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1.
Phys Rev Lett ; 122(12): 127201, 2019 Mar 29.
Article in English | MEDLINE | ID: mdl-30978068

ABSTRACT

Polarized inelastic neutron scattering experiments recently identified the amplitude (Higgs) mode in C_{9}H_{18}N_{2}CuBr_{4}, a two-dimensional near-quantum-critical spin-1/2 two-leg ladder compound, which exhibits a weak easy-axis exchange anisotropy. Here, we theoretically examine the dynamic spin structure factor of such planar coupled spin-ladder systems using large-scale quantum Monte Carlo simulations. This allows us to provide a quantitative account of the experimental neutron scattering data within a consistent quantum spin model. Moreover, we trace the details of the continuous evolution of the amplitude mode from a two-particle bound state of coupled ladders in the classical Ising limit all the way to the quantum spin-1/2 Heisenberg limit with fully restored SU(2) symmetry, where it gets overdamped by the two-magnon continuum in neutron scattering.

2.
Phys Rev Lett ; 121(16): 167201, 2018 Oct 19.
Article in English | MEDLINE | ID: mdl-30387667

ABSTRACT

We investigate the impact of quenched disorder on the zero-temperature dynamic structure factor of two-leg quantum spin ladders. Using linked-cluster expansions and bond-operator mean-field theory, huge effects on individual quasiparticles but also on composite bound states and two-quasiparticle continua are observed. This leads to intriguing quantum structures in dynamical correlation functions well observable in spectroscopic experiments.

3.
Nat Commun ; 9(1): 1085, 2018 03 14.
Article in English | MEDLINE | ID: mdl-29540711

ABSTRACT

A quantum spin liquid state has long been predicted to arise in spin-1/2 Heisenberg square-lattice antiferromagnets at the boundary region between Néel (nearest-neighbor interaction dominates) and columnar (next-nearest-neighbor interaction dominates) antiferromagnetic order. However, there are no known compounds in this region. Here we use d10-d0 cation mixing to tune the magnetic interactions on the square lattice while simultaneously introducing disorder. We find spin-liquid-like behavior in the double perovskite Sr2Cu(Te0.5W0.5)O6, where the isostructural end phases Sr2CuTeO6 and Sr2CuWO6 are Néel and columnar type antiferromagnets, respectively. We show that magnetism in Sr2Cu(Te0.5W0.5)O6 is entirely dynamic down to 19 mK. Additionally, we observe at low temperatures for Sr2Cu(Te0.5W0.5)O6-similar to several spin liquid candidates-a plateau in muon spin relaxation rate and a strong T-linear dependence in specific heat. Our observations for Sr2Cu(Te0.5W0.5)O6 highlight the role of disorder in addition to magnetic frustration in spin liquid physics.

4.
Nat Commun ; 8: 15148, 2017 05 05.
Article in English | MEDLINE | ID: mdl-28474679

ABSTRACT

The notion of a quasiparticle, such as a phonon, a roton or a magnon, is used in modern condensed matter physics to describe an elementary collective excitation. The intrinsic zero-temperature magnon damping in quantum spin systems can be driven by the interaction of the one-magnon states and multi-magnon continuum. However, detailed experimental studies on this quantum many-body effect induced by an applied magnetic field are rare. Here we present a high-resolution neutron scattering study in high fields on an S=1/2 antiferromagnet C9H18N2CuBr4. Compared with the non-interacting linear spin-wave theory, our results demonstrate a variety of phenomena including field-induced renormalization of one-magnon dispersion, spontaneous magnon decay observed via intrinsic linewidth broadening, unusual non-Lorentzian two-peak structure in the excitation spectra and a dramatic shift of spectral weight from one-magnon state to the two-magnon continuum.

