ABSTRACT
We report on the infrared studies of the interlayer charge dynamics of a prototypical pnictide superconductor Ba(Fe(0.926)Co(0.074))(2)As(2). We succeeded in probing the intrinsic interlayer response by performing infrared experiments on the crystals with a cleaved ac surface. Our experiments identify the coexistence of the suppression of the electronic spectral weight and the development of a coherent Drude-like response in the normal state. The formation of the interlayer condensate is clearly observed in the superconducting state and appears to be linked to coherent contribution to the normal-state conductivity.
ABSTRACT
We report on infrared studies of charge dynamics in a prototypical pnictide system: the BaFe2As2 family. Our experiments have identified hallmarks of the pseudogap state in the BaFe2As2 system that mirror the spectroscopic manifestations of the pseudogap in the cuprates. The magnitude of the infrared pseudogap is in accord with that of the spin-density-wave gap of the parent compound. By monitoring the superconducting gap of both P- and Co-doped compounds, we find that the infrared pseudogap is unrelated to superconductivity. The appearance of the pseudogap is found to correlate with the evolution of the antiferromagnetic fluctuations associated with the spin-density-wave instability. The strong-coupling analysis of infrared data further reveals the interdependence between the magnetism and the pseudogap in the iron pnictides.
ABSTRACT
We report an infrared optical study of the pnictide high-temperature superconductor BaFe(1.84)Co(0.16)As(2) and its parent compound BaFe(2)As(2). We demonstrate that electronic correlations are moderately strong and do not change across the spin-density wave transition or with doping. By examining the energy scale and direction of spectral weight transfer, we argue that Hund's coupling J is the primary mechanism that gives rise to correlations.
ABSTRACT
We show that a multilayer analysis of the infrared c-axis response of RBa2Cu3O(7-δ) (R=Y, Gd, Eu) provides important new information about the anomalous normal-state properties of underdoped cuprate high temperature superconductors. In addition to competing correlations which give rise to a pseudogap that depletes the low-energy electronic states below T*â«T(c), it enables us to identify the onset of a precursor superconducting state below T(ons)>T(c). We map out the doping phase diagram of T(ons) which reaches a maximum of 180 K at strong underdoping and present magnetic field dependent data which confirm our conclusions.
ABSTRACT
We report a novel aspect of the competition and coexistence between magnetism and superconductivity in the high-T(c) cuprate La(2-x)Sr(x)CuO4 (La214). With a modest magnetic field applied H parallel c axis, we monitored the infrared signature of pair tunneling between the CuO2 planes and discovered the complete suppression of interlayer coupling in a series of underdoped La214 single crystals. We find that the in-plane superconducting properties remain intact, in spite of enhanced magnetism in the planes.
ABSTRACT
We present infrared magneto-optical measurements of the c-axis conductivity of YBa2Cu3Oy in both the underdoped (y=6.67 and 6.75) and optimally doped (y=6.95) regimes. We show that modest c-axis magnetic fields radically modify the condensate formation and restore conventional BCS-like energetics. Additionally, we demonstrate the pivotal role of interplane coherence in the anomalous high-energy contribution to the superfluid density.
ABSTRACT
We report on a comprehensive optical, transport, and thermodynamic study of the Zintl compound Yb(14)MnSb(11), demonstrating that it is the first ferromagnetic Kondo lattice compound in the underscreened limit. We propose a scenario whereby the combination of Kondo and Jahn-Teller effects provides a consistent explanation of both transport and optical data.
