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1.
Chem Commun (Camb) ; 51(77): 14547, 2015 Oct 04.
Article in English | MEDLINE | ID: mdl-26346591

ABSTRACT

Correction for 'Quantum dot-imprinted polymers with size and shell-selective recognition properties' by S. Gam-Derouich et al., Chem. Commun., 2015, DOI: 10.1039/c5cc05203c.

2.
Chem Commun (Camb) ; 51(80): 14933-6, 2015 Oct 14.
Article in English | MEDLINE | ID: mdl-26307147

ABSTRACT

The emergence of nanotechnology has stimulated a great deal of research to detect engineered nanoparticles spread out in the environment. We address this issue here by designing quantum dot-imprinted polymers for the speciation of nanoparticles based on their size, shape and surface chemistry.

3.
Nano Lett ; 13(4): 1516-21, 2013 Apr 10.
Article in English | MEDLINE | ID: mdl-23461679

ABSTRACT

We experimentally demonstrate the control of the spontaneous emission rate and the radiation pattern of colloidal quantum dots deterministically positioned in a plasmonic patch antenna. The antenna consists of a thin gold microdisk separated from a planar gold layer by a few tens of nanometers thick dielectric layer. The emitters are shown to radiate through the entire patch antenna in a highly directional and vertical radiation pattern. Strong acceleration of spontaneous emission is observed, depending on the antenna geometry. Considering the double dipole structure of the emitters, this corresponds to a Purcell factor up to 80 for dipoles perpendicular to the disk.


Subject(s)
Colloids/chemistry , Gold/chemistry , Quantum Dots , Equipment Design , Light , Nanostructures/chemistry , Nanotechnology , Optics and Photonics , Surface Plasmon Resonance
4.
Philos Trans A Math Phys Eng Sci ; 369(1953): 4064-77, 2011 Oct 28.
Article in English | MEDLINE | ID: mdl-21930565

ABSTRACT

It is now recognized that the International System of Units (SI units) will be redefined in terms of fundamental constants, even if the date when this will occur is still under debate. Actually, the best estimate of fundamental constant values is given by a least-squares adjustment, carried out under the auspices of the Committee on Data for Science and Technology (CODATA) Task Group on Fundamental Constants. This adjustment provides a significant measure of the correctness and overall consistency of the basic theories and experimental methods of physics using the values of the constants obtained from widely differing experiments. The physical theories that underlie this adjustment are assumed to be valid, such as quantum electrodynamics (QED). Testing QED, one of the most precise theories is the aim of many accurate experiments. The calculations and the corresponding experiments can be carried out either on a boundless system, such as the electron magnetic moment anomaly, or on a bound system, such as atomic hydrogen. The value of fundamental constants can be deduced from the comparison of theory and experiment. For example, using QED calculations, the value of the fine structure constant given by the CODATA is mainly inferred from the measurement of the electron magnetic moment anomaly carried out by Gabrielse's group. (Hanneke et al. 2008 Phys. Rev. Lett. 100, 120801) The value of the Rydberg constant is known from two-photon spectroscopy of hydrogen combined with accurate theoretical quantities. The Rydberg constant, determined by the comparison of theory and experiment using atomic hydrogen, is known with a relative uncertainty of 6.6×10(-12). It is one of the most accurate fundamental constants to date. A careful analysis shows that knowledge of the electrical size of the proton is nowadays a limitation in this comparison. The aim of muonic hydrogen spectroscopy was to obtain an accurate value of the proton charge radius. However, the value deduced from this experiment contradicts other less accurate determinations. This problem is known as the proton radius puzzle. This new determination of the proton radius may affect the value of the Rydberg constant . This constant is related to many fundamental constants; in particular, links the two possible ways proposed for the redefinition of the kilogram, the Avogadro constant N(A) and the Planck constant h. However, the current relative uncertainty on the experimental determinations of N(A) or h is three orders of magnitude larger than the 'possible' shift of the Rydberg constant, which may be shown by the new value of the size of the proton radius determined from muonic hydrogen. The proton radius puzzle will not interfere in the redefinition of the kilogram. After a short introduction to the properties of the proton, we will describe the muonic hydrogen experiment. There is intense theoretical activity as a result of our observation. A brief summary of possible theoretical explanations at the date of writing of the paper will be given. The contribution of the proton radius puzzle to the redefinition of SI-based units will then be examined.

