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1.
Sci Rep ; 11(1): 19144, 2021 Sep 27.
Article in English | MEDLINE | ID: mdl-34580344

ABSTRACT

We describe the collective behavior of isotropic droplets dispersed over a spherical smectic bubble, observed under microgravity conditions on the International Space Station (ISS). We find that droplets can form two-dimensional hexagonal structures changing with time. Our analysis indicates the possibility of spatial and temporal periodicity of such structures of droplets. Quantitative analysis of the hexagonal structure including the first three coordination circles was performed. A peculiar periodic-in-time ordering of the droplets, related to one-dimensional motion of droplets with non-uniform velocity, was found.

2.
Soft Matter ; 16(36): 8506-8511, 2020 Sep 23.
Article in English | MEDLINE | ID: mdl-32840550

ABSTRACT

In free-standing smectic films islands (regions of larger thickness than the film) can be considered as two-dimensional analogues of liquid droplets in a three-dimensional medium. The dynamics of droplet coalescence is an important but up to now incompletely solved problem in non-equilibrium mechanics. Here, we report on our investigations of island coalescence with the film meniscus. This phenomenon is analogous to the coalescence of a 3D droplet with a flat liquid surface. We found that the time evolution of island dimension is described by universal power-law dependencies for different stages of coalescence. Limited agreement with existing theory was found. In particular, in the final stage of coalescence the domain dynamics differs from theoretical predictions.

3.
Phys Rev E ; 101(5-1): 052701, 2020 May.
Article in English | MEDLINE | ID: mdl-32575317

ABSTRACT

We investigate in free-standing smectic films coalescence of holes (circular regions with thickness smaller than the surrounding film). This process can be considered as a two-dimensional analog of coalescence of bubbles in a three-dimensional fluid. A high speed video camera was used to study the evolution of domains at different stages of coalescence. Special attention was given to investigations of the dependence of the size of the bridge between two holes at the initial stage of coalescence, which was considered in numerous theoretical works and bears information on the coalescence mechanism. It is established that the scaling law is applicable for the description of the transformation of bridges for holes of different radius R. We found that in the regime corresponding to the experimental situation the length of the bridge H increases with the scaling law H/R=(t/τ_{R})^{1/2}. The characteristic time τ_{R} determined from the scaling law is larger than the theoretical time, which can be connected with dissipation of energy both in the film and inside the holes.

4.
Phys Rev E ; 100(1-2): 019901, 2019 Jul.
Article in English | MEDLINE | ID: mdl-31499913

ABSTRACT

This corrects the article DOI: 10.1103/PhysRevE.99.062702.

5.
Phys Rev E ; 99(6-1): 062702, 2019 Jun.
Article in English | MEDLINE | ID: mdl-31330683

ABSTRACT

Freestanding smectic films give a unique possibility to study two-dimensional coalescence. We report experimental investigations in freestanding films and detailed analysis of coalescence of islands, circular regions of larger thickness than the surrounding film. The driving force of island coalescence is the dislocation tension on the boundary between the island and the film. The obtained experimental results enable one to perform complex analysis of two-dimensional coalescence in Stokes regime and compare it to theoretical predictions. The applicability of scaling arguments for the description of the peculiarities of domain dynamics is demonstrated. The whole process of coalescence is well described by the analytical solution adapted to our case of islands in freestanding smectic films.

6.
Phys Rev E ; 95(1-1): 012711, 2017 Jan.
Article in English | MEDLINE | ID: mdl-28208509

ABSTRACT

We report imaging of the director field near edge dislocations in thermotropic antiferroelecric smectic-C_{A}^{*} (SmC_{A}^{*}) liquid crystal. Measurements were made in freestanding films with thickness from two to ten smectic layers. We find two different orientations of the molecular tilt plane with respect to the edge dislocation line. The orientation is determined by the value of the Burgers vector of the dislocation. Elementary edge dislocation and dislocations with a Burgers vector equal to an odd number of layers orient the tilt plane perpendicular on the two sides of the dislocation. Dislocations with a Burgers vector equal to an even number of layers orient the molecular tilt plane parallel to the dislocation line. Difference in the orientation for an odd Burgers vector can be attributed to breaking of antiferroelectric symmetry by the edge dislocation.

7.
Phys Rev E ; 93(3): 032704, 2016 Mar.
Article in English | MEDLINE | ID: mdl-27078424

ABSTRACT

A two-dimensional hexagonal smectic structure formed by point topological defects and intersecting defect walls was discovered. This unique structure was predicted theoretically about 30 years ago but not observed. For a long time the hexagonal structure was a challenge for experimentalists. A different type of self-organization in smectic films was found and used to form the hexagonal structure. Methods applied for building the hexagonal phase can be used for the formation of complicated liquid-crystal structures.

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