ABSTRACT
Topological photonics has emerged recently as a smart approach for realizing robust optical circuitry, and the study of nonlinear effects is expected to open the door for tunability of photonic topological states. Here we realize experimentally nonlinearity-induced spectral tuning of electromagnetic topological edge states in arrays of coupled nonlinear resonators in the pump-probe regime. When nonlinearity is weak, we observe that the frequencies of the resonators exhibit spectral shifts concentrated mainly at the edge mode and affecting only weakly the bulk modes. For a strong pumping, we describe several scenarios of the transformation of the edge states and their hybridization with bulk modes, and also predict a parametrically driven transition from topological stationary to unstable dynamic regimes.
ABSTRACT
Optical activity is a fundamental phenomenon originating from the chiral nature of crystals and molecules. While intrinsic chiroptical responses of ordinary chiral materials to circularly polarized light are relatively weak, they can be enhanced by specially tailored nanostructures. Here, nanorod metamaterials, comprising a dense array of vertically aligned gold nanorods, is shown to provide a significant enhancement of the circular dichroism response of an embedded material. A nanorod composite, acting as an artificial uniaxial crystal, is filled with chiral mercury sulfide nanocrystals embedded in a transparent polymer. The metamaterial, being inherently achiral, enables optical activity enhancement or suppression. Unique properties of inherently achiral structures to tailor optical activities pave a way for flexible characterization of optical activity of molecules and nanocrystal-based compounds.
