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1.
Opt Express ; 29(4): 5982-5992, 2021 Feb 15.
Article in English | MEDLINE | ID: mdl-33726129

ABSTRACT

Extreme ultraviolet (XUV) radiation finds numerous applications in spectroscopy. When the XUV light is generated via high-order harmonic generation (HHG), it may be produced in the form of attosecond pulses, allowing access to unprecedented ultrafast phenomena. However, the HHG efficiency remains limited. Here we present an observation of a new regime of coherent XUV emission which has a potential to provide higher XUV intensity, vital for applications. We explain the process by high-order parametric generation, involving the combined emission of THz and XUV photons, where the phase matching is very robust against ionization. This introduces a way to use higher-energy driving pulses, thus generating more XUV photons.

2.
Sci Adv ; 5(4): eaau7175, 2019 Apr.
Article in English | MEDLINE | ID: mdl-30972360

ABSTRACT

By experimentally studying high-order harmonic beams generated in gases, we show how the spatial characteristics of these ultrashort extreme-ultraviolet (XUV) beams can be finely controlled when a single fundamental beam generates harmonics in a thin gas medium. We demonstrate that these XUV beams can be emitted as converging beams and thereby get focused after generation. We study this optics-less focusing using a spatially chirped beam that acts as a probe located inside the harmonic generation medium. We analyze the XUV beam evolution with an analytical model and obtain very good agreement with experimental measurements. The XUV foci sizes and positions vary strongly with the harmonic order, and the XUV waist can be located at arbitrarily large distances from the generating medium. We discuss how intense XUV fields can be obtained with optics-less focusing and how the order-dependent XUV beam characteristics are compatible with broadband XUV irradiation and attosecond science.

3.
Opt Express ; 26(12): 15745-15758, 2018 Jun 11.
Article in English | MEDLINE | ID: mdl-30114831

ABSTRACT

We have studied high-order harmonic generation (HHG) in an indium ablation plume driven by intense few-cycle laser pulses centered at 775 nm as a function of the frequency chirp of the laser pulse. We found experimentally that resonant emission lines between 19.7 eV and 22.3 eV (close to the 13th and 15th harmonic of the laser) exhibit a strong, asymmetric chirp dependence, with pronounced intensity modulations. The chirp dependence is reproduced by our numerical time-dependent Schrödinger equation simulations of a resonant HHG by the model indium ion. As demonstrated with our separate simulations of HHG within the strong field approximation, the resonance can be understood in terms of the chirp-dependent HHG photon energy coinciding with the energy of an autoionizing state to ground state transition with high oscillator strength. This supports the validity of the general theory of resonant four-step HHG in the few-cycle limit.

4.
Phys Rev Lett ; 121(2): 023201, 2018 Jul 13.
Article in English | MEDLINE | ID: mdl-30085730

ABSTRACT

High harmonics from laser-ablated plumes are mostly generated from ionic species. We demonstrate that with ultrashort infrared (∼1.82 µm) driving lasers, high harmonics from laser-ablated manganese are predominantly generated from neutral atoms, a transition metal atom with an ionization potential of 7.4 eV. Our results open the possibility to advance laser-ablation technique to study the dynamics of neutral atoms of low ionization potential. Moreover, as manganese contains giant autoionizing resonance, intense and broadband high harmonics have been demonstrated from this resonance at energies from 49 to 53 eV. This opens the possibility to generate intense attosecond pulses directly from the giant resonances, as well as to study these resonances using high-harmonic spectroscopy.

5.
Opt Express ; 25(18): 21068-21083, 2017 Sep 04.
Article in English | MEDLINE | ID: mdl-29041515

ABSTRACT

We theoretically analyze the phase-matching of high-order harmonic generation (HHG) in multi-jet plasmas and find the harmonic orders for which the quasi-phase-matching (QPM) is achieved depending on the parameters of the plasma and the generating beam. HHG by single- and two-color generating fields is analyzed. The QMP is studied experimentally for silver, indium and manganese plasmas using near IR and mid-IR laser fields. The theory is validated by comparison with our experimental observations, as well as published experimental data. In particular, the plasma densities and the harmonic phase coefficients reconstructed from the observed harmonic spectra using our theory agree with the corresponding parameters found using other methods. Our theory allows defining the plasma jet and the generating field properties, which can maximize the HHG efficiency due to QPM.

