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1.
Adv Mater ; 36(19): e2311339, 2024 May.
Article in English | MEDLINE | ID: mdl-38324142

ABSTRACT

SrTiO3 (STO) substrate, a perovskite oxide material known for its high dielectric constant (ɛ), facilitates the observation of various (high-temperature) quantum phenomena. A quantum Hall topological insulating (QHTI) state, comprising two copies of QH states with antiparallel two ferromagnetic edge-spin overlap protected by the U(1) axial rotation symmetry of spin polarization, has recently been achieved in low magnetic field (B) even as high as ≈100 K in a monolayer graphene/thin hexagonal boron nitride (hBN) spacer placed on an STO substrate, thanks to the high ɛ of STO. Despite the use of the heavy STO substrate, however, proximity-induced quantum spin Hall (QSH) states in 2D TI phases, featuring a topologically protected helical edge spin phase within time-reversal-symmetry, is not confirmed. Here, with the use of a monolayer hBN spacer, it is revealed the coexistence of QSH (at B = 0T) and QHTI (at B ≠ 0) states in the same single graphene sample placed on an STO, with a crossover regime between the two at low B. It is also classified that the different symmetries of the two nontrivial helical edge spin phases in the two states lead to different interaction with electron-puddle quantum dots, caused by a local surface pocket of the STO, in the crossover regime, resulting in a spin dephasing only for the QHTI state. The results obtained using STO substrates open the doors to investigations of novel QH spin states with different symmetries and their correlations with quantum phenomena. This exploration holds value for potential applications in spintronic devices.

2.
Phys Rev Lett ; 130(13): 136301, 2023 Mar 31.
Article in English | MEDLINE | ID: mdl-37067327

ABSTRACT

The concept of Berry curvature is essential for various transport phenomena. However, an effect of the Berry curvature on magnetochiral anisotropy, i.e., nonreciprocal magnetotransport, is still elusive. Here, we report that the Berry curvature induces the large magnetochiral anisotropy. In Weyl semimetal WTe_{2}, we observe the strong enhancement of the magnetochiral anisotropy when the Fermi level is located near the Weyl points. Notably, the maximal figure of merit γ[over ¯] reaches 1.2×10^{-6} m^{2} T^{-1} A^{-1}, which is the largest ever reported in bulk materials. Our semiclassical calculation shows that the diverging Berry curvature at the Weyl points strongly enhances the magnetochiral anisotropy.

4.
Sci Rep ; 13(1): 1922, 2023 Feb 02.
Article in English | MEDLINE | ID: mdl-36732549

ABSTRACT

Skyrmions, topologically stable spin structures with particle-like properties, are promising for spintronics applications such as skyrmion racetrack memory. Though reliable control of skyrmion motion is essential for the operation of spintronics devices, the straight motion of skyrmions along the driving force is in general difficult due to an inevitable transverse force originating from their topology. Here, we propose a method of precise manipulation of skyrmions based on surface acoustic waves (SAWs) propagating in two dimensions. Using two standing SAWs, saddle-shape local potentials like quadrupole ion traps are created to trap skyrmions robustly. Furthermore, by tuning the frequencies of the SAWs, we show that trapped skyrmions not only move in straight lines but also move precisely in any direction in a two-dimensional thin film. These results could be helpful for the future design of spintronics devices based on skyrmions.

5.
ACS Nano ; 17(3): 1916-1924, 2023 Feb 14.
Article in English | MEDLINE | ID: mdl-36700561

ABSTRACT

Stacking order is expected to have a significant impact on the properties of van der Waals layered magnets, as it determines the crystallographic and magnetic symmetry. Recent synchrotron-based optical studies on antiferromagnetic MnPS3 have revealed a thickness-dependent symmetry crossover, suggesting possible different stackings in few-layer crystals from the bulk, which, however, has not been explicitly identified. Here, by using a combination of atomic-scale electron microscopy and theoretical calculations, we show that despite the bulk monoclinic stacking persists macroscopically down to bilayer, additional local rippling effect lifts the monoclinic symmetry of the few layers while preserving the trigonal symmetry of individual monolayers, leading to possible monolayer-like behavior in ultrathin MnPS3 samples. This finding reveals the profound impact of rippling on the microscopic symmetry of two-dimensional materials with weak interlayer interactions and raises the possibility of approaching the paradigmatic two-dimensional Néel antiferromagnetic honeycomb lattice in MnPS3 without reaching monolayer thickness.

