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1.
Appl Opt ; 45(20): 4947-56, 2006 Jul 10.
Article in English | MEDLINE | ID: mdl-16807604

ABSTRACT

A saturable-absorber-based technique for spatial filtering of high-average-power laser beams is described. For a focused, radially symmetric beam having its highest intensity at the center, this saturable absorber behaves like a soft aperture with gradually increasing attenuation toward the beam edges, thus selectively transmitting the low divergence components that are confined close to the central axis of the propagating laser beam. This technique has been successfully used to reduce the divergence of a high-power, high-repetition-rate, tunable, narrowband, pulsed dye laser. Our results demonstrate how a judicious choice of operating parameters allows spatial filtering to be achieved with the introduction of a minimum absorption loss of the laser beam in the saturable absorber. Following a time-dependent analysis of a rate equation model describing the propagation and interaction of the laser beam with the saturable absorber, we have also obtained theoretical estimates for the extent of spatial filtering. Our theoretical estimates have been found to be in good agreement with our experimental observations.

2.
Appl Opt ; 44(36): 7814-22, 2005 Dec 20.
Article in English | MEDLINE | ID: mdl-16381533

ABSTRACT

The lasing and photostability characteristics of Rhodamine 6G and Pyrromethene 567 dyes dispersed in polymeric host materials have been investigated as a function of the intensities of incident pump and signal beams in a longitudinally pumped dye laser in an oscillator-amplifier configuration. A substantial reduction in the rate of photodegradation was observed under lasing conditions and with increasing signal intensity in a dye amplifier, establishing that the service lives of these materials improve with an increase in the rate of stimulated emission. We observed approximately 62% amplifier efficiency at 2 Hz operation and 10% reduction in amplifier efficiency at 10 Hz operation after exposure of 72,000 pulses by use of a Pyrromethene disk.

3.
Appl Opt ; 41(33): 7006-11, 2002 Nov 20.
Article in English | MEDLINE | ID: mdl-12463245

ABSTRACT

We have investigated laser action in a binary mixture of dyes, Rh-6G and DCM, resulting in tunable laser emission over an extended frequency region. The two dyes absorb the same pump radiation but fluoresce over frequency ranges that are shifted with respect to each other, thereby resulting in extended tunability. Following a time-dependent analysis of a rate-equation model that describe the operation of such a laser, theoretical estimates for optimum dye concentrations and the corresponding extension of the laser tuning range have been obtained.

4.
Appl Opt ; 41(9): 1704-13, 2002 Mar 20.
Article in English | MEDLINE | ID: mdl-11921799

ABSTRACT

The performance of a copper vapor laser-pumped narrow-band dye laser in oscillator-amplifier configuration with water-based binary mixture solvents is described. Although oscillator efficiency in water-surfactant (sodium lauryl sulfate) solvent was comparable with that that employed pure ethanolic solvent, amplifier efficiency was found to be lower. Experiments that were carried out with vertically polarized pump beams and either horizontally or vertically polarized signal beams show that, in case of both the pump and signal having orthogonal polarization (horizontal) and same polarization (vertical), the extraction efficiency for both ethanolic and water-micelle media increased substantially from 15.7% to 18.5% and from 10% to 12.5%, respectively. However, the relative difference remained nearly the same, indicating that a slower orientational diffusion of excited dye molecules in a micellar medium is not responsible for a decrease in amplifier efficiency. Amplifier efficiency comparable with that containing ethanolic dye solutions could be obtained with a binary solvent that comprises a mixture of water and about 30% n-propanol. The performances of two efficient dyes, Rhodamine-6G and Kiton Red S, using water-based solvents were studied.

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