5.
Phys Rev Lett ; 118(17): 177202, 2017 Apr 28.
Article in English | MEDLINE | ID: mdl-28498681

ABSTRACT

The challenge of one-dimensional systems is to understand their physics beyond the level of known elementary excitations. By high-resolution neutron spectroscopy in a quantum spin-ladder material, we probe the leading multiparticle excitation by characterizing the two-magnon bound state at zero field. By applying high magnetic fields, we create and select the singlet (longitudinal) and triplet (transverse) excitations of the fully spin-polarized ladder, which have not been observed previously and are close analogs of the modes anticipated in a polarized Haldane chain. Theoretical modeling of the dynamical response demonstrates our complete quantitative understanding of these states.

6.
Phys Rev Lett ; 115(20): 207202, 2015 Nov 13.
Article in English | MEDLINE | ID: mdl-26613467

ABSTRACT

A quantitative description of magnons in long-range ordered quantum antiferromagnets is presented which is consistent from low to high energies. It is illustrated for the generic S=1/2 Heisenberg model on the square lattice. The approach is based on a continuous similarity transformation in momentum space using the scaling dimension as the truncation criterion. Evidence is found for significant magnon-magnon attraction inducing a Higgs resonance. The high-energy roton minimum in the magnon dispersion appears to be induced by strong magnon-Higgs scattering.

7.
Article in English | MEDLINE | ID: mdl-26382355

ABSTRACT

We introduce a white-graph expansion for the method of perturbative continuous unitary transformations when implemented as a linked-cluster expansion. The essential idea behind an expansion in white graphs is to perform an optimized bookkeeping during the calculation by exploiting the model-independent effective Hamiltonian in second quantization and the associated inherent cluster additivity. This approach is shown to be especially well suited for microscopic models with many coupling constants, since the total number of relevant graphs is drastically reduced. The white-graph expansion is exemplified for a two-dimensional quantum spin model of coupled two-leg XXZ ladders.

8.
Phys Rev Lett ; 111(13): 137204, 2013 Sep 27.
Article in English | MEDLINE | ID: mdl-24116813

ABSTRACT

The magnetization process of the orthogonal-dimer antiferromagnet SrCu2(BO3)2 is investigated in high magnetic fields of up to 118 T. A 1/2 plateau is clearly observed in the field range 84 to 108 T in addition to 1/8, 1/4, and 1/3 plateaus at lower fields. Using a combination of state-of-the-art numerical simulations, the main features of the high-field magnetization, a 1/2 plateau of width 24 T, a 1/3 plateau of width 34 T, and no 2/5 plateau, are shown to agree quantitatively with the Shastry-Sutherland model if the ratio of inter- to intradimer exchange interactions J'/J=0.63. It is further predicted that the intermediate phase between the 1/3 and 1/2 plateaus is not uniform but consists of a 1/3 supersolid followed by a 2/5 supersolid and possibly a domain-wall phase, with a reentrance into the 1/3 supersolid above the 1/2 plateau.

9.
Phys Rev Lett ; 105(13): 137207, 2010 Sep 24.
Article in English | MEDLINE | ID: mdl-21230808

ABSTRACT

We study the magnetic-field-induced quantum phase transition from a gapped quantum phase that has no magnetic long-range order into a gapless phase in the spin-1/2 ladder compound bis(2,3-dimethylpyridinium) tetrabromocuprate (DIMPY). At temperatures below about 1 K, the specific heat in the gapless phase attains an asymptotic linear temperature dependence, characteristic of a Tomonaga-Luttinger liquid. Inelastic neutron scattering and the specific heat measurements in both phases are in good agreement with theoretical calculations, demonstrating that DIMPY is the first model material for an S=1/2 two-leg spin ladder in the strong-leg regime.


