ABSTRACT
We have realized optical excitation, trapping, and detection of the radioisotope ^{81}Kr with an isotopic abundance of 0.9 ppt. The 124 nm light needed for the production of metastable atoms is generated by a resonant discharge lamp. Photon transport through the optically thick krypton gas inside the lamp is simulated and optimized to enhance both brightness and resonance. We achieve a state-of-the-art ^{81}Kr loading rate of 1800 atoms/h, which can be further scaled up by adding more lamps. The all-optical approach overcomes the limitations on precision and sample size of radiokrypton dating, enabling new applications in the earth sciences, particularly for dating of polar ice cores.
ABSTRACT
An isotope enrichment system for 39Ar has been developed at the Institute of Modern Physics, which is designed to increase the abundance of 39Ar in the incident sample gas. With intense Ar+ beams produced by a 2.45 GHz electron cyclotron resonance ion source and a high mass resolution spectrometer system, Ar isotopes are evidently separated on the target plane and selectively collected by an Al target. The separated Ar isotopes have been identified on the target plane, which is consistent with the simulations. According to the recent cross-checked results with atom trap trace analysis, a high enrichment factor of 39Ar has been successfully achieved. This paper will present the design and test results of this system.
ABSTRACT
We report on the first experimental determination of the hyperfine structure of the 1s(5)-2p(9) transition in (39)Ar. We give a detailed description of the sample preparation, spectroscopy cell cleaning, and spectroscopic setup. The resulting set of parameters consists of the hyperfine constants of the levels involved and the isotopic shift between (39)Ar and (40)Ar. With the achieved precision all laser frequencies necessary for the implementation of atom trap trace analysis for (39)Ar, i.e., laser cooling and repumping frequencies, are now known.