6.
Nat Commun ; 8: 16061, 2017 07 17.
Article in English | MEDLINE | ID: mdl-28714468

ABSTRACT

In high-order harmonic generation, resonant harmonics (RH) are sources of intense, coherent extreme-ultraviolet radiation. However, intensity enhancement of RH only occurs for a single harmonic order, making it challenging to generate short attosecond pulses. Moreover, the mechanism involved behind such RH was circumstantial, because of the lack of direct experimental proofs. Here, we demonstrate the exact quantum paths that electron follows for RH generation using tin, showing that it involves not only the autoionizing state, but also a harmonic generation from dressed-AIS that appears as two coherent satellite harmonics at frequencies ±2Ω from the RH (Ω represents laser frequency). Our observations of harmonic emission from dressed states open the possibilities of generating intense and broadband attosecond pulses, thus contributing to future applications in attosecond science, as well as the perspective of studying the femtosecond and attosecond dynamics of autoionizing states.

7.
Nat Commun ; 5: 4637, 2014 Aug 13.
Article in English | MEDLINE | ID: mdl-25115933

ABSTRACT

A large international effort is nowadays devoted to increase the energy of the extreme ultraviolet pulses by using high-peak power ultrashort fundamental pulses (Terawatt level). Using such fundamental pulses brings specific constraints that need to be addressed. Here we study high-order harmonic generation in gases with 10 fs pulses at Terawatt peak power and demonstrate that extreme ultraviolet beams can be highly structured and complex in various conditions. We use a single-shot spatially resolved spectral detection and demonstrate direct observation of the spatio-temporal coupling occurring in the generating medium. Clear and reproducible complex spatio-spectral structures are observed in the far field. Similar structures are reproduced with simulations and we show that they are intimately associated to the high nonlinearity of high-order harmonic generation. Those findings are of prime importance for the generation of high-energy attosecond pulses and reveal important issues for their applications.

8.
Opt Express ; 22(6): 6239-48, 2014 Mar 24.
Article in English | MEDLINE | ID: mdl-24663972

ABSTRACT

We present an all optical approach to measure the value of the carrier-envelope phase (CEP) of a short intense laser pulse. This method relies on photo-ionization of gases with a guided laser beam. This approach that provides the absolute value of the CEP, is compatible with single shot characterization, is scalable in wavelength, does not suffer from bandwidth limitation and is largely intensity independent. It has also the potential to provide a full characterization of the pulse profile via high order autocorrelation on a single shot basis.

9.
Anesteziol Reanimatol ; (5): 51-5, 2013.
Article in Russian | MEDLINE | ID: mdl-24624859

ABSTRACT

UNLABELLED: Extracorporeal life support (ECLS) is used in pediatric patients with ARDS in recent 20 years with survival rate from 50 to 67% Venovenous ECLS was used in 1 year 2 months old patient with ARDS and pneumonia developed in postoperative period after gastral esophagoplasty. Purposes of ECLS use were stabilization child's condition and normalization of gas composition of blood with relative lungs repose. Indications for ECLS were increasing respiratory failure, hypoxemia, low respiratory index (PaO2/FiO2 ratio 47.3), alveolar-arterial gradient of oxygen (A-aDO) 630 mmHg and absence of positive effect from high frequency oscillation (HFO). MATERIALS AND METHODS: ECLS was used in 1 year 2 months old patient with ARDS and bilateral pneumonia developed in postoperative period after gastral esophagoplasty. Deltasteam system (Medos Medizintechnik AG, Germany) with centrifugal pump and servoregulation of blood flow pressure was used for ECLS. Double-lumen cannula with size 12 French was used ECLS was instituted via right internal jugular vein. RESULTS: The patient did not have expressed heart failure. Thus preference was given to venovenous ECLS and not to venoarterial ECLS. Duration of ECLS use was 72 hours. Auscultation parameters and gas exchange improved haemodynamics stabilized parameters of biochemical and haematological analysis normalized and the dynamics x-ray examination was positive after the ECLS use. Patient was decannulated and extubated. CONCLUSIONS: Venovenous ECLS was an only way of life support in child with heavy ARDS and pneumonia developed in postoperative period More observations are needed for more thorough analysis and recommendations.


