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1.
Nat Commun ; 15(1): 4623, 2024 May 30.
Article in English | MEDLINE | ID: mdl-38816364

ABSTRACT

Finding evidence of non-trivial pairing states is one of the greatest experimental challenges in the field of unconventional superconductivity. Such evidence requires phase-sensitive probes susceptible to the internal structure of the order parameter. We report the measurement of the Little-Parks effect in the unconventional superconductor candidate 4Hb-TaS2. In half of our rings, which are fabricated from single-crystals, we find a π-shift in the transition-temperature oscillations. According to theory, such a π-shift is only possible if the order parameter is non-s-wave. In the absence of crystallographic defects, the shift provides evidence of a multi-component order parameter. Thus, this observation increases the likelihood of the two-component order parameter scenario in 4Hb-TaS2. Furthermore, we show that Tc is enhanced as a function of the out-of-plane field when a constant in-plane field is applied, which we explain using a two-component order-parameter.

3.
Phys Rev Lett ; 129(23): 237001, 2022 Dec 02.
Article in English | MEDLINE | ID: mdl-36563208

ABSTRACT

We study superconductivity in a three-dimensional zero-density Dirac semimetal in proximity to a ferroelectric quantum critical point. We find that the interplay of criticality, inversion-symmetry breaking, and Dirac dispersion gives rise to a robust superconducting state at the charge-neutrality point, where no Fermi surface is present. Using Eliashberg theory, we show that the ferroelectric quantum critical point is unstable against the formation of a ferroelectric density wave (FDW), whose fluctuations, in turn, lead to a first-order superconducting transition. Surprisingly, long-range superconducting and FDW orders are found to cooperate with each other, in contrast to the more usual scenario of phase competition. Therefore, we suggest that driving charge neutral Dirac materials, e.g., Pb_{x}Sn_{1-x}Te, through a ferroelectric quantum critical point may lead to superconductivity intertwined with FDW order.

4.
Nature ; 607(7920): 692-696, 2022 07.
Article in English | MEDLINE | ID: mdl-35896649

ABSTRACT

Doped Mott insulators exhibit some of the most intriguing quantum phases of matter, including quantum spin liquids, unconventional superconductors and non-Fermi liquid metals1-3. Such phases often arise when itinerant electrons are close to a Mott insulating state, and thus experience strong spatial correlations. Proximity between different layers of van der Waals heterostructures naturally realizes a platform for experimentally studying the relationship between localized, correlated electrons and itinerant electrons. Here we explore this relationship by studying the magnetic landscape of tantalum disulfide 4Hb-TaS2, which realizes an alternating stacking of a candidate spin liquid and a superconductor4. We report on a spontaneous vortex phase whose vortex density can be trained in the normal state. We show that time-reversal symmetry is broken in the normal state, indicating the presence of a magnetic phase independent of the superconductor. Notably, this phase does not generate ferromagnetic signals that are detectable using conventional techniques. We use scanning superconducting quantum interference device microscopy to show that it is incompatible with ferromagnetic ordering. The discovery of this unusual magnetic phase illustrates how combining superconductivity with a strongly correlated system can lead to unexpected physics.

5.
Nat Commun ; 12(1): 3311, 2021 Jun 03.
Article in English | MEDLINE | ID: mdl-34083533

ABSTRACT

In systems near phase transitions, macroscopic properties often follow algebraic scaling laws, determined by the dimensionality and the underlying symmetries of the system. The emergence of such universal scaling implies that microscopic details are irrelevant. Here, we locally investigate the scaling properties of the metal-insulator transition at the LaAlO3/SrTiO3 interface. We show that, by changing the dimensionality and the symmetries of the electronic system, coupling between structural and electronic properties prevents the universal behavior near the transition. By imaging the current flow in the system, we reveal that structural domain boundaries modify the filamentary flow close to the transition point, preventing a fractal with the expected universal dimension from forming.

6.
Phys Rev Lett ; 118(22): 227001, 2017 Jun 02.
Article in English | MEDLINE | ID: mdl-28622001

ABSTRACT

We study how an inversion-breaking quantum critical point affects the ground state of a one-dimensional electronic liquid with repulsive interaction and spin-orbit coupling. We find that regardless of the interaction strength, the critical fluctuations always lead to a gap in the electronic spin sector. The origin of the gap is a two-particle backscattering process, which becomes relevant due to renormalization of the Luttinger parameter near the critical point. The resulting spin-gapped state is topological and can be considered as a one-dimensional version of a spin-triplet superconductor. Interestingly, in the case of a ferromagnetic critical point, the Luttinger parameter is renormalized in the opposite manner, such that the system remains nonsuperconducting.

7.
Phys Rev Lett ; 114(10): 100401, 2015 Mar 13.
Article in English | MEDLINE | ID: mdl-25815908

ABSTRACT

We describe a novel topological superfluid state, which forms in a one-dimensional Fermi gas with Rashba-like spin-orbit coupling, a Zeeman field, and intrinsic attractive interactions. In spite of total number conservation and the presence of gapless excitations, Majorana-like zero modes appear in this system and can be linked with interfaces between two distinct phases that naturally form at different regions of the harmonic trap. As a result, the low lying collective excitations of the system, including the dipole oscillations and the long-wavelength phonons are all doubly degenerate. While backscattering from point impurities can lead to a splitting of the degeneracies that scales algebraically with the system size, the smooth confining potential can only cause an exponentially small splitting. We show that the topological state can be uniquely probed by a pumping effect induced by a slow sweep of the Zeeman field from a high initial value down to zero. The effect is expected to be robust to introducing a finite temperature as long as it is much smaller than the interaction induced single particle gap in the final state of the sweep.

8.
Proc Natl Acad Sci U S A ; 110(24): 9633-8, 2013 Jun 11.
Article in English | MEDLINE | ID: mdl-23708121

ABSTRACT

Controlling the coupling between localized spins and itinerant electrons can lead to exotic magnetic states. A novel system featuring local magnetic moments and extended 2D electrons is the interface between LaAlO3 and SrTiO3. The magnetism of the interface, however, was observed to be insensitive to the presence of these electrons and is believed to arise solely from extrinsic sources like oxygen vacancies and strain. Here we show the existence of unconventional electronic phases in the LaAlO3/SrTiO3 system pointing to an underlying tunable coupling between itinerant electrons and localized moments. Using anisotropic magnetoresistance and anomalous Hall effect measurements in a unique in-plane configuration, we identify two distinct phases in the space of carrier density and magnetic field. At high densities and fields, the electronic system is strongly polarized and shows a response, which is highly anisotropic along the crystalline directions. Surprisingly, below a density-dependent critical field, the polarization and anisotropy vanish whereas the resistivity sharply rises. The unprecedented vanishing of the easy axes below a critical field is in sharp contrast with other coupled magnetic systems and indicates strong coupling with the moments that depends on the symmetry of the itinerant electrons. The observed interplay between the two phases indicates the nature of magnetism at the LaAlO3/SrTiO3 interface as both having an intrinsic origin and being tunable.


Subject(s)
Aluminum , Electrons , Lanthanum , Oxides/chemistry , Strontium/chemistry , Titanium/chemistry , Algorithms , Anisotropy , Magnetic Fields , Magnetics , Models, Chemical
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