Stability and instability for low refractive-index-contrast particle trapping in a dual-beam optical trap.

A dual-beam optical trap is used to trap and manipulate dielectric particles. When the refractive index of these particles is comparable to that of the surrounding medium, equilibrium trapping locations within the system shift from stable to unstable depending on fiber separation and particle size. This is due to to the relationship between gradient and scattering forces. We experimentally and computationally study the transitions between stable and unstable trapping of poly(methyl methacrylate) beads for a range of parameters relevant to experimental setups involving giant unilamellar vesicles. We present stability maps for various fiber separations and particle sizes, and find that careful attention to particle size and configuration is necessary to obtain reproducible quantitative results for soft matter stretching experiments.

Fiber-optic trap-on-a-chip platform for probing low refractive index contrast biomaterials.

Dual-beam fiber trapping is a versatile technique for manipulating microparticles. We fabricate and evaluate the performance of a compact trap-on-a-chip design and demonstrate, for what we believe is the first time, trapping of low-contrast (m<1.005) lipid vesicles in solution. Counterpropagating fibers are fixed along the chip channel, and we calibrate the trap by optically displacing polystyrene microspheres from the trap center. Measured scattering forces are ~30-49 pN from each beam. Stable trapping and reversible deformation of lipid vesicles is demonstrated under femtonewton trapping forces. This chip has applications in probing a variety of soft biomaterials, such as biological cells, lipid membranes, and protein assemblies.

Demonstration of nondegenerate spectrum reversal in optical-frequency regime.

This Letter reports theoretical and experimental studies of spectrum reversal with tunable wavelength offset in the optical-frequency regime-two widely separated spectral sidebands can always behave as mirror images of one another with respect to the center frequency of the controlling pump pulse. We call this interesting physical phenomenon "spectral mirror imaging."

Multimodal coherent anti-Stokes Raman spectroscopic imaging with a fiber optical parametric oscillator.

We report on multimodal coherent anti-Stokes Raman scattering (CARS) imaging with a source composed of a femtosecond fiber laser and a photonic crystal fiber (PCF)-based optical parametric oscillator (FOPO). By switching between two PCFs with different zero dispersion wavelengths, a tunable signal beam from the FOPO covering the range from 840 to 930 nm was produced. By combining the femtosecond fiber laser and the FOPO output, simultaneous CARS imaging of a myelin sheath and two-photon excitation fluorescence imaging of a labeled axons in rat spinal cord have been demonstrated at the speed of 20 µs per pixel.

Cross-phase-modulation-induced spectral effects in high-efficiency picosecond fiber optical parametric oscillators.

We explore the spectral effects due to cross-phase modulation and walk-off in picosecond fiber optical parametric oscillators. The output spectrum exhibits pump-power-dependent broadening, which can be quite asymmetric associated with a redshift or a blueshift depending on pump synchronization. By slightly increasing the cavity length, one obtains a blueshifted spectrum and a conversion efficiency as high as 15%.

Fiber optical parametric oscillator for sub-50 fs pulse generation: optimization of fiber length.

We demonstrate generation of 48fs pulses with linear chirp using a short (27mm) fiber optical parametric oscillator (FOPO), which is synchronously pumped by a mode-locked ytterbium-doped fiber laser. We also study the pulse quality for both the short- and long-wavelength operation where the fiber length inside of the oscillator varies from 17 to 61mm. The optimal pulse duration is observed only in the short-wavelength operation. Furthermore, we model the FOPO system as a single-pass parametric amplifier including dispersive pulse broadening and walk-off between the pump and output. The optimal condition arises from the minimization of the walk-off and dispersion. When walk-off is large, the parametric amplification process is most efficient over some reduced effective fiber length, leading to an upper limit in the amount of the observed pulse broadening.

Design and optimization of fiber optical parametric oscillators for femtosecond pulse generation.

In this paper, we use a genetic algorithm and pulse-propagation analysis to design and optimize optical parametric oscillators based on soft-glass microstructured optical fibers. The maximum parametric gain, phase-match, walk-off between pump (1560 nm) and signal (880 nm) pulses, signal feedback ratio and signal-pump synchronization of the cavity are optimized. Pulse propagation analysis suggests that one can implement a fiber optical parametric oscillator capable of generating approximately 200-fs pulses at 880 nm with 43% peak-power conversion, high output pulse quality (time-bandwidth product approximately 0.43) and a wavelength tuning range that is limited only by the glass transmission windows.

