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1.
Phys Rev Lett ; 128(18): 187202, 2022 May 06.
Article in English | MEDLINE | ID: mdl-35594098

ABSTRACT

We report experimental verification of the recently predicted collective modes of spinons, stabilized by backscattering interaction, in a model quantum spin chain material. We exploit the unique geometry of uniform Dzyaloshinskii-Moriya interactions in K_{2}CuSO_{4}Br_{2} to measure the interaction-induced splitting between the two components of the electron spin resonance (ESR) response doublet. From that we directly determine the magnitude of the "marginally irrelevant" backscattering interaction between spinons for the first time.

2.
Phys Rev Lett ; 126(22): 227201, 2021 Jun 04.
Article in English | MEDLINE | ID: mdl-34152175

ABSTRACT

We investigate the amplitude (Higgs) mode associated with longitudinal fluctuations of the order parameter at the continuous spontaneous symmetry breaking phase transition. In quantum magnets, due to the fast decay of the amplitude mode into low-energy Goldstone excitations, direct observation of this mode represents a challenging task. By focusing on a quasi-one-dimensional geometry, we circumvent the difficulty and investigate the amplitude mode in a system of weakly coupled spin chains with the help of quantum Monte Carlo simulations, stochastic analytic continuation, and a chain-mean field approach combined with a mapping to the field-theoretic sine-Gordon model. The amplitude mode is observed to emerge in the longitudinal spin susceptibility in the presence of a weak symmetry-breaking staggered field. A conventional measure of the amplitude mode in higher dimensions, the singlet bond mode, is found to appear at a lower than the amplitude mode frequency. We identify these two excitations with the second (first) breather of the sine-Gordon theory, correspondingly. In contrast to higher-dimensional systems, the amplitude and bond order fluctuations are found to carry significant spectral weight in the quasi-1D limit.

3.
Phys Rev Lett ; 125(18): 187201, 2020 Oct 30.
Article in English | MEDLINE | ID: mdl-33196249

ABSTRACT

We study the transverse dynamical susceptibility of an antiferromagnetic spin-1/2 chain in the presence of a longitudinal Zeeman field. In the low magnetization regime in the gapless phase, we show that the marginally irrelevant backscattering interaction between the spinons creates a nonzero gap between two branches of excitations at small momentum. We further demonstrate how this gap varies upon introducing a second neighbor antiferromagnetic interaction, vanishing in the limit of a noninteracting "spinon gas." In the high magnetization regime, as the Zeeman field approaches the saturation value, we uncover the appearance of two-magnon bound states in the transverse susceptibility. This bound state feature generalizes the one arising from string states in the Bethe ansatz solution of the integrable case. Our results are based on numerically accurate, unbiased matrix-product-state techniques as well as analytic approximations.

4.
Phys Rev Lett ; 120(3): 037204, 2018 Jan 19.
Article in English | MEDLINE | ID: mdl-29400534

ABSTRACT

We describe electron spin resonance in a quantum spin liquid with significant spin-orbit coupling. We find that the resonance directly probes spinon continuum, which makes it an efficient and informative probe of exotic excitations of the spin liquid. Specifically, we consider spinon resonance of three different spinon mean-field Hamiltonians, obtained with the help of projective symmetry group analysis, which model a putative quantum spin liquid state of the triangular rare-earth antiferromagnet YbMgGaO_{4}. The band of absorption is found to be very broad and exhibit strong van Hove singularities of single spinon spectrum as well as pronounced polarization dependence.

5.
Phys Rev Lett ; 116(17): 177201, 2016 Apr 29.
Article in English | MEDLINE | ID: mdl-27176535

ABSTRACT

We propose a universal nonlinear sigma model field theory for one-dimensional frustrated ferromagnets, which applies in the vicinity of a "quantum Lifshitz point," at which the ferromagnetic state develops a spin wave instability. We investigate the phase diagram resulting from perturbations of the exchange and of magnetic field away from the Lifshitz point, and uncover a rich structure with two distinct regimes of different properties, depending upon the value of a marginal, dimensionless, parameter of the theory. In the regime relevant for one-dimensional systems with low spin, we find a metamagnetic transition line to a vector chiral phase. This line terminates in a critical end point, beyond which there is at least one multipolar or "spin nematic" phase. We show that the field theory is asymptotically exactly soluble near the Lifshitz point.

6.
Rep Prog Phys ; 78(5): 052502, 2015 May.
Article in English | MEDLINE | ID: mdl-25892088

ABSTRACT

We review ground states and excitations of a quantum antiferromagnet on triangular and other frustrated lattices. We pay special attention to the combined effects of magnetic field h, spatial anisotropy R and spin magnitude S. The focus of the review is on the novel collinear spin density wave and spin nematic states, which are characterized by fully gapped transverse spin excitations with S(z) = ± 1. We discuss extensively the R - h phase diagram of the antiferromagnet, both in the large-S semiclassical limit and the quantum S = 1/2 limit. When possible, we point out connections with experimental findings.

