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1.
Nat Commun ; 15(1): 5063, 2024 Jun 13.
Article in English | MEDLINE | ID: mdl-38871708

ABSTRACT

Levitated diamond particles in high vacuum with internal spin qubits have been proposed for exploring macroscopic quantum mechanics, quantum gravity, and precision measurements. The coupling between spins and particle rotation can be utilized to study quantum geometric phase, create gyroscopes and rotational matter-wave interferometers. However, previous efforts in levitated diamonds struggled with vacuum level or spin state readouts. To address these gaps, we fabricate an integrated surface ion trap with multiple stabilization electrodes. This facilitates on-chip levitation and, for the first time, optically detected magnetic resonance measurements of a nanodiamond levitated in high vacuum. The internal temperature of our levitated nanodiamond remains moderate at pressures below 10-5 Torr. We have driven a nanodiamond to rotate up to 20 MHz (1.2 × 109 rpm), surpassing typical nitrogen-vacancy (NV) center electron spin dephasing rates. Using these NV spins, we observe the effect of the Berry phase arising from particle rotation. In addition, we demonstrate quantum control of spins in a rotating nanodiamond. These results mark an important development in interfacing mechanical rotation with spin qubits, expanding our capacity to study quantum phenomena.

2.
Nano Lett ; 23(22): 10157-10163, 2023 Nov 22.
Article in English | MEDLINE | ID: mdl-37909774

ABSTRACT

A levitated nonspherical nanoparticle in a vacuum is ideal for studying quantum rotations and is an ultrasensitive torque detector for probing fundamental particle-surface interactions. Here, we optically levitate a silica nanodumbbell in a vacuum at 430 nm away from a sapphire surface and drive it to rotate at GHz frequencies. The relative linear speed between the tip of the nanodumbbell and the surface reaches 1.4 km s-1 at a submicrometer separation. The rotating nanodumbbell near the surface demonstrates a torque sensitivity of (5.0 ± 1.1) × 10-26 N m Hz-1/2 at room temperature. Moreover, we probed the near-field laser intensity distribution beyond the optical diffraction limit with a nanodumbbell levitated near a nanograting. Our numerical simulations show that the system can measure the Casimir torque and will improve the detection limit of non-Newtonian gravity by several orders of magnitude.

3.
Nat Commun ; 13(1): 6148, 2022 Oct 18.
Article in English | MEDLINE | ID: mdl-36257958

ABSTRACT

A remarkable prediction of quantum field theory is that there are quantum electromagnetic fluctuations (virtual photons) everywhere, which leads to the intriguing Casimir effect. While the Casimir force between two objects has been studied extensively for several decades, the Casimir force between three objects has not been measured yet. Here, we report the experimental demonstration of an object under the Casimir force exerted by two other objects simultaneously. Our Casimir system consists of a micrometer-thick cantilever placed in between two microspheres, forming a unique sphere-plate-sphere geometry. We also propose and demonstrate a three-terminal switchable architecture exploiting opto-mechanical Casimir interactions that can lay the foundations of a Casimir transistor. Beyond the paradigm of Casimir forces between two objects in different geometries, our Casimir transistor represents an important development for controlling three-body virtual photon interactions and will have potential applications in sensing and information processing.

4.
Nat Mater ; 21(9): 1024-1028, 2022 Sep.
Article in English | MEDLINE | ID: mdl-35970964

ABSTRACT

Electron spins in van der Waals materials are playing a crucial role in recent advances in condensed-matter physics and spintronics. However, nuclear spins in van der Waals materials remain an unexplored quantum resource. Here we report optical polarization and coherent control of nuclear spins in a van der Waals material at room temperature. We use negatively charged boron vacancy ([Formula: see text]) spin defects in hexagonal boron nitride to polarize nearby nitrogen nuclear spins. We observe the Rabi frequency of nuclear spins at the excited-state level anti-crossing of [Formula: see text] defects to be 350 times larger than that of an isolated nucleus, and demonstrate fast coherent control of nuclear spins. Further, we detect strong electron-mediated nuclear-nuclear spin coupling that is five orders of magnitude larger than the direct nuclear-spin dipolar coupling, enabling multi-qubit operations. Our work opens new avenues for the manipulation of nuclear spins in van der Waals materials for quantum information science and technology.

5.
Nano Lett ; 21(18): 7708-7714, 2021 Sep 22.
Article in English | MEDLINE | ID: mdl-34473524

ABSTRACT

The recently discovered spin defects in hexagonal boron nitride (hBN), a layered van der Waals material, have great potential in quantum sensing. However, the photoluminescence and the contrast of the optically detected magnetic resonance (ODMR) of hBN spin defects are relatively low so far, which limits their sensitivity. Here we report a record-high ODMR contrast of 46% at room temperature and simultaneous enhancement of the photoluminescence of hBN spin defects by up to 17-fold by the surface plasmon of a gold film microwave waveguide. Our results are obtained with shallow boron vacancy spin defects in hBN nanosheets created by low-energy He+ ion implantation and a gold film microwave waveguide fabricated by photolithography. We also explore the effects of microwave and laser powers on the ODMR and improve the sensitivity of hBN spin defects for magnetic field detection. Our results support the promising potential of hBN spin defects for nanoscale quantum sensing.

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