Subject(s)
Extracorporeal Membrane Oxygenation/methods , Hemofiltration/methods , Pneumonia/therapy , Postoperative Complications/therapy , Respiratory Distress Syndrome/therapy , Esophagoplasty , Female , Humans , Infant , Pneumonia/complications , Pneumonia/diagnosis , Postoperative Complications/etiology , Respiratory Distress Syndrome/complications , Respiratory Distress Syndrome/diagnosis , Treatment Outcome
10.
Opt Express ; 20(5): 5196-203, 2012 Feb 27.
Article in English | MEDLINE | ID: mdl-22418325

ABSTRACT

We investigate theoretically the high-order harmonic generation (HHG) by two orthogonally-polarized linearly chirped laser pulses. We show that such generating field has a specific temporal variation of the ellipticity which provides generation of two XUV attosecond pulses with tunable delay between them. This delay is controlled by the delay between the two generating pulses. Perspectives of application of this technique for the attosecond pump - attosecond probe experiments are discussed.


Subject(s)
Lasers , Computer-Aided Design , Equipment Design , Equipment Failure Analysis , Signal Processing, Computer-Assisted
11.
Phys Rev Lett ; 107(4): 043902, 2011 Jul 22.
Article in English | MEDLINE | ID: mdl-21867007

ABSTRACT

We investigate numerically and analytically the polarization properties of high-order harmonics generated by an atom in intense elliptically polarized laser field. The offset angle of the harmonic polarization ellipse can be well described with the semiclassic "simple-man" high-harmonic generation model. The harmonic ellipticity itself, however, can be hardly understood within this model. We show that this ellipticity originates from quantum-mechanical uncertainty of the electron motion. We develop a theoretical approach describing this ellipticity and, more generally, the time evolution of the high-harmonic polarization state within the laser cycle. The analytical results are verified with the exact numerical solution; to make the comparison accurately, we develop a specific technique for separating the contributions of quantum paths in the numerical calculation.

12.
Phys Rev Lett ; 104(12): 123901, 2010 Mar 26.
Article in English | MEDLINE | ID: mdl-20366535

ABSTRACT

We suggest a high-order harmonic generation (HHG) model describing enhancement of the generation efficiency for the harmonic resonant with the transition between the ground and autoionizing state of the generating ion. The results of numerical and analytical calculations based on this model are in good quantitative agreement with the experiments showing HHG enhancement up to 2 orders of magnitude. Moreover, this model reproduces well the essential difference in HHG efficiency for different ions. We show that intense but relatively long attosecond pulses can be generated using the enhanced harmonics.

13.
Biofizika ; 46(5): 807-10, 2001.
Article in Russian | MEDLINE | ID: mdl-11605374

ABSTRACT

The dynamics of the system with a determined chaotic behavior (Lorentz system) was studied by comparing the histograms. It was shown that the dynamics of the system exhibits phenomena similar to those observed in studies of fluctuations in physical systems. In particular, upon comparison of histograms constructed from different time intervals, the "near zone" effect makes itself evident. It was shown that a very slight modulation of only one parameter of the system leads to a change in behavior.


Subject(s)
Models, Theoretical , Nonlinear Dynamics , Physical Phenomena , Physics , Statistical Distributions
15.
Akush Ginekol (Mosk) ; (12): 46-7, 1989 Dec.
Article in Russian | MEDLINE | ID: mdl-2629523

ABSTRACT

Long-term outcomes of stratifying cervicoplasty for organic isthmic-cervical incompetence have been evaluated in 38 women. Pregnancy was achieved in 32 women and continued to term in 22 women; there were 16 cesarean deliveries, and 6 women were delivered vaginally despite recommended operative delivery. Spontaneous abortions occurred in 5 surgically treated women and abortion was induced in 5. Reversal of secondary cervical disease represents an advantage of this mode of treatment.


Subject(s)
Abortion, Habitual/surgery , Uterine Cervical Incompetence/surgery , Abortion, Habitual/epidemiology , Abortion, Habitual/etiology , Adult , Cervix Uteri/surgery , Female , Follow-Up Studies , Humans , Pregnancy , Uterine Cervical Incompetence/complications
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