5.
Laryngorhinootologie ; 76(2): 57-64, 1997 Feb.
Article in German | MEDLINE | ID: mdl-9172631

ABSTRACT

BACKGROUND: Logatomes are nonsense syllables used for analyzing the confusion of phonemes by hearing impaired listeners. They can provide a precise differentiation of phonemic confusions which may be useful in the exact adjustment of programmable hearing aids. METHODS: In this study, two lists of logatomes with 108 three-sound combinations with a structure of consonant-vowel-consonant (c-v-c) and vowel-consonant-vowel (v-c-v) were recorded on a compact disk. Twenty normally hearing adults and 28 patients with a sensorineural hearing loss were tested at a comfortable listening level of about 25 +/- 5 dB above the mean audiometric thresholds at 0,5. 1,0 and 2,0 kHz. An index of reduction of speech perception was calculated. RESULTS: A significant relationship between reduction of logatome perception and pure-tone audiometric thresholds at 1,2,3, and 4 kHz was demonstrated. Moreover, it was possible to distinguish between different groups of hearing impairment. CONCLUSIONS: The logatome test helps to analyze specific effects that hearing loss can have on the recognition of acoustic speech signals. The logatome test may become a valuable addition to speech audiometric tests with further standardization.


Subject(s)
Audiometry, Speech/instrumentation , Hearing Aids , Hearing Loss, Sensorineural/diagnosis , Phonetics , Adult , Aged , Auditory Threshold , Equipment Design , Female , Hearing Loss, High-Frequency/diagnosis , Hearing Loss, High-Frequency/rehabilitation , Hearing Loss, Sensorineural/rehabilitation , Humans , Male , Middle Aged , Reference Values , Sensitivity and Specificity , Speech Acoustics
6.
Opt Lett ; 22(24): 1893-5, 1997 Dec 15.
Article in English | MEDLINE | ID: mdl-18188399

ABSTRACT

Nondegenerate optical parametric oscillators generate above-threshold signal and idler beams that have intensity fluctuations correlated at the quantum level (twin beams). We describe what is to our knowledge the first high-sensitivity spectroscopy experiment using twin beams emitted by a cw optical parametric oscillator: a very weak two-photon absorption signal, in the 10(-7) range, is recorded on the 4S(1/2)-5S(1/2) transition of atomic potassium with a noise background that is reduced by 1.9 dB with respect to the shot-noise limit of the light used in the experiment.

7.
Plant Physiol ; 57(5): 824-30, 1976 May.
Article in English | MEDLINE | ID: mdl-16659578

ABSTRACT

Euglena cells, strains Z and bacillaris, were grown in the dark under various nutritional deficiencies. After 3 days of nondivision, cells were transferred to the light, and the following parameters were measured: the paramylum content at the time of illumination (zero time), the rate of paramylum consumption during the first 10 hours of greening, and the length of the lag phase of chlorophyll synthesis. Similar results were obtained with both strains and can be summarized as follows. (a) The use of various nutritional deficiencies allows the control, to a certain extent, of the amount of paramylum present at zero time. (b) The rate of paramylum consumption is proportional to the cellular paramylum content for values in excess of 50 picograms/cell. (c) The length of the lag phase increases rapidly when the cellular content of paramylum decreases below 50 picograms. This period can be greatly diminished by the addition of an exogenous organíc carbon source. (d) The amount of paramylum (rate of paramylum consumption x length of lag phase) consumed during the lag phase is around 5 to 10 picograms/cell for cells which contain less than 50 picograms of paramylum/cell. It increases when the cellular paramylum content increases, this increment being more rapid for bacillaris than for Z cells.

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