Tuning Exchange Coupling in a New Family of Nanocrystal-Based Granular Multiferroics Using an Applied Electric Field.

In this work, we demonstrate an experimental realization of a granular multiferroic composite, where the magnetic state of a nanocrystal array is modified by tuning the interparticle exchange coupling using an applied electric field. Previous theoretical models of a granular multiferroic composite predicted a unique magnetoelectric coupling mechanism, in which the magnetic spins of the ensemble are governed by interparticle exchange. The extent of these exchange interactions can be controlled by varying the local dielectric environment between grains. We specifically utilize the strong dielectric dependence of ferroelectric materials to modify the interparticle coupling of closely spaced magnetic nanoparticles using either a change in temperature or an electric field. This coupling modifies the ensemble magnetic coercivity and thus the superparamagnetic-to-ferromagnetic phase transition temperature. Through the use of two different ferroelectrics, our results suggest that this magnetoelectric coupling mechanism could be generalized as a new class of multiferroic material, applicable to a broad range of ferroelectric/magnetic nanocrystal composites.

Dzyaloshinskii-Moriya Interaction across an Antiferromagnet-Ferromagnet Interface.

The antiferromagnet- (AFM-)ferromagnet (FM) interfaces are of central importance in recently developed pure electric or ultrafast control of FM spins, where the underlying mechanisms remain unresolved. Here we report the direct observation of an Dzyaloshinskii-Moriya interaction (DMI) across the AFM-FM interface of IrMn/CoFeB thin films. The interfacial DMI is quantitatively measured from the asymmetric spin-wave dispersion in the FM layer using Brillouin light scattering. The DMI strength is enhanced by a factor of 7 with increasing IrMn layer thickness in the range of 1-7.5 nm. Our findings provide deeper insight into the coupling at the AFM-FM interface and may stimulate new device concepts utilizing chiral spin textures such as magnetic Skyrmions in AFM-FM heterostructures.

Note: Automated electrochemical etching and polishing of silver scanning tunneling microscope tips.

Fabrication of sharp and smooth Ag tips is crucial in optical scanning probe microscope experiments. To ensure reproducible tip profiles, the polishing process is fully automated using a closed-loop laminar flow system to deliver the electrolytic solution to moving electrodes mounted on a motorized translational stage. The repetitive translational motion is controlled precisely on the µm scale with a stepper motor and screw-thread mechanism. The automated setup allows reproducible control over the tip profile and improves smoothness and sharpness of tips (radius 27 ± 18 nm), as measured by ultrafast field emission.