Microstructure fiber optical parametric oscillator with femtosecond output in the 1200 to 1350 nm wavelength range.

We describe an ultrafast fiber optical parametric oscillator operating in the 1210 nm to 1340 nm wavelength range. The system consists of a microstructure fiber placed in a Fabry-Perot cavity which is optically pumped with 1030-nm light from an Ytterbium mode-locked fiber laser. The output wavelength is tunable over a 130-nm span by adjusting the position of one cavity mirror. SHG FROG measurements reveal that the output pulse quality varies as a function of pump power and wavelength. Ultrafast sources operating in this range are particularly instrumental for deep-tissue nonlinear biophotonics applications.

Generation of sub-100-fs pulses from a microstructure-fiber-based optical parametric oscillator.

We report on the generation of 70-fs pulses at a center wavelength of 880 nm using a microstructure-fiber-based optical parametric oscillator pumped by a fiber laser operating at 1032 nm. We present optical spectra and autocorrelation measurements that illustrate the generation of ultrashort pulses and the onset of saturation at sufficiently high pump powers. Generation of ultrafast pulses with nanojoule energies provides new opportunities for extending the functionality of mode-locked fiber lasers.

Terahertz time-domain measurement of ballistic electron resonance in a single-walled carbon nanotube.

Understanding the physics of low-dimensional systems and the operation of next-generation electronics will depend on our ability to measure the electrical properties of nanomaterials at terahertz frequencies ( approximately 100 GHz to 10 THz). Single-walled carbon nanotubes are prototypical one-dimensional nanomaterials because of their unique band structure and long carrier mean free path. Although nanotube transistors have been studied at microwave frequencies (100 MHz to 50 GHz), no techniques currently exist to probe their terahertz response. Here, we describe the first terahertz electrical measurements of single-walled carbon nanotube transistors performed in the time domain. We observe a ballistic electron resonance that corresponds to the round-trip transit of an electron along the nanotube with a picosecond-scale period. The electron velocity is found to be constant and equal to the Fermi velocity, showing that the high-frequency electron response is dominated by single-particle excitations rather than collective plasmon modes. These results demonstrate a powerful new tool for directly probing picosecond electron motion in nanostructures.

Octave-spanning, high-power microstructure-fiber-based optical parametric oscillators.

We investigate femtosecond optical parametric oscillators (OPO's) based on short pieces of microstructure fiber that generate sub-picosecond pulses with record average output power (50 mW) and >200 nm of wavelength tunability (yellow to near-IR). Signal and conjugate (idler)fields spanning an octave are also demonstrated. These systems can operate with a wide range of microstructure fibers, pump laser wavelengths and pulse durations, and our analysis shows that in terms of wavelength tunability and output power using short (less than a few cm's) optical fibers leads to performance that is superior to that with longer lengths.

Broad-band optical parametric gain on a silicon photonic chip.

Developing an optical amplifier on silicon is essential for the success of silicon-on-insulator (SOI) photonic integrated circuits. Recently, optical gain with a 1-nm bandwidth was demonstrated using the Raman effect, which led to the demonstration of a Raman oscillator, lossless optical modulation and optically tunable slow light. A key strength of optical communications is the parallelism of information transfer and processing onto multiple wavelength channels. However, the relatively narrow Raman gain bandwidth only allows for amplification or generation of a single wavelength channel. If broad gain bandwidths were to be demonstrated on silicon, then an array of wavelength channels could be generated and processed, representing a critical advance for densely integrated photonic circuits. Here we demonstrate net on/off gain over a wavelength range of 28 nm through the optical process of phase-matched four-wave mixing in suitably designed SOI channel waveguides. We also demonstrate wavelength conversion in the range 1,511-1,591 nm with peak conversion efficiencies of +5.2 dB, which represents more than 20 times improvement on previous four-wave-mixing efficiencies in SOI waveguides. These advances allow for the implementation of dense wavelength division multiplexing in an all-silicon photonic integrated circuit. Additionally, all-optical delays, all-optical switches, optical signal regenerators and optical sources for quantum information technology, all demonstrated using four-wave mixing in silica fibres, can now be transferred to the SOI platform.

All-optical slow-light on a photonic chip.

