in nonlinear systems; thus, nonlinearity just plays the role of bringing forth the two ingredients of granularity and inhomogeneity.

Experimental observation of speckle instability in Kerr random media.

In a disordered nonlinear medium the transmitted speckle pattern was predicted to become unstable as a result of the positive feedback between intensity fluctuations and local variations of the refractive index. We show experimental evidence of speckle instability for light transversally scattered in a liquid crystal cell, where a two-dimensional controlled disorder is imprinted by suitable illumination of a photoconductive wall and nonlinearity is obtained through optical reorientation of the liquid crystal molecules. The speckle pattern spontaneously oscillates at discrete frequencies above a critical threshold, whose dependence on the scattering mean free path confirms the crucial role of disorder in the feedback process.

Vortex emission accompanies the advection of optical localized structures.

We show that the advection of optical localized structures is accompanied by the emission of vortices, with phase singularities appearing in the wake of the drifting structure. Localized structures are obtained in a light-valve experiment and made to drift by a mirror tilt in the feedback loop. Pairs of oppositely charged vortices are detected for small drifts, whereas for large drifts a vortex array develops. Observations are supported by numerical simulations and linear stability analysis of the system equations and are expected to be generic for a large class of translated optical patterns.