7.
Phys Rev Lett ; 113(8): 087204, 2014 Aug 22.
Article in English | MEDLINE | ID: mdl-25192123

ABSTRACT

We consider 2D Heisenberg antiferromagnets on a triangular lattice with spatially anisotropic interactions in a high magnetic field close to the saturation. We show that this system possesses a rich phase diagram in a field or anisotropy plane due to competition between classical and quantum orders: an incommensurate noncoplanar spiral state, which is favored classically, and a commensurate coplanar state, which is stabilized by quantum fluctuations. We show that the transformation between these two states is highly nontrivial and involves two intermediate phases--the phase with coplanar incommensurate spin order and the one with noncoplanar double-Q spiral order. The transition between the two coplanar states is of commensurate-incommensurate type, not accompanied by softening of spin-wave excitations. We show that a different sequence of transitions holds in triangular antiferromagnets with exchange anisotropy, such as Ba(3)CoSb(2)O(9).

8.
Phys Rev Lett ; 110(21): 217210, 2013 May 24.
Article in English | MEDLINE | ID: mdl-23745926

ABSTRACT

We analyze instabilities of the collinear up-up-down state of a two-dimensional quantum spin-S spatially anisotropic triangular lattice antiferromagnet in a magnetic field. We find, within the large-S approximation, that near the end point of the plateau, the collinear state becomes unstable due to the condensation of two-magnon bound pairs rather than single magnons. The two-magnon instability leads to a novel two-dimensional vector chiral phase with alternating spin currents but no magnetic order in the direction transverse to the field. This phase breaks a discrete Z(2) symmetry but preserves a continuous U(1) one of rotations about the field axis. It possesses orbital antiferromagnetism and displays a magnetoelectric effect.

9.
Phys Rev Lett ; 102(13): 137201, 2009 Apr 03.
Article in English | MEDLINE | ID: mdl-19392397

ABSTRACT

We consider the phase diagram of a spatially anisotropic 2D triangular antiferromagnet in a magnetic field. Classically, the ground state is umbrellalike for all fields, but we show that the quantum phase diagram is much richer and contains a 1/3-magnetization plateau, two commensurate planar states, two incommensurate chiral umbrella phases, and, possibly, a spin density wave state separating the two chiral phases. Our analysis sheds light on several recent experimental findings for Cs2CuBr4.

10.
Phys Rev Lett ; 100(15): 156402, 2008 Apr 18.
Article in English | MEDLINE | ID: mdl-18518133

ABSTRACT

We investigate interactions between spins of strongly correlated electrons subject to the spin-orbit interaction. Our main finding is that of a novel, spin-orbit mediated anisotropic spin-spin coupling of the van der Waals type. Unlike the standard exchange, this interaction does not require the wave functions to overlap. We argue that this ferromagnetic interaction is important in the Wigner crystal state where the exchange processes are severely suppressed. We also comment on the anisotropy of the exchange between spins mediated by the spin-orbital coupling.

11.
Phys Rev Lett ; 98(12): 126408, 2007 Mar 23.
Article in English | MEDLINE | ID: mdl-17501145

ABSTRACT

We present analysis of the interacting quantum wire problem in the presence of magnetic field and spin-orbit interaction. We show that an interesting interplay of Zeeman and spin-orbit terms, facilitated by the electron-electron interaction, results in the spin-density wave state when the magnetic field and spin-orbit axes are orthogonal. This strongly affects charge transport through the wire: With the spin-density wave stabilized, single-particle backscattering off a nonmagnetic impurity becomes irrelevant. The sensitivity of the effect to the direction of the magnetic field can be used for experimental verification of this proposal.

12.
Phys Rev Lett ; 98(7): 077205, 2007 Feb 16.
Article in English | MEDLINE | ID: mdl-17359057

ABSTRACT

We investigate the phase diagram of the anisotropic spin-1/2 triangular lattice antiferromagnet, with interchain diagonal exchange J' much weaker than the intrachain exchange J. We find that fluctuations lead to a competition between (commensurate) collinear antiferromagnetic and (zigzag) dimer orders. Both states differ in symmetry from the spiral order known to occur for larger J', and are therefore separated by quantum phase transitions from it. The zero-field collinear antiferromagnet is succeeded in a magnetic field by magnetically ordered spin-density-wave and cone phases, before reaching the fully polarized state. Implications for the anisotropic triangular magnet Cs2CuCl4 are discussed.

13.
Phys Rev Lett ; 93(12): 127202, 2004 Sep 17.
Article in English | MEDLINE | ID: mdl-15447302

ABSTRACT

We investigate the spatially anisotropic square lattice quantum antiferromagnet. The model describes isotropic spin-1/2 Heisenberg chains (exchange constant J) coupled antiferromagnetically in the transverse (J( perpendicular )) and diagonal (J(x)), with respect to the chain, directions. Classically, the model admits two ordered ground states-with antiferromagnetic and ferromagnetic interchain spin correlations-separated by a first-order phase transition at J( perpendicular )=2J(x). We show that in the quantum model this transition splits into two, revealing an intermediate quantum-disordered columnar dimer phase, both in two dimensions and in a simpler two-leg ladder version. We describe quantum-critical points separating this spontaneously dimerized phase from classical ones.

14.
Phys Rev Lett ; 88(16): 167203, 2002 Apr 22.
Article in English | MEDLINE | ID: mdl-11955258

ABSTRACT

Using the random phase approximation, we show that a crossed-chains model of spin-1/2 Heisenberg chains with frustrated interchain couplings has a nondimerized spin-liquid ground state in 2D, with deconfined spinons as the elementary excitations. The results are confirmed by a bosonization study, which shows that the system is an example of a "sliding Luttinger liquid." In an external field, the system develops an incommensurate field-induced long-range order with a finite transition temperature.

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