We demonstrate optically tunable delays in a silicon-on-insulator planar waveguide based on slow light induced by stimulated Raman scattering (SRS). Inside an 8-mm-long nanoscale waveguide, we produce a group-index change of 0.15 and generate controllable delays as large as 4 ps for signal pulses as short as 3 ps. The scheme can be implemented at bandwidths exceeding 100 GHz for wavelengths spanning the entire low-loss fiber-optics communications window and thus represents an important step in the development of chip-scale photonics devices that process light with light.

Tailored anomalous group-velocity dispersion in silicon channel waveguides.

We present the first experimental demonstration of anomalous group-velocity dispersion (GVD) in silicon waveguides across the telecommunication bands. We show that the GVD in such waveguides can be tuned from -2000 to 1000 ps/(nm*km) by tailoring the cross-sectional size and shape of the waveguide.

Large tunable optical delays via self-phase modulation and dispersion.

We demonstrate all-optically tunable delays in optical fiber via a dispersive stage and two stages of nonlinear spectral broadening and filtering. With this scheme, we achieve continuously tunable delays of 3.5- ps pulses and advancements over a total range of more than 1200 pulsewidths. Our technique is applicable to a wide range of pulse durations and delays.

Generation of correlated photons in nanoscale silicon waveguides.

.We experimentally study the generation of correlated pairs of photons through four-wave mixing (FWM) in embedded silicon waveguides. The waveguides, which are designed to exhibit anomalous group-velocity dispersion at wavelengths near 1555 nm, allow phase matched FWM and thus efficient pair-wise generation of non-degenerate signal and idler photons. Photon counting measurements yield a coincidence-to-accidental ratio (CAR) of around 25 for a signal (idler) photon production rate of about 0.05 per pulse. We characterize the variation in CAR as a function of pump power and pump-to-sideband wavelength detuning. These measurements represent a first step towards the development of tools for quantum information processing which are based on CMOS-compatible, silicon-on-insulator technology.

Storage and long-distance distribution of telecommunications-band polarization entanglement generated in an optical fiber.

We demonstrate storage of polarization-entangled photons for 125 micros, a record storage time to date, in a 25-km-long fiber spool, using a telecommunications-band fiber-based source of entanglement. With this source we also demonstrate distribution of polarization entanglement over 50 km by separating the two photons of an entangled pair and transmitting them individually over separate 25-km fibers. The measured two-photon fringe visibilities were 82% in the storage experiment and 86% in the distribution experiment. Preservation of polarization entanglement over such long-distance transmission demonstrates the viability of all-fiber sources for use in quantum memories and quantum logic gates.

Tunable all-optical delays via Brillouin slow light in an optical fiber.

We demonstrate a technique for generating tunable all-optical delays in room temperature single-mode optical fibers at telecommunication wavelengths using the stimulated Brillouin scattering process. This technique makes use of the rapid variation of the refractive index that occurs in the vicinity of the Brillouin gain feature. The wavelength at which the induced delay occurs is broadly tunable by controlling the wavelength of the laser pumping the process, and the magnitude of the delay can be tuned continuously by as much as 25 ns by adjusting the intensity of the pump field. The technique can be applied to pulses as short as 15 ns. This scheme represents an important first step towards implementing slow-light techniques for various applications including buffering in telecommunication systems.

Optical-fiber source of polarization-entangled photons in the 1550 nm telecom band.

We present a fiber-based source of polarization-entangled photons that is well suited for quantum communication applications in the 1550 nm band of standard fiber-optic telecommunications. Polarization entanglement is created by pumping a nonlinear-fiber Sagnac interferometer with two time-delayed orthogonally polarized pump pulses and subsequently removing the time distinguishability by passing the parametrically scattered signal and idler photon pairs through a piece of birefringent fiber. Coincidence detection of the signal and idler photons yields biphoton interference with visibility greater than 90%, while no interference is observed in direct detection of either signal or idler photons. All four Bell states can be prepared with our setup and we demonstrate violations of the Clauser-Horne-Shimony-Holt form of Bell's inequality by up to 10 standard deviations of measurement uncertainty.

Resonant optical interactions with molecules confined in photonic band-gap fibers.

We investigate resonant nonlinear optical interactions and demonstrate induced transparency in acetylene molecules in a hollow-core photonic-band-gap fiber at 1.5 mum. The induced spectral transmission window is used to demonstrate slow-light effects, and we show that the observed broadening of the spectral features is due to collisions of the molecules with the inner walls of the fiber core. Our results illustrate that such fibers can be used to facilitate strong coherent light-matter interactions even when the optical response of the individual molecules is weak.