6.
Sci Adv ; 8(39): eabq5652, 2022 Sep 30.
Article in English | MEDLINE | ID: mdl-36179033

ABSTRACT

Nonlinear phenomena in physical systems can be used for brain-inspired computing with low energy consumption. Response from the dynamics of a topological spin structure called skyrmion is one of the candidates for such a neuromorphic computing. However, its ability has not been well explored experimentally. Here, we experimentally demonstrate neuromorphic computing using nonlinear response originating from magnetic field-induced dynamics of skyrmions. We designed a simple-structured skyrmion-based neuromorphic device and succeeded in handwritten digit recognition with the accuracy as large as 94.7% and waveform recognition. Notably, there exists a positive correlation between the recognition accuracy and the number of skyrmions in the devices. The large degrees of freedom of skyrmion systems, such as the position and the size, originate from the more complex nonlinear mapping, the larger output dimension, and, thus, high accuracy. Our results provide a guideline for developing energy-saving and high-performance skyrmion neuromorphic computing devices.

7.
Sci Rep ; 11(1): 24216, 2021 Dec 20.
Article in English | MEDLINE | ID: mdl-34930965

ABSTRACT

Peltier effects, which produce a heat flux at the junction of two different materials, have been an important technology for heating and cooling by electrical means. Whereas Peltier devices have advantages such as cleanliness, silence, compactness, flexibility, reliability, and efficiency, relatively complicated modular structures are unavoidable, leading to a higher cost than that of commonly used refrigeration technology. Here, we provide a concept of a Peltier device composed of a single magnetic material exhibiting a first-order magnetic transition. Our concept is based on a controllable junction structure consisting of two magnetic phases with opposite Peltier coefficients instead of a semiconductor junction. Using [Formula: see text] samples with the first-order magnetic transition between ferrimagnetic (FI) and antiferromagnetic (AF) states, we successfully made a stable junction structure of AF/FI/AF by a pulse heating method and achieved a maximum Peltier coefficient of 0.58 mV. Our device concept was further verified by a numerical simulation based on a finite element method. The single-material Peltier effect reported here avoids a complex device design involving material junctions and is importantly reconfigurable.

8.
Nat Commun ; 12(1): 5199, 2021 08 31.
Article in English | MEDLINE | ID: mdl-34465792

ABSTRACT

A triplon refers to a fictitious particle that carries angular momentum S=1 corresponding to the elementary excitation in a broad class of quantum dimerized spin systems. Such systems without magnetic order have long been studied as a testing ground for quantum properties of spins. Although triplons have been found to play a central role in thermal and magnetic properties in dimerized magnets with singlet correlation, a spin angular momentum flow carried by triplons, a triplon current, has not been detected yet. Here we report spin Seebeck effects induced by a triplon current: triplon spin Seebeck effect, using a spin-Peierls system CuGeO3. The result shows that the heating-driven triplon transport induces spin current whose sign is positive, opposite to the spin-wave cases in magnets. The triplon spin Seebeck effect persists far below the spin-Peierls transition temperature, being consistent with a theoretical calculation for triplon spin Seebeck effects.

