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1.
Phys Rev Lett ; 118(23): 237402, 2017 Jun 09.
Article in English | MEDLINE | ID: mdl-28644673

ABSTRACT

We present a semiclassical analytic model for spherical core-shell surface plasmon lasers. Within this model, we drop the widely used one-mode approximations in favor of fully electromagnetic Mie theory. This allows for incorporation of realistic gain relaxation rates that so far are massively underestimated. Especially, higher order modes can undermine and even reverse the beneficial effects of the strong Purcell effect in such systems. Our model gives a clear view on gain and resonator requirements, as well as on the output characteristics that will help experimenters to design more efficient particle-based spasers.

2.
Opt Express ; 21(10): 12022-37, 2013 May 20.
Article in English | MEDLINE | ID: mdl-23736424

ABSTRACT

Efficient modelling of the magneto-optic effects of transition metals such as nickel, cobalt and iron is a topic of growing interest within the nano-optics community. In this paper, we present a general discussion of appropriate material models for the linear dielectric properties for such metals, provide parameter fits and formulate the anisotropic response in terms of auxiliary differential equations suitable for time-domain simulations. We validate both our material models and their implementation by comparing numerical results obtained with the Discontinuous Galerkin time-domain (DGTD) method to analytical results and previously published experimental data.


Subject(s)
Light , Magnetic Fields , Metal Nanoparticles/chemistry , Metal Nanoparticles/radiation effects , Models, Chemical , Computer Simulation
3.
Opt Express ; 19(13): 12208-19, 2011 Jun 20.
Article in English | MEDLINE | ID: mdl-21716458

ABSTRACT

We present an advanced numerical formulation to calculate the optical properties of 3D nanoparticles (single or coupled) of arbitrary shape and lack of symmetry. The method is based on the (formally exact) surface integral equation formulation, implemented for parametric surfaces describing particles with arbitrary shape through a unified treatment (Gielis' formula). Extinction, scattering, and absorption spectra of a variety of metal nanoparticles are shown, thus determining rigorously the localised surface-plasmon resonances of nanocubes, nanostars, and nanodimers. Far-field and near-field patterns for such resonances are also calculated, revealing their nature. The flexibility and reliability of the formulation makes it specially suitable for complex scattering problems in Nano-Optics & Plasmonics.


Subject(s)
Models, Theoretical , Nanoparticles/chemistry , Surface Plasmon Resonance/methods , Electromagnetic Fields , Scattering, Radiation , Surface Plasmon Resonance/instrumentation , Surface Properties
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