Subject(s)
Magnetics , Organometallic Compounds/chemistry , Pyridinium Compounds/chemistry , Quantum Theory , Spin Labels , Neutrons , Phase Transition , Scattering, Radiation
10.
Phys Rev Lett ; 101(25): 250402, 2008 Dec 19.
Article in English | MEDLINE | ID: mdl-19113683

ABSTRACT

Motivated by the remarkable properties of SrCu2(BO3) 2 in a magnetic field, we use perturbative continuous unitary transformations to determine the magnetization plateaux of the Shastry-Sutherland model, unveiling an unexpected sequence of plateaux progressively appearing at 2/9, 1/6, 1/9, and 2/15 upon increasing the interdimer coupling. We predict that a 1/6 plateau should be present in SrCu2(BO3)2, even if residual interactions beyond the Shastry-Sutherland are strong enough to modify the other plateaux below 1/3. The method is extended to calculate the magnetization profile within the plateaux, leading to a local structure around triplons that agrees with NMR results on SrCu2(BO3) 2.

11.
Phys Rev Lett ; 100(9): 090401, 2008 Mar 07.
Article in English | MEDLINE | ID: mdl-18352679

ABSTRACT

We show that correlated hopping of triplets, which is often the dominant source of kinetic energy in dimer-based frustrated quantum magnets, produces a remarkably strong tendency to form supersolid phases in a magnetic field. These phases are characterized by simultaneous modulation and ordering of the longitudinal and transverse magnetization, respectively. Using quantum Monte Carlo and a semiclassical approach for an effective hard-core boson model with nearest-neighbor repulsion on a square lattice, we prove, in particular, that a supersolid phase can exist even if the repulsion is not strong enough to stabilize an insulating phase at half-filling. Experimental implications for frustrated quantum antiferromagnets in a magnetic field at zero and finite temperature are discussed.

12.
Phys Rev Lett ; 98(2): 027403, 2007 Jan 12.
Article in English | MEDLINE | ID: mdl-17358648

ABSTRACT

We have performed inelastic neutron scattering on the near ideal spin-ladder compound La4Sr10Cu24O41 as a starting point for investigating doped ladders and their tendency toward superconductivity. A key feature was the separation of one-triplon and two-triplon scattering. Two-triplon scattering is observed quantitatively for the first time and so access is realized to the important strong magnetic quantum fluctuations. The spin gap is found to be 26.4+/-0.3 meV. The data are successfully modeled using the continuous unitary transformation method, and the exchange constants are determined by fitting to be Jleg=186 meV and Jrung=124 meV along the leg and rung, respectively; a substantial cyclic exchange of Jcyc=31 meV is confirmed.

13.
Phys Rev Lett ; 93(26 Pt 1): 267003, 2004 Dec 31.
Article in English | MEDLINE | ID: mdl-15698009

ABSTRACT

Based on a two-dimensional model of coupled two-leg spin ladders, we derive a unified picture of recent neutron scattering data of stripe-ordered La15/8Ba1/8CuO4, namely, of the low-energy magnons around the superstructure satellites and of the triplon excitations at higher energies. The resonance peak at the antiferromagnetic wave vector Q(AF) in the stripe-ordered phase corresponds to a saddle point in the dispersion of the magnetic excitations. Quantitative agreement with the neutron data is obtained for J=130-160 meV and Jcyc/J=0.2-0.25.

14.
Phys Rev Lett ; 90(16): 167201, 2003 Apr 25.
Article in English | MEDLINE | ID: mdl-12731999

ABSTRACT

In the two-leg S=1/2 ladders of Sr14Cu24O41, a modulation of the exchange coupling arises from the charge order within the other structural element, the CuO2 chains. In general, breaking transla-tional invariance by modulation causes gaps within the dispersion of elementary excitations. We show that the gap induced by the charge order can drastically change the magnetic Raman spectrum, leading to the sharp peak observed in Sr14Cu24O41. This sharp Raman line gives insight into the charge-order periodicity and hence into the distribution of carriers. The much broader spectrum of La6Ca8Cu24O41 reflects the response of an undoped ladder in the absence of charge order.