9.
Sci Rep ; 10(1): 7574, 2020 May 05.
Article in English | MEDLINE | ID: mdl-32372015

ABSTRACT

Magneto-piezoelectric effect (MPE) refers to generation of strain in response to electric currents in magnetic metals which lack both time-reversal and space-inversion symmetries. A recent experimental paper demonstrated the MPE in the antiferromagnetic metal EuMnBi2 at 77 K, but the limited temperature range of the MPE measurement hampered detailed discussion on the MPE. Here we extend the measurement temperature range down to liquid He temperature, and studied the dependences of the MPE on the laser position, frequency and amplitude of electric currents, and temperature in the very low temperature range. We show that the MPE signal is enhanced at low temperatures and reaches a maximum magnitude in the antiferromagnetically ordered states of both Eu and Mn ions. An effective piezoelectric coefficient for the MPE at 4.5 K is estimated to be as large as 3500 pC/N, which is much larger than piezoelectric coefficients of typical piezoelectric ceramics, although the magnitude of real MPE displacements should be limited due to strong Joule heating at high electric currents. The present results may open up a new strategy to realize new lead-free piezoelectric materials.

10.
Sci Rep ; 9(1): 19052, 2019 Dec 13.
Article in English | MEDLINE | ID: mdl-31836771

ABSTRACT

In superconductors, a topological configuration of the superconducting order parameter called a superconducting vortex carries magnetization. Such a magnetic topological object behaves like a minute particle generating a magnetic flux. Since the flux is localized with a nanometer scale, the vortex provides a nano-scale probe for local magnetic fields. Here we show that information of magnetic stripes in insulators can be read out by using vortices in an adjacent superconductor film as a probe. The orientation and width of magnetic micro stripes are both transcribed into resistance change of the superconductor through the modulation of vortex mobility affected by local magnetization. By changing the direction of external magnetic fields, zero-field resistance changes continuously according to the stripe orientation, and its modulation magnitude reaches up to 100%. The width of the stripes can also be estimated from the oscillatory magnetoresistance. Our results demonstrate a new possibility for non-volatile analog memory devices based on topological objects.

11.
Phys Rev Lett ; 123(11): 117202, 2019 Sep 13.
Article in English | MEDLINE | ID: mdl-31573271

ABSTRACT

Investigating exotic magnetic materials with spintronic techniques is effective at advancing magnetism as well as spintronics. In this work, we report unusual field-induced suppression of the spin Seebeck effect (SSE) in a quasi-one-dimensional frustrated spin-1/2 magnet LiCuVO_{4}, known to exhibit spin-nematic correlation in a wide range of external magnetic field B. The suppression takes place above |B|≳2 T in spite of the B-linear isothermal magnetization curves in the same B range. The result can be attributed to the growth of the spin-nematic correlation while increasing B. The correlation stabilizes magnon pairs carrying spin 2, thereby suppressing the interfacial spin injection of SSE by preventing the spin-1 exchange between single magnons and conduction electrons at the interface. This interpretation is supported by integrating thermodynamic measurements and theoretical analysis on the SSE.

12.
Nat Commun ; 10(1): 2616, 2019 06 13.
Article in English | MEDLINE | ID: mdl-31197177

ABSTRACT

Electric current has been used to send electricity to far distant places. On the other hand, spin current, a flow of electron spin, can in principle also send angular momentum to distant places. In a magnet, there is a universal spin carrier called a spin wave, a wave-type excitation of magnetization. Since spin waves exhibit a long propagation length, it should be able to send angular momentum that can generate torque and force at a distant place: a new function of magnets. Here we observe mechanical angular momentum transmission and force generation due to spin waves injected into Y3Fe5O12 by the spin-Seebeck effect. The spin-wave current, transmitted through a Y3Fe5O12 micro cantilever, was found to create a mechanical force on the cantilever as a non-local reaction of the spin-Seebeck effect. Spin-wave current can be generated remotely even in open circuits, and it can be used to drive micro mechanical devices.

14.
Sci Rep ; 7(1): 4576, 2017 07 04.
Article in English | MEDLINE | ID: mdl-28676629

ABSTRACT

Spin pumping enables the generation of d.c. and gigahertz-band (GHz-band) voltages from an applied microwave via magnetization dynamics when combined with inverse spin Hall effects. However, generating such voltages in the in-between frequency region, or the megahertz (MHz) band, has been difficult since ferromagnetic resonance usually occurs in the GHz band. Here we show that in spite of GHz-band microwaves applied, MHz-band voltages can be generated by spin pumping with use of nonlinear magnetization dynamics in Y3Fe5O12. The mechanism is ascribed to the MHz-band oscillation of the amplitude of the magnetization precession, which is projected onto a rectified voltage component via spin pumping. The present finding could be useful for frequency down-conversion thanks to the simple and durable structure, continuous-wave operation, and the tunability of an output frequency with low magnetic fields.

15.
Biosci Biotechnol Biochem ; 78(1): 60-6, 2014.
Article in English | MEDLINE | ID: mdl-25036484

ABSTRACT

Ascorbate (AsA) is an important antioxidant and an enzyme cofactor involved in various metabolic pathways. In this study, we investigated the effects of estrogen (ES)-inducible transient expression of genes encoding enzymes involved in the d-mannose/l-galactose (d-Man/l-Gal) pathway for plant AsA biosynthesis on AsA levels under light and dark conditions. No significant difference was observed in AsA levels between Arabidopsis plants transiently expressing phosphomannose isomerase (PMI1), GDP-d-Man pyrophosphorylase (GMP/VTC1), GDP-Man-3',5'-epimerase (GME), and l-Gal 1-phosphate phosphatase (GPP/VTC4), but AsA levels in the plants transiently expressing GDP-l-Gal phosphorylase (GGP/VTC2) were 2.5-fold higher than those in control plants 7 d after ES treatment. The increase in AsA levels under continuous light conditions and the decrease in AsA levels under dark conditions were enhanced and suppressed, respectively, in the ES-treated plants. These results suggest that GGP/VTC2 acts as a rate-limiting step regulating AsA biosynthesis in response to light and dark conditions.


Subject(s)
Arabidopsis Proteins/genetics , Arabidopsis/genetics , Arabidopsis/metabolism , Ascorbic Acid/biosynthesis , Darkness , Gene Expression Regulation, Plant , Phosphoric Monoester Hydrolases/genetics , Arabidopsis/enzymology , Arabidopsis/radiation effects , Arabidopsis Proteins/metabolism , Ascorbic Acid/metabolism , Biocatalysis , Estrogens/pharmacology , Gene Expression Regulation, Plant/drug effects , Gene Expression Regulation, Plant/radiation effects , Intracellular Space/drug effects , Intracellular Space/metabolism , Intracellular Space/radiation effects , Phosphoric Monoester Hydrolases/metabolism
17.
Nihon Shokakibyo Gakkai Zasshi ; 104(1): 57-63, 2007 Jan.
Article in Japanese | MEDLINE | ID: mdl-17230008

ABSTRACT

We present the case of a 67-year-old man with primary malignant fibrous histiocytoma (MFH) of the diaphragm. He was admitted to our hospital with anorexia and loss of body weight. High serum levels of AST, ALT, ALP and gamma-GTP were observed. Several imaging studies disclosed a large tumor on the right side of the diaphragm to the right lobe of the liver. The entire tumor was resected, and histopathological examination of the specimen revealed the characteristics of MFH. MFH originating from the diaphragm is very rare, and we present the case of this patient in addition to a discussion of previous literature.


Subject(s)
Diaphragm/pathology , Histiocytoma, Malignant Fibrous/diagnosis , Histiocytoma, Malignant Fibrous/pathology , Liver Function Tests , Liver Neoplasms/diagnosis , Liver Neoplasms/pathology , Muscle Neoplasms/pathology , Aged , Diagnostic Imaging , Diaphragm/surgery , Histiocytoma, Malignant Fibrous/surgery , Humans , Liver Neoplasms/surgery , Male , Muscle Neoplasms/diagnosis , Muscle Neoplasms/surgery , Neoplasm Invasiveness
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