15.
Phys Rev Lett ; 87(16): 167204, 2001 Oct 15.
Article in English | MEDLINE | ID: mdl-11690239

ABSTRACT

Spectral densities are computed in unprecedented detail for quantum antiferromagnetic spin 1/2 two-leg ladders. These results were obtained due to a major methodical advance achieved by optimally chosen unitary transformations. The approach is based on dressed integer excitations. Considerable weight is found at high energies in the two-particle sector. Precursors of fractional spinon physics occur supporting the conclusion that there is no necessity to resort to fractional excitations in order to describe features at higher energies.

16.
Phys Rev Lett ; 87(12): 127002, 2001 Sep 17.
Article in English | MEDLINE | ID: mdl-11580541

ABSTRACT

Phonon-assisted two-magnon absorption is studied in the spin- 1/2 two-leg ladders of (Ca,La)(14)Cu(24)O(41) for E parallel c (legs) and E parallel a (rungs). We verify the theoretically predicted existence of two-magnon singlet bound states, which give rise to peaks at approximately equal to 2140 and 2800 cm(-1). The two-magnon continuum is observed at approximately equal to 4000 cm(-1). Two different theoretical approaches (Jordan-Wigner fermions and perturbation theory) describe the data very well for J parallel approximately equal to 1020-1100 cm(-1), J parallel/J perpendicular approximately equal to 1-1.2. At high energies, the magnetic contribution to sigma(omega) is strikingly similar in the ladders and in the undoped high-T(c) cuprates, which emphasizes the importance of strong quantum fluctuations in the latter.

17.
Radiobiol Radiother (Berl) ; 31(4): 361-71, 1990.
Article in German | MEDLINE | ID: mdl-2236524

ABSTRACT

Dose distributions of a combination from telecobalt-arc-therapy and afterloading-therapy for radiation therapy of gynecological cancers were calculated, using a computer program developed in our institute. Taking as a basis CT-scans the bone structures were taken into consideration like inhomogeneities. Conclusions about the individual dose on sensitive organs into the irradiated area like bladder and rectum become possible. The influence of changing parameters such like distance of axis of arc-therapy can be shown clearly.


Subject(s)
Brachytherapy , Genital Neoplasms, Female/radiotherapy , Radioisotope Teletherapy , Radiotherapy Planning, Computer-Assisted , Cobalt Radioisotopes/therapeutic use , Female , Genital Neoplasms, Female/diagnostic imaging , Humans , Tomography, X-Ray Computed
18.
Chronobiol Int ; 7(5-6): 463-5, 1990.
Article in English | MEDLINE | ID: mdl-2097079

ABSTRACT

Rubidium (Rb+) has an antidepressive effect and shortens the circadian period in animals, whereas Li+, another alcalic metal, lengthens it. When we treated a depressive Li+ nonresponder with Rb+, we found an improvement of depression as well as a phase advance of the temperature rhythm in relation to the rest-activity rhythm.


Subject(s)
Bipolar Disorder/drug therapy , Body Temperature/drug effects , Circadian Rhythm/drug effects , Rubidium/therapeutic use , Aged , Bipolar Disorder/physiopathology , Body Temperature/physiology , Circadian Rhythm/physiology , Drug Resistance , Female , Humans , Lithium/therapeutic use
19.
Radiobiol Radiother (Berl) ; 30(1): 69-76, 1989.
Article in German | MEDLINE | ID: mdl-2727284

ABSTRACT

For use in afterloading therapy there was constructed a special combination consisting of X-ray multiplier and a gynaecological table. Because of the constant magnification of radiographs topometric examinations became easier. Examining the displacement of points of interest when the patient is restored from a lithotomic position into a position with stretched legs we concluded that from the point of view of treatment planning it will be necessary to carry out afterloading irradiation with stretched legs like in the teletherapy. Only in such a way it is possible to calculate a common dose distribution of teletherapy and afterloading therapy.


Subject(s)
Brachytherapy/methods , Genital Neoplasms, Female/radiotherapy , Posture , Brachytherapy/instrumentation , Female , Humans
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